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Bulky Trialkylsilyl Acetylene in the Cadiot—Chodkiewicz Cross-Coupling Reaction.

Authors :
Marino, Joseph P.
Hanh Nho Nguyen
Source :
Journal of Organic Chemistry. 9/20/2002, Vol. 67 Issue 19, p6841. 4p. 2 Diagrams, 2 Charts.
Publication Year :
2002

Abstract

Bulky trialkylsilyl-protected alkynes such as triethylsilyl (TES), tert-butyldimethylsilyl (TBS), and triisopropylsilyl (TIPS) acetylenes underwent the CadiotChodkiewicz cross-coupling reaction with different bromoalkynes to form a variety of synthetically useful unsymmetrical diynes in good yields. The diyne alcohol 10 was transformed regio- and stereo-selectively into enynes by hydrotelluration, carbometalation, and reduction reactions. [ABSTRACT FROM AUTHOR]

Subjects

Subjects :
*ACETYLENE compounds
*ALKYNES

Details

Language :
English
ISSN :
00223263
Volume :
67
Issue :
19
Database :
Academic Search Index
Journal :
Journal of Organic Chemistry
Publication Type :
Academic Journal
Accession number :
7551918
Full Text :
https://doi.org/10.1021/jo025745x