Low-Temperature Sintering and Electric Properties of Pb0.99( Zr0.95 Ti0.05)0.98 Nb0.02 O3 Ferroelectric Ceramics with CuO Additive.

The low-temperature sintering and electric properties of Pb0.99( Zr0.95 Ti0.05)0.98 Nb0.02 O3 ( PZTN 95/5) ferroelectric ceramics with CuO addition was investigated. The CuO addition significantly promoted the densification and reduced the sintering temperature of PZTN 95/5 ceramics by more than 200°C. The 0.2 wt% CuO-added sample sintered at 1150°C exhibited the optimum relative density of 96.7% and excellent electric properties with values of Pr = 37.80 μC/cm2, TC = 223°C, εr = 329, and tan δ = 0.016, which were superior to that of PZTN 95/5 ceramics sintered at 1350°C. [ABSTRACT FROM AUTHOR]