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Air- and Water-Stable Catalysts for Hydroamination/Cyclization. Synthesis and Application of CCC−NHC Pincer Complexes of Rh and Ir.

Authors :
Eike B. Bauer
G. T. Senthil Andavan
T. Keith Hollis
Ramel J. Rubio
Joon Cho
Glenn R. Kuchenbeiser
Theodore R. Helgert
Christopher S. Letko
Fook S. Tham
Source :
Organic Letters. Mar2008, Vol. 10 Issue 6, p1175-1178. 4p.
Publication Year :
2008

Abstract

The scope of CCC−NHC pincer complex synthetic methodology by metalation/transmetalation has been extended to Ir. Structural characterization revealed that it is isomorphous with the Rh complex. Both Rh and Ir complexes are efficient catalysts for the hydroamination/cyclization of secondary amines in the presence of air and/or water. [ABSTRACT FROM AUTHOR]

Details

Language :
English
ISSN :
15237060
Volume :
10
Issue :
6
Database :
Academic Search Index
Journal :
Organic Letters
Publication Type :
Academic Journal
Accession number :
32793682
Full Text :
https://doi.org/10.1021/ol8000766