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Inference of joule-class THz radiation sources from microchannel targets driven with hundreds of joule, picosecond lasers is reported. THz sources of this magnitude are useful for nonlinear pumping of matter and for charged-particle acceleration and manipulation. Microchannel targets demonstrate increased laser-THz conversion efficiency compared to planar foil targets, with laser energy to THz energy conversion up to approximately 0.9% in the best cases., Comment: 9 pages, 2 figures

We report a systematic investigation into the processes behind a near hundredfold enhanced second harmonic wave generated from a laser-induced air plasma, by examining the temporal dynamics of the frequency conversion processes, and the polarization of the emitted second harmonic beam. Contrary to typical nonlinear optical processes, the enhanced second harmonic generation efficiency is only observed within a sub-picosecond time window and found to be nearly constant across fundamental pulse durations spanning from 0.1 ps to over 2 ps. We further demonstrate that with the adopted orthogonal pump-probe configuration, the polarization of second harmonic field exhibits a complex dependence on the polarization of both input fundamental beams, contrasting with most of the previous experiments with a single-beam geometry.

A highly adaptable and robust THz energy meter has been designed and implemented to detect energetic THz pulses from high intensity (greater than 1E18 watts per square centimeter) laser plasma interactions on OMEGA EP. THz radiation from the laser driven target is detected by a shielded pyrometer. A second identical pyrometer is used for background subtraction. The detector can be configured to detect THz pulses in the 1 mm to 30 microns (0.3 to 10 THz) range and pulse energies from joules to microjoules via changes in filtration, aperture size and position. Additional polarization selective filtration can also be used to determine THz pulse polarization. The design incorporates significant radiation and EMP shielding to survive and operate within the OMEGA EP radiation environment. We describe the design, operational principle, calibration and testing of the THz energy meter. The pyrometers were calibrated using a benchtop laser and show linear sensitivity up to 1000 nJ of absorbed energy. Initial results from four OMEGA EP THz experiments detected up to 15 microjoules at the detector, which can correspond to 100s of mJ depending on THz emission and reflection models.

Terahertz wave emission from condensed matter excited by intense laser pulses not only reflects the details in laser-matter interaction but also offers bright terahertz wave sources. Flowing liquid targets possess the advantage of providing a fresh area for each laser pulse. To demonstrate a debris-free target under laser excitation, we investigate the use of liquid nitrogen as a target. By creating a flowing liquid nitrogen line in the ambient environment, we successfully observe broadband terahertz wave emission under short pulse excitation. Our cryogenic line is able to sustain the excitation of a high-repetition-rate (1 kHz) laser. The terahertz peak field emitted from liquid nitrogen is comparable to that from liquid water, yet a broader bandwidth is observed. This demonstration prompts new opportunities in choosing potential materials for studying terahertz wave generation process and in understanding laser-induced ionization in different liquids., Comment: 16 pages, 4 figures

We experimentally show the spectrally averaged nonlinear refractive index and absorption coefficient for liquid water, water vapor, {\alpha}-pinene, and Si using a full-phase analysis in the terahertz regime through a standard time-domain spectrometer. Our results confirm that the nonlinear index of refraction of the liquid samples in this regime exceeds the near-infrared optical nonlinear index by six orders of magnitude. In the case of liquid water and water vapor at atmospheric pressure, we find a nonlinear index of 7.8x10^-10 cm^2/W and 6x10^-11 cm^2/W respectively, which are both much larger than expected., Comment: 5 pages, 2 figures, 1 table

Metals have been studied as terahertz sources for decades. Recent research has shown the potential of metals in generating extremely high THz pulse energy excited by intense laser pulses. To avoid the metal surface debris caused by laser pulses, here, we report the results of the broadband terahertz wave emission from a flowing liquid metal line excited by sub-picosecond laser pulses. The THz signal emitted from the liquid gallium line shows stronger field with broader bandwidth comparing with the signal from water under the identical optical excitation conditions. Our preliminary study suggests that the liquid metals have the potential to serve as efficient and powerful THz sources for the intense lasers with a high repetition rate.

The values of the nonlinear refractive index coefficient for various materials in the terahertz frequency range exceed the ones in both visible and NIR ranges by several orders of magnitude. We report the direct measurement of the nonlinear refractive index coefficient of liquid water by using the Z-scan method with broadband pulsed THz beam. Our experimental result shows that nonlinear refractive index coefficient in water is positive and can be as large as 3.5$\times$10$^{-10}$ cm$^{2}$/W in the THz frequency range, which exceeds the ones for the visible and NIR ranges by 6 orders of magnitude., Comment: 7 pages, 3 figures

Terahertz radiation generation from liquid water has long been considered to be impossible due to strong absorption. A few very recent works reported terahertz generation from water, but the mechanism is not clear and the efficiency demands to be enhanced. We show experimentally that strong single-cycle terahertz radiation with field strength of $\rm 0.2~MV cm^{-1}$ is generated from a water line/column of $\sim 200 \mu m$ in diameter irradiated by a mJ femtosecond laser beam. This strength is 100-fold higher than that produced from air. We attribute the mechanism to the laser-ponderomotive-force-induced current with the symmetry broken around the water-column interface. This mechanism can explain our following observations: the radiation can be generated only when the laser propagation axis deviates from the column center; the deviation determines its field strength and polarity; it is always p-polarized no matter whether the laser is p- or s-polarized. This study provides a simple and efficient scheme of table-top terahertz sources based on liquid water., Comment: 4 figures

