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Di-2-pyridyl ketone oxime in copper chemistry: di-, tri-, penta- and hexanuclear complexes.

Authors :
Afrati T
Zaleski CM
Dendrinou-Samara C
Mezei G
Kampf JW
Pecoraro VL
Kessissoglou DP
Source :
Dalton transactions (Cambridge, England : 2003) [Dalton Trans] 2007 Jul 07 (25), pp. 2658-68. Date of Electronic Publication: 2007 Apr 24.
Publication Year :
2007

Abstract

The use of di-2-pyridyl ketone oxime (Hpko)/X- "blends" (X- = OH-, Cl-, ClO4-) in copper chemistry has yielded neutral binuclear and cationic trinuclear, pentanuclear or hexanuclear complexes. Various synthetic procedures have led to the synthesis of compounds [Cu5(pko)7].[ClO4]3.2CH3OH.2H2O (1), [Cu3(pko)3(OH)(Cl)]2[Ph4B]2.4DMF.2H2O (2), [Cu2(pko)4] (3), {[Cu6(pko)6ClO4(CH3CN)6][Cu6(pko)6(ClO4)3(CH3CN)4]}.8ClO4.14CH3CN.H2O (4). The structures of the complexes have been determined by single-crystal X-ray crystallography.

Details

Language :
English
ISSN :
1477-9226
Issue :
25
Database :
MEDLINE
Journal :
Dalton transactions (Cambridge, England : 2003)
Publication Type :
Academic Journal
Accession number :
17576491
Full Text :
https://doi.org/10.1039/b700902j