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The Antarctic Slope Current is guided by the topographic gradient of the Antarctic continental slope and creates a dynamical barrier between the continental shelf and the open ocean. The current's vertical structure varies around the continent affecting cross‐slope water mass exchange with consequences for Antarctic mass loss, ventilation of the deep ocean, and carbon uptake. The Antarctic Slope Current is surface‐intensified in many regions but bottom‐intensified in regions of dense overflows. This study investigates the role of dense overflows in modifying the dynamics of the bottom‐intensified flow using a 0.1° global ocean‐sea ice model. The occurrence of bottom‐intensification is tightly linked with dense overflows and bottom speeds correlate with dense overflows on interannual time scales. A lack of vertical connectivity between the bottom and surface flow, however, suggests that the along‐slope bottom water flows are coincidentally co‐located with the Antarctic Slope Current, rather than dynamically a part of the current. Plain Language Summary: The Antarctic Slope Current is a narrow ocean current that travels around Antarctica following the continental slope. It separates the shallow and cold continental shelf from much warmer waters in the open ocean. Intrusions of the relatively warm water across the continental slope impacts melting of Antarctic ice shelves and global sea level rise. Understanding what controls the strength and variability of the Antarctic Slope Current is therefore important. The Antarctic Slope Current usually has the largest velocities near the surface, but there are regions where there is also a strong bottom flow. We use a coupled ocean‐sea ice model and show that the bottom flow is controlled by the export of very dense shelf water that flows down the continental slope in a few locations around the continent. However, the bottom and surface flow does not vary together on interannual time scales which tells us that the two components of the Antarctic Slope Current are largely independent. The result is important as the formation of dense shelf water is expected to reduce in the future which will impact the deep flow, but not the surface component. Key Points: Simulations reveal a close spatial relationship between the bottom‐intensified Antarctic Slope Current and Dense Shelf Water exportInterannual variability of Dense Shelf Water is reflected in the bottom speed of the bottom‐intensified Antarctic Slope CurrentThe surface component varies independently from the bottom‐intensified flow implying two distinct, co‐located currents [ABSTRACT FROM AUTHOR]

Abstract The Antarctic Slope Current is guided by the topographic gradient of the Antarctic continental slope and creates a dynamical barrier between the continental shelf and the open ocean. The current's vertical structure varies around the continent affecting cross‐slope water mass exchange with consequences for Antarctic mass loss, ventilation of the deep ocean, and carbon uptake. The Antarctic Slope Current is surface‐intensified in many regions but bottom‐intensified in regions of dense overflows. This study investigates the role of dense overflows in modifying the dynamics of the bottom‐intensified flow using a 0.1° global ocean‐sea ice model. The occurrence of bottom‐intensification is tightly linked with dense overflows and bottom speeds correlate with dense overflows on interannual time scales. A lack of vertical connectivity between the bottom and surface flow, however, suggests that the along‐slope bottom water flows are coincidentally co‐located with the Antarctic Slope Current, rather than dynamically a part of the current.

Aerosols are essential climate variables that need to be observed at a global scale to monitor the evolution of the atmospheric composition and potential climate impacts. We used the measurements performed over the May 2007–December 2019 period by a ground-based sun photometer installed at the island of La Réunion (21°S, 55°E), together with a linear regression fitting model, to assess the climatology and types of aerosols reaching this observation site located in a sparsely documented pristine area, and the forcings responsible for the variability of the observed aerosol optical depth (AOD) and related trend. The climatology of the aerosol optical depth (AOD) at 440 nm (AOD440) and Ångström exponent between 500 and 870 nm (α) revealed that sea salts could be considered as the La Réunion AOD440 and α baselines (0.06 ± 0.03 and 0.61 ± 0.40, respectively, from December to August), which were mainly modulated by biomass burning (BB) plumes passing over La Réunion (causing a doubling of AOD440 and α up to 0.13 ± 0.07 and 1.06 ± 0.34, respectively, in October). This was confirmed by the retrieved aerosol volume size distributions showing that the coarse-mode (fine-mode) dominated the total volume concentration for AOD440 lower (higher) than 0.2 with a mean radius equal to 3 μm (0.15 μm). The main contribution to the AOD440 variability over La Réunion was evaluated to be the BB activity (67.4 ± 28.1%), followed by marine aerosols (16.3 ± 4.2%) and large-scale atmospheric structures (5.5 ± 1.7%). The calculated trend for AOD440 equaled 0.02 ± 0.01 per decade (2.6 ± 1.3% per year). These results provide a scientific reference base for upcoming studies dedicated to the quantification of the impact of wildfire emissions on the southwestern Indian Ocean's atmospheric composition and radiative balance. [ABSTRACT FROM AUTHOR]

