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Optical and scintillation characteristics of Lu2Y(Al5-xGax)O12:Ce,Mg multicomponent garnet crystals.

Authors :
Chewpraditkul, Warut
Pattanaboonmee, Nakarin
Chewpraditkul, Weerapong
Kamada, Kei
Kim, Kyoung Jin
Yoshikawa, Akira
Makowski, Michał
Witkowski, Marcin E.
Drozdowski, Winicjusz
Beitlerova, Alena
Kucerkova, Romana
Babin, Vladimir
Nikl, Martin
Source :
Optical Materials. Dec2022:Part A, Vol. 134, pN.PAG-N.PAG. 1p.
Publication Year :
2022

Abstract

Optical and scintillation characteristics of Mg2+-codoped Lu 2 Y(Al 5-x Ga x)O 12 :Ce (x = 2, 3) multicomponent garnet crystals grown by the micro-pulling down method were investigated. At RT, the shortening of scintillation decay time and a decrease of light yield (LY) value measured for a higher Ga containing samples can be explained by thermal ionization of the Ce3+ 5d 1 excited state. At 662 keV γ-rays, Lu 2 YAl 3 Ga 2 O 12 : Ce, 0.05%Mg exhibits high LY value of 29,000 ph/MeV along with scintillation decay times of 50 ns (86%) + 73 ns (14%). Co-doping with larger Mg2+ content leads to a decrease of LY value, scintillation decay time, and afterglow level. Radioluminescence quenching observed at low temperature region in correlation with large thermoluminescence peaks can be caused by trapping of electrons at intrinsic shallow traps. • Luminescence and scintillation properties of Lu 2 Y(Al 5-x Ga x)O 12 :Ce,Mg (x = 2, 3) crystals are investigated. • Temperature dependencies of photo-and radioluminescence are presented. • Lu 2 YAl 3 Ga 2 O 12 :Ce,0.05%Mg shows high light yield of 29,000 photons/MeV. • Lu 2 YAl 3 Ga 2 O 12 :Ce,0.05%Mg shows quenching temperature at 435 K due to thermal ionization. • Afterglow and thermoluminescence characteristics are investigated. [ABSTRACT FROM AUTHOR]

Details

Language :
English
ISSN :
09253467
Volume :
134
Database :
Academic Search Index
Journal :
Optical Materials
Publication Type :
Academic Journal
Accession number :
160438299
Full Text :
https://doi.org/10.1016/j.optmat.2022.113186