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Quantum collision model provides a promising tool for investigating system-bath dynamics. Most of the studies on quantum collision models work in the resonant regime. In quantum dynamics, the off-resonant interaction often brings in exciting ffects. It is thereby attractive to investigate quantum collision models in the off-resonant regime. On the other hand, a bath with a negative absolute temperature is anticipated to be instrumental in developing thermal devices. The design of an effective bath with negative absolute temperature coupled to a qubit is significant for developing such thermal devices. We establish an effective negative-absolute-temperature bath coupled to a qubit with a quantum collision model in a far-off-resonant regime. We conduct a detailed and systematic investigation on the off-resonant collision model. There is an additional constraint on the collision duration resulting from the far-off resonant collision. The dynamics of the collision model in the far-off-resonant regime are different from the one beyond the far-off-resonant regime. Numerical simulations confirm the validity of the proposed approach., Comment: 7 pages, 3 figures

The recently discovered spin-triplet superconductor candidate UTe2 with Tc = 2 K has attracted enormous attention because it possesses many interesting properties, such as the extremely high upper critical field Hc2(0), chiral superconductivity and spontaneous time-reversal symmetry breaking, etc., all these suggest that it may be the long-sought spin-triplet superconductor. Here we report the discovery of superconductivity up to Tc = 4K in one of its siblings, i.e., UAs2 under high pressures. Interestingly, the UAs2 shows metallic behavior with an antiferromagnetic (AFM) transition at about 274 K under ambient pressure. Upon applying pressure, this transition is pushed down to lower temperatures with improved electric conductivity. When the pressure rises to about 20-22 GPa, superconductivity occurs together with the emergence of a linear temperature dependence of normal state resistance, the latter is a hallmark of the strange-metal state. The superconductivity with the highest Tc = 4 K is reached under a pressure of about 26.8 GPa, and it is robust against magnetic field with the upper critical field {\mu}0Hc2(0) ~ 12 T, far beyond the Pauli limit. Higher pressures will suppress the superconductivity and bring back the Fermi liquid behavior, showing a clear signature of quantum criticality. Our results open a new avenue for investigating the unconventional superconductivity concerning the mysterious 5f-band electrons in this uranium-based system., Comment: 16 pages of main text, 4 figures + 7 extended data figures

The discovery of superconductivity in 3$d$-transition metal compounds with strong magnetism is interesting but rare. Especially for Mn-based compounds, there exist only very limited materials that show superconductivity. Here, we report the discovery of superconductivity up to 14.2 K in a Mn-based material MnB$_4$. By applying high pressures, we found the continuous suppression of a weak insulating behavior and the occurrence of superconductivity after about 30 GPa. With further increasing pressure, $T_\text{c}$ is gradually enhanced and reaches the maximum value of about 14.2 K at 150 GPa with a Fermi-Liquid behavior in the normal states. The synchrotron X-ray diffraction data reveal the unchanged monoclinic (S.G: $P2_1/c$) symmetry but an unusual crossover of the lattice parameters $b$ and $c$. Theoretical calculations based on the electron-phonon coupling picture reveal a very low $T_\text{c}$ (less than 1 K), manifesting an exotic pairing mechanism beyond the Bardeen-Cooper-Schrieffer (BCS) theory. Our findings show a promising way to explore high $T_\text{c}$ superconductivity by combining the 3d-transition metal magnetic elements and light elements., Comment: 36 pages total; 24 pages of main text with 5 figures, 12 pages of supplement with 1 table and 8 figures

