α(PS)–γ(Ge) digital anti-coincidence spectroscopy and its application to activity measurement of 225Ac.

Activity of 225Ac was measured by the digital anti-coincidence spectroscopy technique using a 4πα–γ detector configuration, composed of a sandwich type 4π plastic scintillator and Ge detectors. Ultrathin plastic scintillators were used for selective detection of α-particles emitted from 225Ac and its progenies, and the α-counting efficiencies of a 4π plastic scintillation detector for individual nuclides in the decay chain were determined as well. A list-mode multichannel analyzer was employed to record coincidence/anti-coincidence events for off-line analyses. The time difference distribution spectra revealed α-particle emission following 213Po decay without β-particle interference from 213Bi. • Selective α-particle detection using ultrathin plastic scintillators for 225Ac. • Individual α-efficiencies determined by 4πα(PS)–γ(Ge) anti-coincidence spectroscopy. • α-particles from short-lived 213Po(T 1/2 = 3.7 μs) detected without interference. • Effect of β-particle from 213Bi confirmed from γ–α/β time difference distribution. • Results were consistent with those obtained using the CN method with LSC. [ABSTRACT FROM AUTHOR]