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Innovative use of wet carbon conversion in alkali-activated slag: Improved microstructures and mechanical characteristics.

Authors :
Han, Yi
Yang, Bo
Meng, Li-Yi
Oh, Seokhoon
Kim, TaeSoo
Wang, Xiao-Yong
Source :
Construction & Building Materials. Jan2024, Vol. 411, pN.PAG-N.PAG. 1p.
Publication Year :
2024

Abstract

Nano-calcium carbonate (nano-CaCO 3) has garnered significant attention due to its remarkable efficacy in enhancing the properties and microstructure of concrete. In this study, the wet carbon conversion method was used to synthesize solid nano-CaCO 3 from CO 2 , which was then added to AAS. Subsequently, the compressive strength and resistivity of the AAS mortar were assessed, and the AAS paste underwent microscopic characterization using experimental methods, including X-ray diffraction (XRD) and Fourier-transformed infrared (FTIR), and scanning electron microscope (SEM) et.al. The effects of the nano-CaCO 3 on the microstructure, mechanical characteristics, and durability of the AAS were determined. The microscopic analysis results clearly demonstrate that the nano-CaCO 3 prepared using this method exerts significant physical and chemical effects, leading to a notable improvement in the compactness of the AAS microstructure. Moreover, the experimental findings provide further confirmation that the addition of nano-CaCO 3 results in a substantial enhancement of both the compressive strength and resistivity of AAS mortar, particularly in the early stages. Specifically, the inclusion of 6% nano-calcium carbonate led to a remarkable 29.8% increase in compressive strength at 1 curing day. Furthermore, the analysis of carbon dioxide emissions from AAS reveals that incorporating nano-CaCO 3 effectively reduces the carbon footprint associated with AAS. This implies that adopting this approach not only enhances the performance of AAS but also contributes to a reduction in the environmental impact, thus actively promoting sustainable construction and engineering projects. • The wet carbon conversion method synthesizes nano-CaCO 3 to enhance alkali-activated slag (AAS) performance. • Nano-CaCO 3 enhances AAS microstructure compactness through physical and chemical effects. • Nano-CaCO 3 reacts with the aluminum phase in AAS, forming carboaluminate. [ABSTRACT FROM AUTHOR]

Details

Language :
English
ISSN :
09500618
Volume :
411
Database :
Academic Search Index
Journal :
Construction & Building Materials
Publication Type :
Academic Journal
Accession number :
174786669
Full Text :
https://doi.org/10.1016/j.conbuildmat.2023.134487