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Prompt gamma rays of terbium induced by inelastic scattering of fission neutrons.

Authors :
Ophoven, Niklas
Ilic, Zeljko
Mauerhofer, Eric
Randriamalala, Tsitohaina H.
Vezhlev, Egor
Stieghorst, Christian
Révay, Zsolt
Jolie, Jan
Strub, Erik
Source :
Journal of Radioanalytical & Nuclear Chemistry. Mar2024, Vol. 333 Issue 3, p1287-1300. 14p.
Publication Year :
2024

Abstract

Prompt gamma rays of terbium emitted after (n,nʹγ) inelastic scattering reactions induced by irradiation of a terbium(III) hexahydrate (TbCl3·6H2O) sample with a beam of fission neutrons were investigated with the instrument FaNGaS (Fast Neutron-induced Gamma-ray Spectrometry) at an angle of 90° between neutron beam and detector. At sample position, the fast-neutron flux was 1.13 × 108 cm−2 s−1 and the neutron beam has an average energy of 2.30 MeV. We identified 124 prompt gamma lines from the 159Tb(n,nʹγ)159Tb reaction. Presence of prompt gamma rays from oxygen and chlorine was used for a concise verification of recently published results. Relative gamma-ray intensities, effective cross sections and fast-neutron spectrum-averaged partial production cross sections of the gamma lines are given including comparisons with available literature data. We found a reasonable agreement and the multitude of unreported lines adds decisive value to nuclear spectroscopy. Additionally, we estimated the detection limit of terbium as 1 mg for a counting time of 12 h. [ABSTRACT FROM AUTHOR]

Details

Language :
English
ISSN :
02365731
Volume :
333
Issue :
3
Database :
Academic Search Index
Journal :
Journal of Radioanalytical & Nuclear Chemistry
Publication Type :
Academic Journal
Accession number :
176222966
Full Text :
https://doi.org/10.1007/s10967-023-09344-y