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The Hapke model has been widely used in the field of soil remote sensing. However, the latest development of the Hapke model (i.e., Hapke-HSR model) adopted a simple hypothesis to consider the influence of the soil moisture content (SMC), which brought great difficulties to SMC parameter inversion. This paper presents a method to improve the Hapke model using the improved multilayer radiative transfer model of soil reflectance (MARMIT-2), which can effectively improve the ability of the Hapke-HSR model to characterize the variation in the SMC. Finally, we used the soil database to comprehensively verify the ability of the improved Hapke model. The results show that the improved Hapke can effectively characterize the spectral characteristics of soil and show a higher fitting accuracy (RMSE = 0.009) compared with the Hapke-HSR model (RMSE = 0.031), especially at a high SMC (≥30%). Therefore, the improved Hapke model can better understand soil physical properties and improve the inversion accuracy of soil–vegetation physical parameters, which can be used to enhance agricultural water use efficiency. [ABSTRACT FROM AUTHOR]