Dispersion properties in the visible range of carrier concentration of topologically protected Bi1-xSex films revealed by spectroscopic ellipsometry.

Highlights • A significant dispersion of penetration depth with Bi 0.38 Se 0.62 films versus phonon energy was found. • A dispersive plasma energy was introduced to traditional MDF model for modelling topological insulators. • Spectroscopic ellipsometry was shown to be a useful tool for characterizing the properties of the topological insulators. Abstract Optical properties evolution of Bi 1- x Se x films with different compositions were investigated by spectroscopic ellipsometry (SE). A significant dispersion of penetration depth of Bi 0.38 Se 0.62 films was observed, which would lead to a varying carrier concentration with the different wavelength because of the topologically protected surface state. To describe the special properties of topological insulators, dispersive plasma energy was introduced into traditional dielectric function model. Optical properties of Bi 0.38 Se 0.62 film were acquired by this modified model and the topologically protected surface state could be represented from the dispersion properties of free carrier concentration with the smaller plasma energy versus the deeper penetration depth. We demonstrated that SE is a useful tool for characterizing the properties of the topological insulators. [ABSTRACT FROM AUTHOR]