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Zirconium-catalyzed heterodehydrocoupling of primary phosphines with silanes and germanes.

Authors :
Roering AJ
MacMillan SN
Tanski JM
Waterman R
Source :
Inorganic chemistry [Inorg Chem] 2007 Aug 20; Vol. 46 (17), pp. 6855-7. Date of Electronic Publication: 2007 Jul 25.
Publication Year :
2007

Abstract

Triamidoamine-supported zirconium complexes catalyze the heterodehydrocoupling of primary phosphines with silane and germanes. In this catalysis, P-Si or P-Ge products are observed exclusively with no competitive P-P bond formation. Phosphido complexes (N3N)ZrPHR (N3N = N(CH2CH2NSiMe3)33-, R = Ph, 2; Cy, 3) were observed to be the catalyst resting state, and complex 2 was structurally characterized.

Details

Language :
English
ISSN :
0020-1669
Volume :
46
Issue :
17
Database :
MEDLINE
Journal :
Inorganic chemistry
Publication Type :
Academic Journal
Accession number :
17649993
Full Text :
https://doi.org/10.1021/ic7013144