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45. New insights into sulfite activation by amorphous Fe1−xNixS for RhB removal: the synergistic effect of free radical and non-free radical pathway.

Author

Zhang, Jinyuan, Xing, Ziqin, Liu, Jianxin, Wang, Yawen, Zhang, Xiaochao, Li, Rui, Wang, Yunfang, and Fan, Caimei

Subjects
FREE radicals, RADICALS (Chemistry), ORGANIC water pollutants, HETEROGENEOUS catalysts, CHARGE exchange, RHODAMINE B
Abstract

Advanced oxysulfur radical-based advanced oxidation processes (OSR-AOPs) usually use heterogeneous catalysts to activate sulfite to degrade organic pollutants in water. In this study, we report the mechanism of sulfite activation by amorphous Fe1−xNixS to degrade rhodamine B (RhB) in different pH ranges. Compared with FeS, Fe1−xNixS had a wide pH application range and high activity. For Fe1−xNixS, Ni-doping sped up electron transfer inside the catalyst and the reduced S2− promoted the ≡Fe(III)/≡Fe(II) cycle, which together improved the sulfite activation by Fe1−xNixS. The results indicated a pH dependence of RhB degradation in the Fe1−xNixS/sulfite system. The free radical pathway of SO3˙−, SO5˙− and ˙OH generated in the process was dominant under acidic condition, whereas it was mainly a non-free radical pathway of electron transfer between the catalyst and the pollutant under alkaline conditions. Both free radical and non-free radical pathways existed in Fe1−xNixS/sulfite under neutral conditions. The results shed significant light on promoting sulfite-based AOPs to remove pollutants from water. [ABSTRACT FROM AUTHOR]

Published
2024
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46. Disentangling the Spatiotemporal Dynamics, Drivers, and Recovery of NPP in Co-Seismic Landslides: A Case Study of the 2017 Jiuzhaigou Earthquake, China.

Author

Duan, Yuying, Pei, Xiangjun, Luo, Jing, Zhang, Xiaochao, and Luo, Luguang

Subjects
MODIS (Spectroradiometer), GRASSLAND restoration, EARTHQUAKES, WORLD Heritage Sites, ECOLOGICAL resilience, LANDSLIDES
Abstract

The 2017 Jiuzhaigou earthquake, registering a magnitude of 7.0, triggered a series of devastating geohazards, including landslides, collapses, and mudslides within the Jiuzhaigou World Natural Heritage Site. These destructive events obliterated extensive tracts of vegetation, severely compromising carbon storage in the terrestrial ecosystems. Net Primary Productivity (NPP) reflects the capacity of vegetation to absorb carbon dioxide. Accurately assessing changes in NPP is crucial for unveiling the recovery of terrestrial ecosystem carbon storage after the earthquake. To this end, we designed this study using the Moderate Resolution Imaging Spectroradiometer (MODIS) Net Primary Productivity datasets. The findings are as follows. NPP in the co-seismic landslide areas remained stable between 525 and 575 g C/m2 before the earthquake and decreased to 533 g C/m2 after the earthquake. This decline continued, reaching 483 g C/m2 due to extreme rainfall events in 2018, 2019, and 2020. Recovery commenced in 2021, and by 2022, NPP had rebounded to 544 g C/m2. The study of NPP recovery rate revealed that, five years after the earthquake, only 18.88% of the co-seismic landslide areas exhibited an NPP exceeding the pre-earthquake state. However, 17.14% of these areas had an NPP recovery rate of less than 10%, indicating that recovery has barely begun in most areas. The factor detector revealed that temperature, precipitation, and elevation significantly influenced NPP recovery. Meanwhile, the interaction detector highlighted that lithology, slope, and aspect also played crucial roles when interacting with other factors. Therefore, the recovery of NPP is not determined by a single factor, but rather by the interactions among various factors. The ecosystem resilience study demonstrated that the current recovery of NPP primarily stems from the restoration of grassland ecosystems. Overall, while the potential for NPP recovery in co-seismic landslide areas is optimistic, it will require a considerable amount of time to return to the pre-earthquake state. [ABSTRACT FROM AUTHOR]

Published
2024
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