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We report the discovery of five white dwarf + ultracool dwarf systems identified as common proper motion wide binaries in the Gaia Catalogue of Nearby Stars. The discoveries include a white dwarf + L subdwarf binary, VVV 1256-62AB, a gravitationally bound system located 75.6(+1.9/-1.8) pc away with a projected separation of 1375(+35/-33) au. The primary is a cool DC white dwarf with a hydrogen dominated atmosphere, and has a total age of 10.5(+3.3/-2.1) Gyr, based on white dwarf model fitting. The secondary is an L subdwarf with a metallicity of [M/H] = -0.72(+0.08/-0.10) (i.e. [Fe/H] = -0.81+/-0.10) and Teff = 2298(+45/-43) K based on atmospheric model fitting of its optical to near infrared spectrum, and likely has a mass just above the stellar/substellar boundary. The sub-solar metallicity of the L subdwarf and the system's total space velocity of 406 km/s indicates membership in the Galactic halo, and it has a flat eccentric Galactic orbit passing within 1~kpc of the centre of the Milky Way every ~0.4Gyr and extending to 15-31 kpc at apogal. VVV 1256-62B is the first L subdwarf to have a well-constrained age, making it an ideal benchmark of metal-poor ultracool dwarf atmospheres and evolution., Comment: 15 pages, 12 figures

Plasma-based electron and positron wakefield acceleration has made great strides in the past decade. However one major challenge for its applications to coherent light sources and colliders is the relatively large energy spread of the accelerated beams, currently at a few percent level. This energy spread is usually correlated with particle position in the beam arising from the longitudinal chirp of the wakefield amplitude. Therefore a dechirper is highly desirable for reducing this spread down to $\sim0.1\%$ level, while at the same time for maintaining the emittance of the accelerated beam. Here we propose that a low-density hollow channel plasma can act as a near-ideal dechirper for both electrons and positrons. We demonstrate the concept through large-scale three-dimensional particle-in-cell simulations. We show that the initial positive correlated energy spread (chirp) on the beam exiting a plasma accelerator can be compensated by the nearly linear self-wake induced by the beam in the hollow channel from few percent level down to $\leq 0.1\%$. Meanwhile, the beam emittance can be preserved due to the negligible transverse field inside the channel. This passive method may significantly improve the beam quality of plasma-based accelerators, paving the way for their applications to future compact free electron lasers and colliders., Comment: 13 pages, 5 figures

Low-temperature thermal conductivity measurements were performed on single crystals of TlNi$_2$Se$_2$, a nickel-chalcogenide heavy-electron superconductor with $T_c$ $\simeq$ 3.7 K. In zero field, the residual electronic contribution at $T$ $\rightarrow$ 0 K ($\kappa_0/T$) was well separated from the total thermal conductivity, which is less than 0.45\% of its normal-state value. Such a tiny residual $\kappa_0/T$ is unlikely contributed by the nodal quasiparticles. Nodeless gap structure is supported by the very weak field dependence of $\kappa_0(H)/T$ in low magnetic fields. In the whole field range, $\kappa_0(H)/T$ exhibits an "$S$"-shape curve, as in the case of nickel pnictides BaNi$_2$As$_2$ and SrNi$_2$P$_2$. This common feature of nickel-based superconductors can be explained by multiple nodeless superconducting gaps., Comment: 5 pages, 3 figures

The thermal conductivity of the doped topological crystalline insulator, Sn$_{0.6}$In$_{0.4}$Te superconducting single crystal with $T_c =$ 4.1 K, was measured down to 50 mK. It is found that the residual linear term $\kappa_0/T$ is negligible in zero magnetic field. The $\kappa_0/T$ shows a slow field dependence at low magnetic field. These results suggest that the superconducting gap is nodeless, unless there exist point nodes with directions perpendicular to the heat current. Due to its high-symmetry fcc crystal structure of Sn$_{0.6}$In$_{0.4}$Te, however, such point nodes can be excluded. Therefore we demonstrate that this topological superconductor candidate has a full superconducting gap in the bulk. It is likely the unconventional odd-parity $A_{1u}$ state which supports a surface Andreev bound state., Comment: 5 pages, 4 figures

