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The recently observed temperature-dependent quasiphase transition of the single-file water chain confined within a carbon nanotube in experiments has been validated by simple lattice theory and molecular dynamic simulations. It has been pointed out that atomic charges in water model is an important issue, yet how the values will affect the structural details and thermodynamic properties of the quasiphase transition has not been fully revealed. In this work, we performed orientational-biased replica exchange Monte Carlo simulations in the canonical ensemble to explore the effect of atomic charges in SPC/E water model on the quasiphase transition of a single-file water chain. Based on the atomic charge values reported from literature, three distinct quasiphases are reproduced, comprising a fully hydrogen-bonded water chain at lower temperatures, a more ordered dipolar orientation along the x-axis at intermediate temperatures, and a completely disordered structure at higher temperatures. Then by increasing the atomic charge value, we find that the fragmentation of the entire water chain into shorter water segments, the orientational ordering of water dipoles, and the transition towards complete disorder are all inhibited. Consequently, the transition temperatures between three quasiphases have been shifted to higher temperatures. The thermodynamic analysis demonstrates that the increased atomic charge values enhance the hydrogen bonding between neighbouring water molecules also the electrostatic attraction within the water chain, leading to a longer water dipole correlation length even at higher temperatures. These findings shed light on the vital role of atomic charges in water models and also the electrostatic interaction in regulating the orientational ordering of water molecules under nanoconfinement., Comment: 14 pages and 7 figures in Main text, 4 figures in Appendix

The kinematic information of the Radcliffe Wave (RW) is essential for determining its existence and gaining insights into its origin and evolution. In this work, we present an accurate measurement of the vertical velocity ($V_Z$) of RW by incorporating the radial velocity (RV) measures through two methods, which is crucial but was neglected previously. First, the velocities are measured towards young stars, using their RV measurements from APOGEE-2 and proper motion measurements from Gaia DR3. Second, we combine RV measurements toward clouds with proper motion measurements of associated Young Stellar Objects (YSOs) to determine the vertical velocities of the clouds. The results reveal that the oscillations in $V_Z$ are not synchronous with the vertical coordinate $Z$, which differs from the conclusions of previous studies. Instead, we find a 5 km$\cdot$s$^{-1}$$\cdot$kpc$^{-1}$ gradient in $V_Z$ along the RW, exhibiting a dipole-like pattern. Consequently, the kinematic arrangement does not show a corresponding coherence with the spatial arrangement, bringing the Radcliffe Wave model into question., Comment: 9 pages, 6 figures, Accepted for publication in ApJ

Astigmatic unitary transformations allow for the adiabatic connections of all feasible states of paraxial Gaussian beams on the same modal sphere, i.e., Hermite-Laguerre-Gaussian (HLG) modes. Here, we present a comprehensive investigation into the unitary modal evolution of complex structured Gaussian beams, comprised by HLG modes from disparate modal spheres, via astigmatic transformation. The non-synchronized higher-order geometric phases in cyclic transformations originates a Talbot-effect-like modal evolution in the superposition state of these HLG modes, resulting in pattern variations and revivals in transformations with specific geodesic loops. Using Ince-Gaussian modes as an illustrative example, we systematically analyze and experimentally corroborate the beamforming mechanism behind the pattern evolution. Our results outline a generic modal conversion theory of structured Gaussian beams via astigmatic unitary transformation, offering a new approach for shaping spatial modal structure. These findings may inspire a wide variety of applications based on structured light., Comment: 7 pages, 5 figures

YbB$_6$ is a predicted topological insulator, with experimental evidence for conducting surface states of yet-unproven origin. However, its lack of a natural cleavage plane, and resultant surface-dependent polarity, has obscured its study. We use scanning tunneling microscopy to image the cleaved surface of YbB$_6$, exhibiting several coexisting terminations with distinct atomic structures. Our spectroscopic measurements show band-bending between the terminations, resulting in both conducting and fully-gapped regions. In the conductive regions, we observe spectral peaks that are suggestive of van Hove singularities arising from Rashba spin-split quantum well states. The insulating regions rule out the possibility that YbB$_6$ is a strong topological insulator, while the spin-polarized conducting regions suggest possible utility for spintronic devices., Comment: Submitted to Physical Review Letters

