Phase separation and enhanced magnetoresistance in the strained epitaxial La0.625Ca0.375MnO3 (001) films.

La0.625Ca0.375MnO3 films have been epitaxially grown on the (LaAlO3)0.3(Sr2AlTaO6)0.35 (001) substrates at different oxygen pressures and show varying tetragonal distortion. Results indicate a tendency that larger tetragonal distortion can stabilize the antiferromagnetic-insulator phase in the thin films. Colossal magnetoresistance (CMR) and anisotropic magnetoresistance (AMR) have been greatly enhanced only in the strained films over a broad temperature, probably responding to the anisotropic fluctuation of the nanoscale orientation-ordered patterns near the temperature of the phase separation region or metal-insulator transition. Hence, the inhomogeneous phase competition may contribute to the CMR and the extraordinary AMR effect for manganite devices. [ABSTRACT FROM AUTHOR]