The specific heat and thermal conductivity of the insulating ferrimagnet Y$_3$Fe$_5$O$_{12}$ (Yttrium Iron Garnet, YIG) single crystal were measured down to 50 mK. The ferromagnetic magnon specific heat $C$$_m$ shows a characteristic $T^{1.5}$ dependence down to 0.77 K. Below 0.77 K, a downward deviation is observed, which is attributed to the magnetic dipole-dipole interaction with typical magnitude of 10$^{-4}$ eV. The ferromagnetic magnon thermal conductivity $\kappa_m$ does not show the characteristic $T^2$ dependence below 0.8 K. To fit the $\kappa_m$ data, both magnetic defect scattering effect and dipole-dipole interaction are taken into account. These results complete our understanding of the thermodynamic and thermal transport properties of the low-lying ferromagnetic magnons., Comment: 5 pages, 5 figures

We investigate the order parameter dynamics of the stripe-ordered nickelate, La$_{1.75}$Sr$_{0.25}$NiO$_4$, using time-resolved resonant X-ray diffraction. In spite of distinct spin and charge energy scales, the two order parameters' amplitude dynamics are found to be linked together due to strong coupling. Additionally, the vector nature of the spin sector introduces a longer re-orientation time scale which is absent in the charge sector. These findings demonstrate that the correlation linking the symmetry-broken states does not unbind during the non-equilibrium process, and the time scales are not necessarily associated with the characteristic energy scales of individual degrees of freedom., Comment: 4 figures. Accepted by Physical Review Letter

The thermal conductivity $\kappa$ of superconductor Ir$_{1-x}$Pt$_{x}$Te$_2$ ($x$ = 0.05) single crystal with strong spin-orbital coupling was measured down to 50 mK. The residual linear term $\kappa_0/T$ is negligible in zero magnetic field. In low magnetic field, $\kappa_0/T$ shows a slow field dependence. These results demonstrate that the superconducting gap of Ir$_{1-x}$Pt$_{x}$Te$_2$ is nodeless, and the pairing symmetry is likely conventional s-wave, despite the existence of strong spin-orbital coupling and a quantum critical point., Comment: 5 pages, 4 figures

Electronic orderings of charges, orbitals and spins are observed in many strongly correlated electron materials, and revealing their dynamics is a critical step toward understanding the underlying physics of important emergent phenomena. Here we use time-resolved resonant soft x-ray scattering spectroscopy to probe the dynamics of antiferromagnetic spin ordering in the manganite Pr$_{0.7}$Ca$_{0.3}$MnO$_3$ following ultrafast photo-exitation. Our studies reveal a glass-like recovery of the spin ordering and a crossover in the dimensionality of the restoring interaction from quasi-1D at low pump fluence to 3D at high pump fluence. This behavior arises from the metastable state created by photo-excitation, a state characterized by spin disordered metallic droplets within the larger charge- and spin-ordered insulating domains. Comparison with time-resolved resistivity measurements suggests that the collapse of spin ordering is correlated with the insulator-to-metal transition, but the recovery of the insulating phase does not depend on the re-establishment of the spin ordering., Comment: Scientific Reports, in press

Anderson localization is a general phenomenon of wave physics, which stems from the interference between multiple scattering paths1,2. It was originally proposed for electrons in a crystal, but later was also observed for light3-5, microwaves6, ultrasound7,8, and ultracold atoms9-12. Actually, in a crystal, besides electrons there may exist other quasiparticles such as magnons and spinons. However the search for Anderson localization of these magnetic excitations is rare so far. Here we report the first observation of spinon localization in copper benzoate, an ideal compound of spin-1/2 antiferromagnetic Heisenberg chain, by ultra-low-temperature specific heat and thermal conductivity measurements. We find that while the spinon specific heat Cs displays linear temperature dependence down to 50 mK, the spinons thermal conductivity ks only manifests the linear temperature dependence down to 300 mK. Below 300 mK, ks/T decreases rapidly and vanishes at about 100 mK, which is a clear evidence for Anderson localization. Our finding opens a new window for studying such a fundamental phenomenon in condensed matter physics., Comment: 17 pages, including 4 figures

High-quality K(Fe$_{1-x}$Co$_x$)$_2$As$_2$ single crystals have been grown by using KAs flux method. Instead of increasing the superconducting transition temperature $T_{\rm c}$ through electron doping, we find that Co impurities rapidly suppress $T_{\rm c}$ down to zero at only $x \approx$ 0.04. Such an effective suppression of $T_{\rm c}$ by impurities is quite different from that observed in Ba$_{0.5}$K$_{0.5}$Fe$_2$As$_2$ with multiple nodeless superconducting gaps. Thermal conductivity measurements in zero field show that the residual linear term $\kappa_0/T$ only change slightly with $3.4\%$ Co doping, despite the sharp increase of scattering rate. The implications of these anomalous impurity effects are discussed., Comment: 5 pages, 4 figs