Recent advances in planar optics with geometric-phase superstructures have brought a new paradigm in the control of structured light and, in particular, has substantially enhanced the capabilities of generating and detecting orbital angular momentum (OAM) states of light and associated spatial modes. However, the structured modal interface that can reciprocally link OAM states via adiabatic control and access-associated higher-order geometric phase remains absent in planar optics. In this work, we propose and experimentally demonstrate a planar optical astigmatic retarder fabricated with liquid-crystal (LC) geometric phase. The LC superstructure was designed with the principle of fractional Fourier transformation and is capable of reciprocal conversion between all possible OAM states on the same modal sphere. Such a planar device paves the way towards an easily deployed modal interface of paraxial OAM states, unlocks the resource of higher-order geometric phase, and has promising applications in high-dimensional classical/quantum information.

Since the diffraction behavior of a light field is fully determined by its spatial wavefunction, i.e., its spatial complex amplitude (SCA), full characterization of spatial wavefunction, plays a vital role in modern optics from both the fundamental and applied aspects. In this work, we present a novel complex-amplitude profiler based on spatial Stokes tomography with the capability to fully determine the SCA of a light field in a single shot with high precision and resolution. The SCA slice observed at any propagation plane provides complete information about the light field, thus allowing us to further retrieve the complete beam structure in 3 dimensions space, as well as the exact modal constitution in terms of spatial degrees of freedom. The principle demonstrated here provides an important advancement for the full characterization of light beams with a broad spectrum of potential applications in various areas of optics, especially for the growing field of structured light.

Rapid rotation may exist in physical systems such as non-central heavy ion collisions and neutron stars. Using functional renormalization group analysis of the quark-meson model, we investigate the effects of real and imaginary rotation on the chiral phase transition. Our results confirm previous studies conducted with other model calculations and shed light on the importance of boundary conditions in the infrared region of the theory., Comment: 14 pages, 12 figures

Reciprocal spin-orbit coupling (SOC) via geometric phase with flat optics provides a promising platform for shaping and controlling paraxial structured light. Current devices, from the pioneering q-plates to the recent J-plates, provide only spin-dependent wavefront modulation without amplitude control. However, achieving control over all the spatial dimensions of paraxial SOC states requires spin-dependent control of corresponding complex amplitude, which remains challenging for flat optics. Here, to address this issue, we present a new type of flat-optics elements termed structured geometric phase gratings that is capable of conjugated complex-amplitude control for orthogonal input circular polarizations. By using a microstructured liquid crystal photoalignment technique, we engineered a series of flat-optics elements and experimentally showed their excellent precision in arbitrary SOC control. This principle unlocks the full-field control of paraxial structured light via flat optics, providing a promising way to develop an information exchange and processing units for general photonic SOC states, as well as extra-/intracavity mode convertors for high-precision laser beam shaping.

Orbital angular momentum (OAM) conservation plays an important role in shaping and controlling structured light with nonlinear optics. The OAM of a beam originating from three-wave mixing should be the sum or difference of the other two inputs because no light-matter OAM exchange occurs in parametric nonlinear interactions. Here, we report anomalous OAM conservation during parametric upconversion, in which a Hermite-Gauss mode signal interacts with a specially engineered pump capable of astigmatic transformation in a crystal, resulting in Laguerre-Gaussian mode sum-frequency generation (SFG). The anomaly here refers to the fact that the pump and signal carry no net OAM, while their SFG does. We show that the lost OAM with the opposite sign that maintains OAM conservation in the system is hidden in the residual pump. This unexpected OAM selection rule improves our understanding of OAM conservation in parametric nonlinear systems and may inspire new ideas for controlling OAM states via nonlinear optics, especially in quantum applications.

In this paper, we compute the H- and Z-eigenvalues of even order symmetric tensors by using the adaptive cubic regularization algorithm.