An accurate map of intracellular organelle pH is crucial for comprehending cellular metabolism and organellar functions. However, a unified intracellular pH spectrum using a single probe is still lack. Here, we developed a novel quantum entanglement-enhanced pH-sensitive probe called SITE-pHorin, which featured a wide pH-sensitive range and ratiometric quantitative measurement capabilities. Subsequently, we measured the pH of various organelles and their sub-compartments, including mitochondrial sub-spaces, Golgi stacks, endoplasmic reticulum, lysosomes, peroxisomes, and endosomes in COS-7 cells. For the long-standing debate on mitochondrial compartments pH, we measured the pH of mitochondrial cristae as 6.60 \pm 0.40, the pH of mitochondrial intermembrane space as 6.95 \pm 0.30, and two populations of mitochondrial matrix pH at approximately 7.20 \pm 0.27 and 7.50 \pm 0.16, respectively. Notably, the lysosome pH exhibited a single, narrow Gaussian distribution centered at 4.79 \pm 0.17. Furthermore, quantum chemistry computations revealed that both the deprotonation of the residue Y182 and the discrete curvature of deformed benzene ring in chromophore are both necessary for the quantum entanglement mechanism of SITE-pHorin. Intriguingly, our findings reveal an accurate pH gradient (0.6-0.9 pH unit) between mitochondrial cristae and matrix, suggesting prior knowledge about \Delta pH (0.4-0.6) and mitochondrial proton motive force (pmf) are underestimated., Comment: 64 pages, 7 figures, the supplemental material contains 13 supplemental figures and 4 supplemental tables

Feature extraction is a critical technology to realize the automatic transmission of feature information throughout product life cycles. As CAD models primarily capture the 3D geometry of products, feature extraction heavily relies on geometric information. However, existing feature extraction methods often yield inaccurate outcomes due to the diverse interpretations of geometric information. This report presents a set-based feature extraction approach to address this uncertainty issue. Unlike existing methods that seek accurate feature results, our approach aims to transform the uncertainty of geometric information into a set of feature subgraphs. First, we define the convexity of basic geometric entities and introduce the concept of two-level attributed adjacency graphs. Second, a feature extraction workflow is designed to determine feature boundaries and identify feature subgraphs from CAD models. This set of feature subgraphs can be used for further feature recognition. A feature extraction system is programmed using C++ and UG/Open to demonstrate the feasibility of our proposed approach., Comment: 13 pages

Advanced Persistent Threat (APT) attacks have caused significant damage worldwide. Various Endpoint Detection and Response (EDR) systems are deployed by enterprises to fight against potential threats. However, EDR suffers from high false positives. In order not to affect normal operations, analysts need to investigate and filter detection results before taking countermeasures, in which heavy manual labor and alarm fatigue cause analysts miss optimal response time, thereby leading to information leakage and destruction. Therefore, we propose Endpoint Forecasting and Interpreting (EFI), a real-time attack forecast and interpretation system, which can automatically predict next move during post-exploitation and explain it in technique-level, then dispatch strategies to EDR for advance reinforcement. First, we use Cyber Threat Intelligence (CTI) reports to extract the attack scene graph (ASG) that can be mapped to low-level system logs to strengthen attack samples. Second, we build a serialized graph forecast model, which is combined with the attack provenance graph (APG) provided by EDR to generate an attack forecast graph (AFG) to predict the next move. Finally, we utilize the attack template graph (ATG) and graph alignment plus algorithm for technique-level interpretation to automatically dispatch strategies for EDR to reinforce system in advance. EFI can avoid the impact of existing EDR false positives, and can reduce the attack surface of system without affecting the normal operations. We collect a total of 3,484 CTI reports, generate 1,429 ASGs, label 8,000 sentences, tag 10,451 entities, and construct 256 ATGs. Experimental results on both DARPA Engagement and large scale CTI dataset show that the alignment score between the AFG predicted by EFI and the real attack graph is able to exceed 0.8, the forecast and interpretation precision of EFI can reach 91.8%.