The dynamics of an order parameter's amplitude and phase determines the collective behaviour of novel states emerged in complex materials. Time- and momentum-resolved pump-probe spectroscopy, by virtue of its ability to measure material properties at atomic and electronic time scales and create excited states not accessible by the conventional means can decouple entangled degrees of freedom by visualizing their corresponding dynamics in the time domain. Here, combining time-resolved femotosecond optical and resonant x-ray diffraction measurements on striped La1.75Sr0.25NiO4, we reveal unforeseen photo-induced phase fluctuations of the charge order parameter. Such fluctuations preserve long-range order without creating topological defects, unlike thermal phase fluctuations near the critical temperature in equilibrium10. Importantly, relaxation of the phase fluctuations are found to be an order of magnitude slower than that of the order parameter's amplitude fluctuations, and thus limit charge order recovery. This discovery of new aspect to phase fluctuation provides more holistic view for the importance of phase in ordering phenomena of quantum matter., Comment: 23 pages, 6 figures. Published version can be found at Nature Communications 3, 838 (2012)

The thermal conductivity of optimally doped NaFe$_{0.972}$Co$_{0.028}$As ($T_c \sim$ 20 K) and overdoped NaFe$_{0.925}$Co$_{0.075}$As ($T_c \sim$ 11 K) single crystals were measured down to 50 mK. No residual linear term $\kappa_0/T$ is found in zero magnetic field for both compounds, which is an evidence for nodeless superconducting gap. Applying field up to $H$ = 9 T ($\approx H_{c2}/4$) does not noticeably increase $\kappa_0/T$ in NaFe$_{1.972}$Co$_{0.028}$As, which is consistent with multiple isotropic gaps with similar magnitudes. The $\kappa_0/T$ of overdoped NaFe$_{1.925}$Co$_{0.075}$As shows a relatively faster field dependence, indicating the increase of the ratio between the magnitudes of different gaps, or the enhancement of gap anisotropy upon increasing doping., Comment: 5 pages, 4 figures

We report resistivity $\rho$ and thermal conductivity $\kappa$ measurements on Ca$_3$Ir$_4$Sn$_{13}$ single crystals, in which superconductivity with $T_c \approx 7$ K was claimed to coexist with ferromagnetic spin-fluctuations. Among three crystals, only one crystal shows a small hump in resistivity near 20 K, which was previously attributed to the ferromagnetic spin-fluctuations. Other two crystals show the $\rho \sim T^2$ Fermi-liquid behavior at low temperature. For both single crystals with and without the resistivity anomaly, the residual linear term $\kappa_0/T$ is negligible in zero magnetic field. In low fields, $\kappa_0(H)/T$ shows a slow field dependence. These results demonstrate that the superconducting gap of Ca$_3$Ir$_4$Sn$_{13}$ is nodeless, thus rule out nodal gap caused by ferromagnetic spin-fluctuations., Comment: 5 pages, 4 figures

We present the ultra-low-temperature heat transport study of iron-based superconductors Ba(Fe$_{1-x}$Ru$_x$)$_2$As$_2$ and BaFe$_2$(As$_{1-x}$P$_x$)$_2$. For optimally doped Ba(Fe$_{0.64}$Ru$_{0.36}$)$_2$As$_2$, a large residual linear term $\kappa_0/T$ at zero field and a $\sqrt{H}$ dependence of $\kappa_0(H)/T$ are observed, which provide strong evidences for nodes in the superconducting gap. This result demonstrates that the isovalent Ru doping can also induce nodal superconductivity, as P does in BaFe$_2$(As$_{0.67}$P$_{0.33}$)$_2$. Furthermore, in underdoped Ba(Fe$_{0.77}$Ru$_{0.23}$)$_2$As$_2$ and heavily underdoped BaFe$_2$(As$_{0.82}$P$_{0.18}$)$_2$, $\kappa_0/T$ manifests similar nodal behavior, which shows the robustness of nodal superconductivity in the underdoped regime and puts constraint on theoretical models., Comment: 5 pages, 4 figures - with two underdoped samples added, this paper supersedes arXiv:1106.5417

