High Q chiroptical responses with maximum chirality in all-dielectric metasurfaces driven by quasi-bound states in the continuum.

Chiral metasurfaces have attracted considerable attention because of their immense potential for diverse applications requiring chiral light-matter interactions. Recently, boosted by a mechanism based on the concept of bound states in the continuum (BICs), high Q factor chiroptical resonances have been exhibited by breaking the inversion symmetries of planar metasurfaces. However, the optical chirality of these chiral metasurfaces is generally intolerable with respect to the structural geometries, especially the geometric asymmetry. Here, we present a novel chiral quasi-BIC with strong optical chirality in an all-dielectric metasurface. By simultaneously breaking the in-plane C 2 rotational and mirror symmetries, the chiral metasurface shows enhanced chiroptical resonances with near-unity CD (∼0.996) and high Q factors (∼2274) at terahertz frequencies. Further analyses based on numerical simulations reveal that the CD of the chiroptical resonance depicts exceptional remarkable tolerableness to the geometry asymmetry δ when δ are present in a broad range, while the corresponding Q factor is modulated accordingly. The results may develop a novel approach to manipulating the advanced optical chirality for potential applications requiring strong CD with enhanced light-matter interactions. [ABSTRACT FROM AUTHOR]