Groups with various types of operators, in particular the recently introduced Rota-Baxter groups, have generated renowned interest with close connections to numerical integrals, Yang-Baxter equation, integrable systems and post-Hopf algebras. This paper gives the general notion of operated groups and provides explicit constructions of free operated groups, free differential groups and free Rota-Baxter groups., Comment: 21 pages

Rota-Baxter associative algebras and Rota-Baxter Lie algebras are both important in mathematics and mathematical physics, with the former a basic structure in quantum field renormalization and the latter a operator form of the classical Yang-Baxter equation. An outstanding problem posed by Gubarev is to determine whether there is a Poincar\'e-Birkhoff-Witt theorem for the universal enveloping Rota-Baxter associative algebra of a Rota-Baxter Lie algebra. This paper resolves this problem positively, working with operated algebras and applying the method of Gr\"obner-Shirshov bases., Comment: There was an error in considering all the compositions in Sec 3.1

So far, the behavior of the pionic leading-twist distribution amplitude (DA) $\phi_{2;\pi}(x,\mu)$ $-$ which is universal physical quantity and enters the high-energy processes involving pion based on the factorization theorem $-$ has not been completely consistent. The form of $\phi_{2;\pi}(x,\mu)$ is usually described by phenomenological models and constrained by the experimental data of the exclusive processes containing pion or the moments calculated with the QCD sum rules and lattice QCD theory. Obviously, an appropriate model is very important for us to determine the exact behavior of $\phi_{2;\pi}(x,\mu)$. In this paper, by adopting the least squares method to fit the $\xi$-moments calculated with QCD sum rules based on the background field theory, we perform an analysis for several commonly used models of the pionic leading-twist DA in the literature, such as the truncation form of the Gegenbauer polynomial series, the light-cone harmonic oscillator model, the form from the Dyson-Schwinger equations, the model from the light-front holographic AdS/QCD and a simple power-law parametrization form., Comment: 10 pages, 2 figures

Optical interferometers are pillars of modern precision metrology, but their resolution is limited by the wavelength of the light source, which cannot be infinitely reduced. Magically, this limitation can be circumvented by using an entangled multiphoton source because interference produced by an N-photon amplitude features a reduced de Broglie wavelength {\lambda}/N. However, the extremely low efficiency in multiphoton state generation and coincidence counts actually negates the potential of using multiphoton states in practical measurements. Here, we demonstrate a novel interferometric technique based on structured nonlinear optics, i.e., parametric upconversion of a structured beam, capable of superresolution measurement in real time. The main principle relies in that the orbital angular momentum (OAM) state and associated intramodal phase within the structured beam are both continuously multiplied in cascading upconversion to mimic the superresolved phase evolution of a multiphoton amplitude. Owing to the use of bright sensing beams and OAM mode projection, up to a 12-photon de Broglie wavelength with almost perfect visibility is observed in real time and, importantly, by using only a low-cost detector. Our results open the door to real-time superresolution interferometric metrology and provide a promising way toward multiphoton superiority in practical applications.

Rydberg atoms have great potential in electric field measurement and have an advantage with a large frequency bandwidth from the kHz to the THz scale. However, the sensitivity for measuring a weak MHz electric field signal is limited by the spectroscopic resolution, because the weak electric field induces only a small perturbation of the population and energy level shift of the Rydberg atoms. Here, we report highly sensitive measurement of a weak MHz electric field using electromagnetically induced transparency with Rydberg atoms in a thermal atomic system. Using the heterodyne method on a 30-MHz electric field, we successfully measure the minimum electric field strength to be \textcolor{black}{37.3 $\mathrm{\mu V/cm}$} with a sensitivity up to $-65$ dBm/Hz and a linear dynamic range over 65 dB. Additionally, we measure an amplitude-modulated signal and demodulate the signal with a fidelity over 98\%. This work extends the sensitivity of atomic sensors for measuring MHz electric fields, which advances atomic electric field-sensing technology., Comment: 6 pages, 4 figures

Autocorrelation measurement based on second-harmonic generation (SHG), the best-known technique for measuring the temporal duration of ultrashort pulses, could date back to the birth of ultrafast lasers. Here, we propose and experimentally demonstrate that such well-established technique can also be used to measure the orbital angular momentum of ultrashort Laguerre-Gauss (LG) pulses. By analysing the far-field pattern of the SHG signal, the full spatial structure of ultrashort LG pulses, including both azimuthal and radial indices, are unambiguously determined. Our results provide an important advancement for the well-established autocorrelation technique by extending it to reach its full potential in laser characterization, especially for structured ultrashort pulses.