We present the ultra-low-temperature heat transport study of an iron-based superconductor Ba(Fe$_{0.64}$Ru$_{0.36}$)$_2$As$_2$ ($T_c$ = 20.2 K), in which the superconductivity is induced by isovalent Ru substitution. In zero field we find a large residual linear term $\kappa_0/T$, more than 40% of the normal-state value. At low field, the $\kappa_0/T$ shows an $H^{1/2}$ dependence. These provide strong evidences for nodes in the superconducting gap of Ba(Fe$_{0.64}$Ru$_{0.36}$)$_2$As$_2$, which mimics that in another isovalently substituted superconductor BaFe$_2$(As$_{1-x}$P$_x$)$_2$. Our results show that the isovalent Ru substitution can also induce nodal superconductivity in BaFe$_2$As$_2$, as P does, and they may have the same origin. We further compare them with other two nodal superconductors LaFePO and LiFeP., Comment: 4 pages, 4 figures

We present resonant soft X-ray scattering (RSXS) results from small band width manganites (Pr,Ca)MnO$_3$, which show that the CE-type spin ordering (SO) at the phase boundary is stabilized only below the canted antiferromagnetic transition temperature and enhanced by ferromagnetism in the macroscopically insulating state (FM-I). Our results reveal the fragility of the CE-type ordering that underpins the colossal magnetoresistance (CMR) effect in this system, as well as an unexpected cooperative interplay between FM-I and CE-type SO which is in contrast to the competitive interplay between the ferromagnetic metallic (FM-M) state and CE-type ordering., Comment: Accepted for publication in Phys. Rev. Lett

Quantum phase transitions occur at zero temperature upon variation of some nonthermal control parameters. The Ising chain in a transverse field is probably the most-studied model undergoing such a transition, from ferromagnetic to paramagnetic state1,2. This model can be exactly solved by using a Jordan-Wigner transformation, which transforms the spins into noninteracting spinless fermions1. At the quantum critical point, the magnetic excitations can carry arbitrarily low energy and dominate the low temperature properties. Here we report the unveiling of such quantum critical point in quasi-one-dimensional Ising ferromagnet CoNb2O6 by ultra-low-temperature thermal conductivity measurements. We find that in the paramagnetic state, phonons are scattered by the magnetic excitations above certain temperature Ts, which corresponds to a gap. As predicted by the theoretical model1, this gap linearly goes to zero with decreasing the transverse field, thus determining the quantum critical point of the Ising chain., Comment: 14 pages, 3 figures

The interplay between magnetism and superconductivity has been a central issue in unconventional superconductors. While the dynamic magnetism could be the source of electron pairing, the static magnetism is generally believed to compete with superconductivity. In this sense, the observation of Q phase, the coupled spin-density wave order and superconductivity, in the heavy-fermion superconductor CeCoIn5 is very puzzling. Whether this Q phase origins from the novel Fulde-Ferrel-Larkin-Ovchinnikov state is under hot debate. Here we report the resistivity and thermal conductivity study of a newly discovered heavy-fermion superconductor Ce2PdIn8 down to 50 mK. We find an unusual field-induced quantum critical point at the upper critical field Hc2 and unconventional nodal superconductivity in Ce2PdIn8. The jump of thermal conductivity k(H)/T near Hc2 suggests a first-order-like phase transition at low temperatures. These results mimic the features of the Q phase in CeCoIn5, implying that Ce2PdIn8 is another promising compound to investigate the exotic Q phase and FFLO state. The comparison between CeCoIn5 and Ce2PdIn8 may help to clarify the origin of the Q phase., Comment: 18 pages, 4 figures

Reply to comment by T. Terashima et al. on "Quantum criticality and nodal superconductivity in the FeAs-based superconductor KFe$_2$As$_2$", Comment: 1 page, 1 figure, to appear in Phys. Rev. Lett

The in-plane resistivity $\rho$ and thermal conductivity $\kappa$ of FeAs-based superconductor KFe$_2$As$_2$ single crystal were measured down to 50 mK. We observe non-Fermi-liquid behavior $\rho(T) \sim T^{1.5}$ at $H_{c_2}$ = 5 T, and the development of a Fermi liquid state with $\rho(T) \sim T^2$ when further increasing field. This suggests a field-induced quantum critical point, occurring at the superconducting upper critical field $H_{c_2}$. In zero field there is a large residual linear term $\kappa_0/T$, and the field dependence of $\kappa_0/T$ mimics that in d-wave cuprate superconductors. This indicates that the superconducting gaps in KFe$_2$As$_2$ have nodes, likely d-wave symmetry. Such a nodal superconductivity is attributed to the antiferromagnetic spin fluctuations near the quantum critical point., Comment: 4 pages, 4 figures - replaces arXiv:0909.4855