Aerosols are essential climate variables that need to be observed at a global scale to monitor the evolution of the atmospheric composition and potential climate impacts. We used the measurements performed over the May 2007–December 2019 period by a ground-based sun photometer installed at the island of La Réunion (21°S, 55°E), together with a linear regression fitting model, to assess the climatology and types of aerosols reaching this observation site located in a sparsely documented pristine area, and the forcings responsible for the variability of the observed aerosol optical depth (AOD) and related trend. The climatology of the aerosol optical depth (AOD) at 440 nm (AOD440) and Ångström exponent between 500 and 870 nm (α) revealed that sea salts could be considered as the La Réunion AOD440 and α baselines (0.06 ± 0.03 and 0.61 ± 0.40, respectively, from December to August), which were mainly modulated by biomass burning (BB) plumes passing over La Réunion (causing a doubling of AOD440 and α up to 0.13 ± 0.07 and 1.06 ± 0.34, respectively, in October). This was confirmed by the retrieved aerosol volume size distributions showing that the coarse-mode (fine-mode) dominated the total volume concentration for AOD440 lower (higher) than 0.2 with a mean radius equal to 3 μm (0.15 μm). The main contribution to the AOD440 variability over La Réunion was evaluated to be the BB activity (67.4 ± 28.1%), followed by marine aerosols (16.3 ± 4.2%) and large-scale atmospheric structures (5.5 ± 1.7%). The calculated trend for AOD440 equaled 0.02 ± 0.01 per decade (2.6 ± 1.3% per year). These results provide a scientific reference base for upcoming studies dedicated to the quantification of the impact of wildfire emissions on the southwestern Indian Ocean’s atmospheric composition and radiative balance.

The present study contributes to the scientific effort for a better understanding of the potential of the Australian biomass burning events to influence tropospheric trace gas abundances at the regional scale. In order to exclude the influence of the long-range transport of ozone precursors from biomass burning plumes originating from Southern America and Africa, the analysis of the Australian smoke plume has been driven over the period December 2019 to January 2020. This study uses satellite (IASI, MLS, MODIS, CALIOP) and ground-based (sun-photometer, FTIR, ozone radiosondes) observations. The highest values of aerosol optical depth (AOD) and carbon monoxide total columns are observed over Southern and Central Australia. Transport is responsible for the spatial and temporal distributions of aerosols and carbon monoxide over Australia, and also the transport of the smoke plume outside the continent. The dispersion of the tropospheric smoke plume over Oceania and Southern Pacific extends from tropical to extratropical latitudes. Ozone radiosonde measurements performed at Samoa (14.4°S, 170.6°W) and Lauder (45.0°S, 169.4°E) indicate an increase in mid-tropospheric ozone (6–9 km) (from 10% to 43%) linked to the Australian biomass burning plume. This increase in mid-tropospheric ozone induced by the transport of the smoke plume was found to be consistent with MLS observations over the tropical and extratropical latitudes. The smoke plume over the Southern Pacific was organized as a stretchable anticyclonic rolling which impacted the ozone variability in the tropical and subtropical upper-troposphere over Oceania. This is corroborated by the ozone profile measurements at Samoa which exhibit an enhanced ozone layer (29%) in the upper-troposphere. Our results suggest that the transport of Australian biomass burning plumes have significantly impacted the vertical distribution of ozone in the mid-troposphere southern tropical to extratropical latitudes during the 2019–20 extreme Australian bushfires.

