Back to Search Start Over

Near-infrared responsive magnetic photocatalyst based on NaYF4:Yb3+/Er3+@Cu2O@MoS2@Fe3O4 for the efficient degradation of organic contaminants.

Authors :
Ma, Yuangong
Zhang, Wensheng
Wu, Zhifang
Liang, Zhishan
Huang, Youlin
Tan, Qingmei
Liu, Tianren
Han, Dongxue
Niu, Li
Source :
New Journal of Chemistry. 5/7/2024, Vol. 48 Issue 17, p7688-7698. 11p.
Publication Year :
2024

Abstract

In the realm of photocatalysis, effectively utilizing solar energy, especially the near-infrared (NIR) spectrum, presents substantial challenges. To tackle this issue, a novel composite of NaYF4:Yb3+/Er3+@Cu2O@MoS2@Fe3O4 (denoted as NYE@Cu2O@MoS2@Fe3O4) was ingeniously fabricated and assessed for the photodegradation of organic contaminants. By harnessing the distinct properties of upconversion materials, narrow bandgap semiconductors, and magnetic substances, the NYE@Cu2O@MoS2@Fe3O4 catalyst possesses a photodegradation rate of 92% for the rhodamine B dye under NIR light radiation, which is superior to NYE@Cu2O (50%) and NYE@Cu2O@MoS2 (85%). The enhanced performance in the near-infrared photocatalysis of NYE@Cu2O@MoS2@Fe3O4 is mainly attributed to the synergistic effect of various components, which promotes an increase in photo-induced carrier generation and facilitates their efficient transfer and energy utilization under NIR irradiation. This study provides a possible route for the near-infrared photocatalytic degradation of pollutants in areas with limited light or even dark conditions. [ABSTRACT FROM AUTHOR]

Details

Language :
English
ISSN :
11440546
Volume :
48
Issue :
17
Database :
Academic Search Index
Journal :
New Journal of Chemistry
Publication Type :
Academic Journal
Accession number :
176911873
Full Text :
https://doi.org/10.1039/d4nj00415a