The in-plane resistivity $\rho$ and thermal conductivity $\kappa$ of extremely overdoped KFe$_2$As$_2$ ($T_c$ = 3.0 K) single crystal were studied. It is found that $\rho \sim T^{1.5}$ at low temperature, a typical non-Fermi liquid behavior of electrons scattered by antiferromagnetic spin fluctuations. In zero field, we observed a large residual linear term $\kappa_0/T$, about one third of the normal-state value. In low magnetic fields, $\kappa_0/T(H)$ increases very fast. Such a behavior of $\kappa_0/T$ mimics the d-wave cuprate superconductors, therefore provides clear evidence for nodes in the superconducting gap of KFe$_2$As$_2$. Based on the Fermi surface topology of KFe$_2$As$_2$, it is believed that the dominant intraband pairing via antiferromagnetic spin fluctuations results in the unconventional superconducting gap with nodes., Comment: This paper is replaced by arXiv:0910.2806, which includes a detailed study of the quantum criticality in KFe2As2. The paper arXiv:0910.2806 supersedes this paper

We study the stability of various kinds of graphene samples under soft X-ray irradiation. Our results show that in single layer exfoliated graphene (a closer analogue to two dimensional material), the in-plane carbon-carbon bonds are unstable under X-ray irradiation, resulting in nanocrystalline structures. As the interaction along the third dimension increases by increasing the number of graphene layers or through the interaction with the substrate (epitaxial graphene), the effect of X-ray irradiation decreases and eventually becomes negligible for graphite and epitaxial graphene. Our results demonstrate the importance of the interaction along the third dimension in stabilizing the long range in-plane carbon-carbon bonding, and suggest the possibility of using X-ray to pattern graphene nanostructures in exfoliated graphene., Comment: 4 pages, 3 figures, Phys. Rev. B rapid communication, in press

The in-plane thermal conductivity $\kappa$ of overdoped FeAs-based superconductor BaFe$_{1.73}$Co$_{0.27}$As$_2$ ($T_c$ = 8.1 K) single crystal was measured down to 80 mK. In zero field, the residual linear term $\kappa_0/T$ is negligible, suggesting a nodeless superconducting gap in the $ab$-plane. In magnetic field, $\kappa_0/T$ increases rapidly, very different from that of conventional s-wave superconductors. This anomalous $\kappa_0/T(H)$ may reveal an exotic superconducting gap structure in overdoped BaFe$_{1.73}$Co$_{0.27}$As$_2$: the vanishing hole ($\beta$) pocket has a much larger gap than the electron ($\gamma$ and $\delta$) pockets which contain most of the carriers. Such an exotic gap structure is an evidence for superconducting state induced by interband interactions, in which the band with the {\it smaller} density of states has a {\it larger} gap., Comment: 5 pages, 3 figures

The in-plane thermal conductivity $\kappa$ of the iron selenide superconductor FeSe$_x$ ($T_c$ = 8.8 K) were measured down to 120 mK and up to 14.5 T ($\simeq 3/4 H_{c2}$). In zero field, the residual linear term $\kappa_0/T$ at $ T \to 0$ is only about 16 $\mu$W K$^{-2}$ cm$^{-1}$, less than 4% of its normal state value. Such a small $\kappa_0/T$ does not support the existence of nodes in the superconducting gap. More importantly, the field dependence of $\kappa_0/T$ in FeSe$_x$ is very similar to that in NbSe$_2$, a typical multi-gap s-wave superconductor. We consider our data as strong evidence for multi-gap nodeless superconductivity in FeSe$_x$. This kind of superconducting gap structure may be generic for all Fe-based superconductors., Comment: 5 pages, 4 figures

The in-plane thermal conductivity $\kappa$ of electron-doped iron-arsenide superconductor BaFe$_{1.9}$Ni$_{0.1}$As$_2$ ($T_c$ = 20.3 K) single crystal was measured down to 70 mK. In zero field, the absence of a residual linear term $\kappa_0/T$ at $ T \to 0$ is strong evidence for nodeless superconducting gap. In magnetic field, $\kappa_0/T$ shows a slow field dependence up to $H$ = 14.5 T ($\approx$ 30% $H_{c_2}$). This is consistent with the superconducting gap structure demonstrated by angle-resolved photoemission spectroscopy experiments in BaFe$_{1.85}$Co$_{0.15}$As$_2$ ($T_c$ = 25.5 K), where isotropic superconducting gaps with similar size on hole and electron pockets were observed., Comment: In-field data re-measured with sample cooled in magnetic field from above Tc