Despite a number of studies on biomass burning (BB) emissions in the atmosphere, observation of the associated aerosols and pollutants requires continuous efforts. Brazil, and more broadly Latin America, is one of the most important seasonal sources of BB, particularly in the Amazon region. Uncertainty about aerosol loading in the source regions is a limiting factor in terms of understanding the role of aerosols in climate modelling. In the present work, we investigated the Amazon BB episode that occurred during August 2019 and made the international headlines, especially when the smoke plumes plunged distant cities such as São Paulo into darkness. Here, we used satellite and ground-based observations at different locations to investigate the long-range transport of aerosol plumes generated by the Amazon fires during the study period. The monitoring of BB activity was carried out using fire related pixel count from the moderate resolution imaging spectroradiometer (MODIS) onboard the Aqua and Terra platforms, while the distribution of carbon monoxide (CO) concentrations and total columns were obtained from the infrared atmospheric sounding interferometer (IASI) onboard the METOP-A and METOP-B satellites. In addition, AERONET sun-photometers as well as the MODIS instrument made aerosol optical depth (AOD) measurements over the study region. Our datasets are consistent with each other and highlight AOD and CO variations and long-range transport of the fire plume from the source regions in the Amazon basin. We used the Lagrangian transport model FLEXPART (FLEXible PARTicle) to simulate backward dispersion, which showed good agreement with satellite and ground measurements observed over the study area. The increase in Rossby wave activity during the 2019 austral winter the Southern Hemisphere may have contributed to increasing the efficiency of large-scale transport of aerosol plumes generated by the Amazon fires during the study period.

Volcanic plumes can be transported across vast distances and can have an impact on solar ultraviolet radiation (UVR) reaching the surface due to the scattering and absorption caused by aerosols. The dispersion of the volcanic plume from the Puyehue-Cordón Caulle volcanic complex (PCCVC) eruption was investigated to determine the effect on aerosol loading at Cape Point, South Africa. The eruption occurred on 4 June 2011 and resulted in a plume reaching a height of between 9 and 12 km and was dispersed across the Southern Hemisphere. Satellite sulphur dioxide (SO2) observations and a dispersion model showed low concentrations of SO2 at the secondary site. However, satellite observations of volcanic ash and ground-based aerosol measurements did show increases between 10 and 20 June 2011 at the secondary site. Furthermore, there was good agreement with the dispersion model results and observations from satellites with most of the plume located between latitudes 40°–60° South.

A series of large-eddy simulation (LES) models consisting of two-dimensional (2D) idealised street canyons with building height variability (BHV) are examined. Building blocks with two different heights are placed alternately in the computational domains, constructing repeated street canyons of building-height-to-street-width (aspect) ratio (AR) = 1, 0.5, 0.25 and 0.125 together with BHV = 0.2, 0.4 and 0.6. LES results show that the air exchange rate (ACH) increases with increasing aerodynamic resistance. Apart from AR, BHV is another factor affecting the aerodynamic resistance and thus the ACH. The (vertical) dispersion coefficient σz of plume transport is also closely related to the aerodynamic resistance, suggesting that introducing BHV in urban areas could help improve the air quality. [ABSTRACT FROM AUTHOR]

