The Danish Lagrangian Model (DALM): Development of a new local-scale high-resolution air pollution model.

This paper describes the DAnish Lagrangian Model (DALM), which is a new high-resolution air pollution model based on the concept of Lagrangian particles. The new model is developed from the simpler Gaussian plume-in-grid Urban Background Model (UBM) and is to be integrated with the DEHM/UBM/AirGIS modeling system, developed at Aarhus University. In the first part of the paper, the theoretical foundation of the model is presented, and the implementation of a large set of physical and numerical parameterizations is discussed. The second part describes the validation of DALM against measurements, applying different combinations of the implemented parameterizations. This validation demonstrates that DALM can accurately reproduce spatiotemporal patterns in the measured data and that its performance is more sensitive to parameterizations of vertical compared to horizontal transport. Conclusively, the combination of parameterizations yielding the best model performance is determined based on a ranking system, and future improvements to DALM are outlined. [Display omitted] • A new comprehensive local-scale Lagrangian air pollution model is in development. • The new model is validated against measurements from Danish monitoring stations. • Some sets of planetary boundary layer parameterizations show a better performance. [ABSTRACT FROM AUTHOR]