Surface air concentration and deposition of lead-210 in French Guiana: two years of continuous monitoring

To make up for the lack of data on 210Pb aerosol deposition in tropical regions and to use this radionuclide as an aerosol tracer, a monitoring station was run for two years at Petit-Saut, French Guiana. Lead-210 concentration in air at ground level was monitored continuously together with atmospheric total deposition. The air concentration has a mean value of 0.23±0.02 mBq m−3 during both wet and dry seasons, and it is only weakly affected by the precipitation mechanism. This result was unexpected in a wet tropical region, with a high precipitation rate. In contrast, deposition clearly correlates with precipitation for low/moderate rainfall (<15 cm per 15-day), while this correlation is masked by strong fluctuations at high rainfall. The estimated mean annual deposition over the last ten years is 163±75 Bq m−2 y−1. This provides a procedure for estimating this mean flux at other sites in French Guiana. [Copyright &y& Elsevier]