We study the broadband optical conductivity and ultrafast carrier dynamics of epitaxial graphene in the few-layer limit. Equilibrium spectra of nominally buffer, monolayer, and multilayer graphene exhibit significant terahertz and near-infrared absorption, consistent with a model of intra- and interband transitions in a dense Dirac electron plasma. Non-equilibrium terahertz transmission changes after photoexcitation are shown to be dominated by excess hole carriers, with a 1.2-ps mono-exponential decay that reflects the minority-carrier recombination time., Comment: 4 pages, 3 figures, final version

Self-doping in graphene has been studied by examining single-layer epitaxially grown graphene samples with differing characteristic lateral terrace widths. Low energy electron microscopy was used to gain real-space information about the graphene surface morphology, which was compared with data obtained by angle-resolved photoemission spectroscopy to study the effect of the monolayer graphene terrace width on the low energy dispersions. By altering the graphene terrace width, we report significant changes in the electronic structure and quasiparticle relaxation time of the material, in addition to a terrace width-dependent doping effect., Comment: Published in Applied Physics Letters 93, 243119 (2008)

The interplay of electron-phonon (el-ph) and electron-electron (el-el) interactions in epitaxial graphene is studied by directly probing its electronic structure. We found a strong coupling of electrons to the soft part of the A1g phonon evident by a kink at 150+/-15 meV, while the coupling of electrons to another expected phonon E2g at 195 meV can only be barely detected. The possible role of the el-el interaction to account for the enhanced coupling of electrons to the A1g phonon, and the contribution of el-ph interaction to the linear imaginary part of the self energy at high binding energy are also discussed. Our results reveal the dominant role of the A1g phonon in the el-ph interaction in graphene, and highlight the important interplay of el-el and el-ph interactions in the self energy of graphene., Comment: accepted to Phys. Rev. B

The capability to control the type and amount of charge carriers in a material and, in the extreme case, the transition from metal to insulator is one of the key challenges of modern electronics. By employing angle resolved photoemission spectroscopy (ARPES) we find that a reversible metal to insulator transition and a fine tuning of the charge carriers from electrons to holes can be achieved in epitaxial bilayer and single layer graphene by molecular doping. The effects of electron screening and disorder are also discussed. These results demonstrate that epitaxial graphene is suitable for electronics applications, as well as provide new opportunities for studying the hole doping regime of the Dirac cone in graphene., Comment: 4 pages, 4 figures

By performing angle-resolved photoemission spectroscopy of the bilayer colossal magnetoresistive (CMR) manganite, $La_{2-2x}Sr_{1+2x}Mn_{2}O_{7}$, we provide the complete mapping of the Fermi level spectral weight topology. Clear and unambiguous bilayer splitting of the in-plane 3d$_{x^2-y^2}$ band, mapped throughout the Brillouin zone, and the full mapping of the 3d$_{3z^2-r^2}$ band are reported. Peculiar doping and temperature dependencies of these bands imply that as transition from the ferromagnetic metallic phase approaches, either as a function of doping or temperature, coherence along the c-axis between planes within the bilayer is lost, resulting in reduced interplane coupling. These results suggest that interplane coupling plays a large role in the CMR transition., Comment: 8 pages, 6 figures

We studied the effect of quantum confinement on the size of the band gap in single layer epitaxial graphene. Samples with different graphene terrace sizes are studied by using low energy electron microscopy (LEEM) and angle-resolved photoemission spectroscopy (ARPES). The direct correlation between the terrace size extracted from LEEM and the gap size extracted from ARPES shows that quantum confinement alone cannot account for the large gap observed in epitaxial graphene samples.