In the widely-studied two-color laser scheme for terahertz (THz) radiation from a gas, the frequency ratio of the two lasers is usually fixed at $\omega_2/\omega_1=$1:2. We investigate THz generation with uncommon frequency ratios. Our experiments show, for the first time, efficient THz generation with new ratios of $\omega_2/\omega_1=$1:4 and 2:3. We observe that the THz polarization can be adjusted by rotating the longer-wavelength laser polarization and the polarization adjustment becomes inefficient by rotating the other laser polarization; the THz energy shows similar scaling laws with different frequency ratios. These observations are inconsistent with multi-wave mixing theory, but support the gas-ionization model. This study pushes the development of the two-color scheme and provides a new dimension to explore the long-standing problem of the THz generation mechanism., Comment: 6 pages, 3 figures

We report on the broadband THz response of InGaAs/GaAs HEMTs operating at 1.63 THz and room temperature deep in the saturation regime. We demonstrate that responses show linear increase with drain-to-source voltage (or drain bias current) and reach very high values up to 170V/W. We also develop a phenomenological theory valid both in the ohmic and in the saturation regimes., Comment: 11 pages, 3 figures

In modern terahertz (THz) sensing and imaging spectroscopy, water is considered a nemesis to be avoided due to strong absorption in the THz frequency range. Here we report the first experimental demonstration and theoretical implications of using femtosecond laser pulses to generate intense broadband THz emission from water vapor. When we focused an intense laser pulse in water vapor contained in a gas cell or injected from a gas jet nozzle, an extraordinarily strong THz field from optically excited water vapor is observed. Water vapor has more than 50% greater THz generation efficiency than dry nitrogen. It had previously been assumed that the nonlinear generation of THz waves in this manner primarily involves a free-electron plasma, but we show that the molecular structure plays an essential role in the process. In particular, we found that THz wave generation from H2O vapor is significantly stronger than that from D2O vapor. Vibronic activities of water cluster ions, occurring naturally in water vapor, may possibly contribute to the observed isotope effect along with rovibrational contributions from the predominant monomers., Comment: 5 pages, 4 figures

In condensed matter physics, the study of electronic states with SU(N) symmetry has attracted considerable and growing attention in recent years, as systems with such a symmetry can often have a spontaneous symmetry-breaking effect giving rise to a novel ground state. For example, pseudospin quantum Hall ferromagnet of broken SU(2) symmetry has been realized by bringing two Landau levels close to degeneracy in a bilayer quantum Hall system. In the past several years, the exploration of collective states in other multi-component quantum Hall systems has emerged. Here we show the conventional pseudospin quantum Hall ferromagnetic states with broken SU(2) symmetry collapsed rapidly into an unexpected state with broken SU(4) symmetry, by in-plane magnetic field in a two-subband GaAs/AlGaAs two-dimensional electron system at filling factor around $\nu=4$. Within a narrow tilting range angle of 0.5 degrees, the activation energy increases as much as 12 K. While the origin of this puzzling observation remains to be exploited, we discuss the possibility of a long-sought pairing state of electrons with a four-fold degeneracy., Comment: 13 pages, 4 figures

Resistively detected nuclear magnetic resonance (NMR) is observed inside the ring-like structure, with a quantized Hall conductance of 6e^2/h, in the phase diagram of a two subband electron system. The NMR signal persists up to 400 mK and is absent in other states with the same quantized Hall conductance. The nuclear spin-lattice relaxation time, T1, is found to decrease rapidly towards the ring center. These observations are consistent with the assertion of the ring-like region being a ferromagnetic state that is accompanied by collective spin excitations., Comment: 4 pages, 4 figures

In a two-subband GaAs/AlGaAs two-dimensional electron system, the phase diagram of longitudinal resistivity \rho_xx in density and magnetic field plane exhibits an intriguing structure centered at filling factor \nu = 4 which is strikingly different from the ring-like structures at lower magnetic fields. Thermal activation measurements reveal an anticrossing gap on each boundary of the structure where intersubband Landau Levels with parallel or antiparallel spin are brought into degeneracy. While the physics of the anticrossing can be ascribed to the pseudospin quantum Hall ferromagnetism, as reported earlier by Muraki et al, the mapping and modeling of the phase diagram topology allow us to establish a more complete picture of the consequences of real spin / pseudo-spin interactions for the two subband system., Comment: Accepted by Physical Review B

In a GaAs/AlGaAs two-dimensional electron system with two occupied subbands, the experimentally determined phase diagram in the density-magnetic field plane exhibits rich topological features. Ring-like structures are observed at even integer filling factors, in the phase diagram. Even with the identical quantized Hall resistance values as those given rise by the ordinary integer quantum Hall effect due to the Landau level quantization; the activation energies of these states within the rings are much smaller. These ring structures cannot account for by the simple single particle picture. We argue that ferromagnetic quantum Hall states, due to the interaction of two energy levels with opposite spin and different subband indices, are responsible for these unusual structures., Comment: Physical Review letter in press