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Anisotropic Ru3+ 4d5 magnetism in the α-RuCl3 honeycomb system: Susceptibility, specific heat, and zero-field NMR.
- Source :
-
Physical Review B: Condensed Matter & Materials Physics . May2015, Vol. 91 Issue 18, p180401-1-180401-4. 4p. - Publication Year :
- 2015
-
Abstract
- Hexagonal α-Ru trichloride single crystals exhibit a strong magnetic anisotropy and we show that upon applying fields up to 14 T in the honeycomb plane the successive magnetic order at T1 = 14 K and T2 = 8 K could be completely suppressed whereas in the perpendicular direction the magnetic order is robust. Furthermore the field dependence of Χ(T) implies coexisting ferro- and antiferromagnetic exchange between in-plane components of Ru3+spins, whereas for out-of-plane components a strong antiferromagnetic exchange becomes evident. 101Ru zero-field nuclear magnetic resonance in the ordered state evidence a complex (probably non coplanar chiral) long-range magnetic structure. The large orbital moment on Ru3+ is found in density-functional calculations. [ABSTRACT FROM AUTHOR]
Details
- Language :
- English
- ISSN :
- 10980121
- Volume :
- 91
- Issue :
- 18
- Database :
- Academic Search Index
- Journal :
- Physical Review B: Condensed Matter & Materials Physics
- Publication Type :
- Academic Journal
- Accession number :
- 108399971
- Full Text :
- https://doi.org/10.1103/PhysRevB.91.180401