The pi bands of epitaxially grown graphene are studied by using high resolution angle resolved photoemission spectroscopy. Clear deviations from the conical dispersion expected for massless Dirac fermions and an anomalous increase of the scattering rate are observed in the vicinity of the Dirac point energy. Possible explanations for such anomalies are discussed in terms of many-body interactions and the opening of a gap. We present detailed experimental evidences in support of the gap scenario. This finding reveals a fundamental intrinsic property of epitaxial graphene and demonstrates the possibility of engineering the band gap in epitaxial graphene., Comment: 5 pages, 5 figures

Graphene has shown great application potentials as the host material for next generation electronic devices. However, despite its intriguing properties, one of the biggest hurdles for graphene to be useful as an electronic material is its lacking of an energy gap in the electronic spectra. This, for example, prevents the use of graphene in making transistors. Although several proposals have been made to open a gap in graphene's electronic spectra, they all require complex engineering of the graphene layer. Here we show that when graphene is epitaxially grown on the SiC substrate, a gap of ~ 0.26 is produced. This gap decreases as the sample thickness increases and eventually approaches zero when the number of layers exceeds four. We propose that the origin of this gap is the breaking of sublattice symmetry owing to the graphene-substrate interaction. We believe our results highlight a promising direction for band gap engineering of graphene., Comment: 10 pages, 4 figures; updated references

With the current interest in the rare-earth tellurides as high temperature charge density wave materials, a greater understanding of the physics of these systems is needed, particularly in the case of the ditellurides. We report a detailed study of the band structure of LaTe_2 in the charge density wave state using high-resolution angle resolved photoemission spectroscopy (ARPES). From this work we hope to provide insights into the successes and weaknesses of past theoretical study as well as helping to clear up prior ambiguities by providing an experimental basis for future work in the tellurides., Comment: 6 pages, 7 figures, Proceedings of the ICESS 10(August 2006), Journal of Electron Spectroscopy and Related Phenomena - Published May 2007

We present the first direct study of charge density wave (CDW) formation in quasi-2D single layer LaTe_2 using high-resolution angle resolved photoemission spectroscopy (ARPES) and low energy electron diffraction (LEED). CDW formation is driven by Fermi surface (FS) nesting, however characterized by a surprisingly smaller gap (50meV) than seen in the double layer RTe_3 compounds, extending over the entire FS. This establishes LaTe_2 as the first reported semiconducting 2D CDW system where the CDW phase is FS nesting driven. In addition, the layer dependence of this phase in the tellurides and the possible transition from a stripe to a checkerboard phase is discussed., Comment: 4 pages, 4 figures, Published in Phys. Rev. Lett

We discuss the nature of electron-lattice interaction in optimally doped Bi$_2$Sr$_2$CaCu$_2$O$_{8+\delta}$ samples, using isotope effect (IE) in angle resolved photoemission spectroscopy (ARPES) data. The IE in the ARPES line width and the IE in the ARPES dispersion are both quite large, implying a strong electron-lattice correlation. The strength of the electron-lattice interaction is ``intermediate,'' i.e. stronger than the Migdal-Eliashberg regime but weaker than the small polaron regime, requiring a more general picture of the ARPES ``kink'' than the commonly used Migdal-Eliashberg picture. The two IEs also imply a complex interaction, due to their strong momentum dependence and their differing sign behaviors. In sum, we propose an intermediate-strength coupling of electrons to localized lattice vibrations via charge density fluctuations.

In this paper, we present a high resolution angle resolved photoemission spectroscopy (ARPES) study of the electronic properties of graphite. We found that the nature of the low energy excitations in graphite is particularly sensitive to interlayer coupling as well as lattice disorder. As a consequence of the interlayer coupling, we observed for the first time the splitting of the $\pi$ bands by $\approx$ 0.7 eV near the Brillouin zone corner K. At low binding energy, we observed signatures of massless Dirac fermions with linear dispersion (as in the case of graphene), coexisting with quasiparticles characterized by parabolic dispersion and finite effective mass. We also report the first ARPES signatures of electron-phonon interaction in graphite: a kink in the dispersion and a sudden increase in the scattering rate. Moreover, the lattice disorder strongly affects the low energy excitations, giving rise to new localized states near the Fermi level. These results provide new insights on the unusual nature of the electronic and transport properties of graphite., Comment: 10 pages, 15 figures

Originating from relativistic quantum field theory, Dirac fermions have been recently applied to study various peculiar phenomena in condensed matter physics, including the novel quantum Hall effect in graphene, magnetic field driven metal-insulator-like transition in graphite, superfluid in 3He, and the exotic pseudogap phase of high temperature superconductors. Although Dirac fermions are proposed to play a key role in these systems, so far direct experimental evidence of Dirac fermions has been limited. Here we report the first direct observation of massless Dirac fermions with linear dispersion near the Brillouin zone (BZ) corner H in graphite, coexisting with quasiparticles with parabolic dispersion near another BZ corner K. In addition, we report a large electron pocket which we attribute to defect-induced localized states. Thus, graphite presents a novel system where massless Dirac fermions, quasiparticles with finite effective mass, and defect states all contribute to the low energy electronic dynamics., Comment: Nature Physics, in press

