Synthesis of some new 1-acyl-5-aryl-3-(5-methyl-1- p-tolyl-1 H-1,2,3-triazol-4-yl)-4,5-dihydro-1 H-pyrazole.

Some new compounds ( E)-3-aryl-1-(5-methyl-1- p-tolyl-1 H-1,2,3-triazol-4-yl)-prop-2-en-1-ones 5a-e were prepared by 1-(5-methyl-1- p-tolyl-1 H-1,2,3-triazol-4-yl)-ethanone and various aromatic aldehydes. Then one pot reaction was happened by compounds 5a-e with hydrazine hydrate in acetic acid or propionic acid, respectively, to give the title compounds 1acyl-5-aryl-3-(5-methyl-1- p-tolyl-1 H-1,2,3-triazol-4-yl)-4,5-dihydro-1 H-pyrazoles 6a-i. All structures were established by MS, IR, CHN, 1H-NMR and 13C-NMR spectral data. J. Heterocyclic Chem., (2012). [ABSTRACT FROM AUTHOR]