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Crafting in situ boron and selenium-doped carbon nitride nanosheets for turbocharged benzaldehyde to benzyl alcohol under solar spectrum.
- Source :
-
Diamond & Related Materials . Jun2024, Vol. 146, pN.PAG-N.PAG. 1p. - Publication Year :
- 2024
-
Abstract
- This research focuses on the fabrication and application of in situ boron and selenium-doped carbon nitride nanosheets as effective photocatalysts using sun spectrum irradiation to convert turbocharged benzaldehyde to benzyl alcohol. To optimize the doping method for enhanced activity, the effect of changing dopant concentrations on catalytic efficiency was thoroughly investigated. Furthermore, a through analysis of the reactive species involved in the conversion process helped to clarify the photocatalytic process. Based on charge transfer and low recombination, the results indicate that boron and selenium dopants work synergistically to improve catalytic efficiency. This research helps to improve the development of new photocatalytic materials for the sustainable and ecologically friendly transformation of organic molecules under solar spectrum irradiation. The regeneration of NADH using B,Se-CN photocatalyst demonstrates very good efficiency. It also demonstrated the high conversion efficiency of benzaldehyde to benzyl alcohol. This study emphasizes the possible use of B,Se-CN composite in the area of photoinduced conversion-based organic transformation. The knowledge gathered from this research opens up new avenues for the development and enhancement of effective photocatalysts that might be used in a range of solar-powered organic transformation processes. [Display omitted] • B,Se-CN photocatalyst was synthesis via two-step process through thermal polycondensation of M, B and SU. • The light harvesting photocatalyst had the capacity to photo-regenerate the 1,4 NADH and bio-transformation. • The synthesized photocatalyst potential as stable catalyst for production of 1,4 NADH (yield and benzyl alcohol. • Demonstrated synergistic enhancement of catalytic efficiency by dopants, contributing to sustainable alcohol formation. [ABSTRACT FROM AUTHOR]
Details
- Language :
- English
- ISSN :
- 09259635
- Volume :
- 146
- Database :
- Academic Search Index
- Journal :
- Diamond & Related Materials
- Publication Type :
- Academic Journal
- Accession number :
- 177847908
- Full Text :
- https://doi.org/10.1016/j.diamond.2024.111140