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Particulate matter source apportionment in a village situated in industrial region of Central Europe.

Authors :
Pokorná, P.
Hovorka, J.
Kroužek, J.
Hopke, P.K.
Source :
Journal of the Air & Waste Management Association (Taylor & Francis Ltd). Dec2013, Vol. 63 Issue 12, p1412-1421. 10p.
Publication Year :
2013

Abstract

The bilinear receptor model positive matrix factorization (PMF) was used to apportion particulate matter with an aerodynamic diameter of 1–10 μm (PM1–10) sources in a village, Březno, situated in an industrial region of northern Bohemia in Central Europe. The receptor model analyzed the data sets of 90- and 60-min integrations of PM1–10mass concentrations and elemental composition for 27 elements. The 14-day sampling campaigns were conducted in the village in summer 2008 and winter 2010. Also, to ensure seasonal and regional representativeness of the data sets recorded in the village, the spatial-temporal variability of the 24-hr PM10and PM1–10within 2008–2010 in winter and summer across the multiple sites was evaluated. There were statistically significant interseasonal differences of the 24-hr PM data, but not intrasummer or intrawinter differences of the 24-hr PM1–10data across the multiple sites. PMF resolved seven sources of PM1–10. They were high-temperature coal combustion; combustion in local heating boilers; marine aerosol; mineral dust; primary biological/wood burning; road dust, car brakes; and gypsum. The main summer factors were assigned to mineral dust (38.2%) and primary biological/wood burning (33.1%). In winter, combustion factors dominated (80%) contribution to PM1–10. The conditional probability function (CPF) helped to identified local sources of PM1–10. The source of marine aerosol from the North Sea and English Channel was indicated by the Hybrid Single Particle Lagrangian Integrated Trajectory Model (HYSPLIT). [ABSTRACT FROM PUBLISHER]

Details

Language :
English
ISSN :
10962247
Volume :
63
Issue :
12
Database :
Academic Search Index
Journal :
Journal of the Air & Waste Management Association (Taylor & Francis Ltd)
Publication Type :
Academic Journal
Accession number :
93632331
Full Text :
https://doi.org/10.1080/10962247.2013.825215