A universal high energy anomaly in the single particle spectral function is reported in three different families of high temperature superconductors by using angle-resolved photoemission spectroscopy. As we follow the dispersing peak of the spectral function from the Fermi energy to the valence band complex, we find dispersion anomalies marked by two distinctive high energy scales, E_1=~ 0.38 eV and E_2=~0.8 eV. E_1 marks the energy above which the dispersion splits into two branches. One is a continuation of the near parabolic dispersion, albeit with reduced spectral weight, and reaches the bottom of the band at the gamma point at ~0.5 eV. The other is given by a peak in the momentum space, nearly independent of energy between E_1 and E_2. Above E_2, a band-like dispersion re-emerges. We conjecture that these two energies mark the disintegration of the low energy quasiparticles into a spinon and holon branch in the high T_c cuprates., Comment: accepted for publication in Phys. Rev. Lett

This paper reports the synthesis and detailed characterization of graphite thin films produced by thermal decomposition of the (0001) face of a 6H-SiC wafer, demonstrating the successful growth of single crystalline films down to approximately one graphene layer. The growth and characterization were carried out in ultrahigh vacuum (UHV) conditions. The growth process and sample quality were monitored by low-energy electron diffraction, and the thickness of the sample was determined by core level x-ray photoelectron spectroscopy. High-resolution angle-resolved photoemission spectroscopy shows constant energy map patterns, which are very sharp and fully momentum-resolved, but nonetheless not resolution limited. We discuss the implications of this observation in connection with scanning electron microscopy data, as well as with previous studies.

Angle resolved photoelectron spectroscopy (ARPES) on azimuthally disordered graphite demonstrates that sharp quasiparticle dispersions along the radial direction can coexist with a complete lack of dispersion along the azimuthal direction. This paradoxical coexistence can be explained in terms of van Hove singularities in the angular density of states. In addition, nondispersive features at the energies of band maxima and saddle points are observed and possible explanations are discussed. This work opens a possibility of studying the electronic structure of layered materials using ARPES even when large single crystals are difficult to obtain., Comment: 4 pages, 3 figures

The joint density of states (JDOS) of Bi2Sr2CaCu2O8+x is calculated by evaluating the autocorrelation of the single particle spectral function A(k,omega) measured from angle resolved photoemission spectroscopy (ARPES). These results are compared with Fourier transformed (FT) conductance modulations measured by scanning tunneling microscopy (STM). Good agreement between the two experimental probes is found for two different doping values examined. In addition, by comparing the FT-STM results to the autocorrelated ARPES spectra with different photon polarization, new insight on the form of the STM matrix elements is obtained. This shines new light on unsolved mysteries in the tunneling data., Comment: Revised now available at: Phys. Rev. Lett. 96, 067005 (2006)

The sudden change of the velocity, so-called "kink," of the dispersing peak in angle resolved photoelectron spectroscopy is a well-known feature in the high temperature superconducting cuprates. Currently, the origin of the kink is being much debated, but a consensus has not emerged yet. Here, we present a study of the momentum evolution of the kink structure from the nodal region towards the anti-nodal region, for optimally doped Bi2212 sample. We show that the observed temperature dependence of the kink structure in both regions of the momentum space is consistent with a scenario in which phonons contribute strongly to the kink.

In conventional superconductors, the electron pairing that allows superconductivity is caused by exchange of virtual phonons, which are quanta of lattice vibration. For high-transition-temperature (high-Tc) superconductors, it is far from clear that phonons are involved in the pairing at all. For example, the negligible change in Tc of optimally doped Bi2Sr2CaCu2O8 (Bi2212) upon oxygen isotope substitution (16O to 18O leads to Tc decreasing from 92 to 91 K) has often been taken to mean that phonons play an insignificant role in this material. Here we provide a detailed comparison of the electron dynamics of Bi2212 samples containing different oxygen isotopes, using angle-resolved photoemission spectroscopy. Our data show definite and strong isotope effects. Surprisingly, the effects mainly appear in broad high-energy humps, commonly referred to as "incoherent peaks". As a function of temperature and electron momentum, the magnitude of the isotope effect closely correlates with the superconducting gap - that is, the pair binding energy. We suggest that these results can be explained in a dynamic spin-Peierls picture, where the singlet pairing of electrons and the electron-lattice coupling mutually enhance each other.