Abstract: We report observations of normalized enhancement ratios (NER) for 32 wildfires measured at Mount Bachelor Observatory in central Oregon during June–September 2004–2011. All 32 plumes resulted from wildfires originating in the western United States and Canada. The observed NER of PM1 (particulate matter < 1 micron) to carbon monoxide (ΔPM1/ΔCO) ranged from 0.06 to 0.42 μg m−3 ppbv−1. The NER of ozone to CO (ΔO3/ΔCO) ranged from 0.01 to 0.51 ppbv ppbv−1 for the 13 observed plumes with a significant ΔO3/ΔCO NER (p ≤ 0.01, R 2 ≥ 0.30). For wildfire plumes transported <540 km, or approximately <2 days, the ΔPM1/ΔCO NER is found to increase with increasing distance, suggesting that there is significant secondary organic aerosol (SOA) production in these plumes. However, two plumes transported over greater time periods have relatively low ΔPM1/ΔCO NER, indicating that PM1 loss is greater than SOA production in these plumes. Of the three plumes transported the longest distance to MBO, only two have significant O3 production. These two plumes were transported in boundary layer air masses, while the third was transported in a free tropospheric air mass, suggesting that conversion of nitrogen oxides (NO X ) to peroxyacetyl nitrate (PAN) may be a factor affecting O3 production in these plumes. Two wildfire plumes are mixed with urban emissions from the Seattle/Tacoma metropolitan area, and have relatively higher ΔO3/ΔCO NER than other wildfire plumes transported over similar distances. [Copyright &y& Elsevier]

Abstract: Cal-Mex 2010 Field Study is a US-Mexico collaborative project to investigate cross-border transport of emissions in the California-Mexico border region, which took place from May 15 to June 30, 2010. The current study presents an overview of the meteorological conditions and plume transport patterns during Cal-Mex 2010 based on the analysis of surface and vertical measurements (radiosonde, ceilometers and tethered balloon) conducted in Tijuana, Mexico and the modeling output using a trajectory model (FLEXPRT-WRF) and a regional model (WRF). The WRF model has been applied for providing the meteorological daily forecasts that are verified using the available observations. Both synoptic-scale and urban-scale forecasts (including wind, temperature, and humidity) agree reasonably well with the NCEP-FNL reanalysis data and the measurements; however, the WRF model frequently underestimates surface temperature and planetary boundary layer (PBL) height during nighttime compared to measurements. Based on the WRF-FLEXPART simulations with particles released in Tijuana in the morning, four representative plume transport patterns are identified as “plume-southeast”, “plume-southwest”, “plume-east” and “plume-north”, indicating the downwind direction of the plume; this will be useful for linking meteorological conditions with observed changes in trace gases and particular matter (PM). Most of the days during May and June are classified as plume-east and plume-southeast days, showing that the plumes in Tijuana are mostly carried to the southeast and east of Tijuana within the boundary layer during daytime. The plume transport directions are generally consistent with the prevailing wind directions on 850 hPa. The low level (below 800 m) wind, temperature, and moisture characteristics are different for each plume transport category according to the measurements from the tethered balloon. Future studies (such as using data assimilation and ensemble forecasts) will be performed to improve the temperature, wind and PBL simulations. [Copyright &y& Elsevier]

Knowledge on atmospheric abundance of peroxyacetyl nitrate (PAN) is important in assessing the severity of photochemical pollution, and for understanding chemical transformation of reactive odd nitrogen and its impact on the budget of tropospheric ozone (O3). In summer 2006, continuous measurements of PAN were made using an automatic GC–ECD analyzer with an on-line calibrator at a suburban site of Lanzhou (LZ) and a remote site of Mt. Waliguan (WLG) in western China, with concurrent measurements of O3, total reactive nitrogen (NO y ) and carbon monoxide (CO). At LZ, several photochemical episodes were observed during the study, and the average mixing ratio of PAN (plus or minus standard deviation) was 0.76 (±0.89) ppbv with the maximum value of 9.13 ppbv, compared to an average value of 0.44 (±0.16) ppbv at remote WLG. The PAN mixing ratios in LZ exhibited strong diurnal variations with a maximum at noon, while enhanced concentrations of PAN were observed in the evening and a minimum in the afternoon at WLG. The daily O3 and PAN concentration maxima showed a strong correlation (r 2 = 0.91) in LZ, with a regression slope (PAN/O3) of 0.091 ppbv ppbv−1. At WLG, six well-identified pollution plumes (lasting 2–8 h) were observed with elevated concentrations of PAN (and other trace gases), and analysis of backward particle release simulation shows that the high-PAN events at WLG were mostly associated with the transport of air masses that had passed over LZ. [Copyright &y& Elsevier]