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1. Alcoholysis of acylpalladium(II) complexes relevant to the alternating copolymerization of ethene and carbon monoxide and the alkoxycarbonylation of alkenes: The importance of cis-coordinating phosphines

Author

van Leeuwen, Piet W.N.M., Spek, Anthony L., Lutz, Martin, Fraanje, Jan, Goubitz, Kees, Zuideveild, Martin, A., Swennenhuis, Bert H.G., Freixa, Zoraida, and Kamer, Pual C.J.

Subjects
Esters -- Research, Esters -- Chemical properties, Alcohols -- Research, Alcohols -- Chemical properties, Coordination compounds -- Research, Coordination compounds -- Chemical properties, Chemistry
Abstract

The alcoholysis of a variety of acetylpalladium complexes is studied and found that cis-coordination of alcohol and acetyl is needed to form an ester. The outer -sphere attack of alkoxides/alcohols is not viable mechanism for alcoholysis.

Published
2003

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