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As the proportion of renewable energy generation continues to increase, the participation of new energy stations with high-proportion energy storage in power system frequency regulation is of significant importance for stable and secure operation of the new power system. To address this issue, an energy storage control method based on quantum walks and model predictive control (MPC) has been proposed. First, historical frequency deviation signals and energy storage charge-discharge state signals are collected. Simulation data are generated through amplitude encoding and quantum walks, followed by quantum decoding. Subsequently, the decoded data are inputted into the MPC framework for real-time control, with parameters of the predictive model continuously adjusted through a feedback loop. Finally, a novel power system frequency regulation model with high-proportion new energy storage stations is constructed on the MATLAB/Simulink platform. Simulation verification is conducted with the proportional-integral-derivative (PID) and MPC methods as comparative approaches. Simulation results under step disturbances and random disturbances demonstrate that the proposed method exhibits stronger robustness and better control accuracy. [ABSTRACT FROM AUTHOR]