As the complexity and destructiveness of Advanced Persistent Threat (APT) increase, there is a growing tendency to identify a series of actions undertaken to achieve the attacker's target, called attack investigation. Currently, analysts construct the provenance graph to perform causality analysis on Point-Of-Interest (POI) event for capturing critical events (related to the attack). However, due to the vast size of the provenance graph and the rarity of critical events, existing attack investigation methods suffer from problems of high false positives, high overhead, and high latency. To this end, we propose SPARSE, an efficient and real-time system for constructing critical component graphs (i.e., consisting of critical events) from streaming logs. Our key observation is 1) Critical events exist in a suspicious semantic graph (SSG) composed of interaction flows between suspicious entities, and 2) Information flows that accomplish attacker's goal exist in the form of paths. Therefore, SPARSE uses a two-stage framework to implement attack investigation (i.e., constructing the SSG and performing path-level contextual analysis). First, SPARSE operates in a state-based mode where events are consumed as streams, allowing easy access to the SSG related to the POI event through semantic transfer rule and storage strategy. Then, SPARSE identifies all suspicious flow paths (SFPs) related to the POI event from the SSG, quantifies the influence of each path to filter irrelevant events. Our evaluation on a real large-scale attack dataset shows that SPARSE can generate a critical component graph (~ 113 edges) in 1.6 seconds, which is 2014 X smaller than the backtracking graph (~ 227,589 edges). SPARSE is 25 X more effective than other state-of-the-art techniques in filtering irrelevant edges.

It is well-known that magnetic moments are very harmful to superconductivity. A typical example is the element Mn whose compounds usually exhibit strong magnetism. Thus, it is very hard to achieve superconductivity in materials containing Mn. Here, we report enhanced superconductivity with the superconducting transition temperature ($T_\text{c}$) up to a record high-value of about 26 K in a beta-phase Ti$_{1-x}$Mn$_x$ alloy containing rich magnetic element Mn under high pressures. This is contrary to the intuition that the magnetic moments always suppress superconductivity. Under high pressures, we also found that in the middle-pressure regime, the Pauli limit of the upper critical field is surpassed. The synchrotron X-ray diffraction data shows an unchanged beta-phase with a continuous contraction of the cell volume, which is well supported by the first-principles calculations. Although the theoretical results based on electron-phonon coupling (EPC) can interpret the $T_\text{c}$ value in a certain pressure region, the monotonic enhancement of superconductivity by pressure cannot seek support from the theory. Our results show a surprising enhancement of superconductivity in Ti$_{1-x}$Mn$_x$ alloy with a considerable Mn content., Comment: 28 pages, 5 figures. Comments are welcome and appreciated

Entropy production is a fundamental concept that plays a crucial role in the second law of thermodynamics and the measure of irreversibility. It imposes rigorous constraints on the kinds of transformations allowed in thermodynamic processes. Using an optical setup, here we experimentally demonstrate the division of entropy production of an open quantum system into a population-related component and a coherence-related component, validating previous theoretical predictions. The coherence-related component represents a genuine quantum contribution with no classical counterpart. By adjusting bath temperatures and initial coherences of the system, we first derive the total entropy production due to both populations and coherences, then remove all the coherences of the system to solely obtain the population-related contribution. The difference between these two results permits to isolate the coherence-related term. Based on this division, our experiment ultimately proves that irreversibility at the quantum level can be reduced through properly harnessing the two contributions to entropy production., Comment: 7 pages, 3 figures

The deposition and intercalation of metal atoms can induce superconductivity in monolayer and bilayer graphenes. For example, it has been experimentally proved that Li-deposited graphene is a superconductor with critical temperature $T_{c}$ of 5.9 K, Ca-intercalated bilayer graphene C$_{6}$CaC$_{6}$ and K-intercalated epitaxial bilayer graphene C$_{8}$KC$_{8}$ are superconductors with $T_{c}$ of 2-4 K and 3.6 K, respectively. However, the $T_{c}$ of them are relatively low. To obtain higher $T_{c}$ in graphene-based superconductors, here we predict a new Ca-intercalated bilayer graphene C$_{2}$CaC$_{2}$, which shows higher Ca concentration than the C$_{6}$CaC$_{6}$. It is proved to be thermodynamically and dynamically stable. The electronic structure, electron-phonon coupling (EPC) and superconductivity of C$_{2}$CaC$_{2}$ are investigated based on first-principles calculations. The EPC of C$_{2}$CaC$_{2}$ mainly comes from the coupling between the electrons of C-$p_{z}$ orbital and the high- and low-frequency vibration modes of C atoms. The calculated EPC constant $\lambda$ of C$_{2}$CaC$_{2}$ is 0.75, and the superconducting $T_{c}$ is 18.9 K, which is much higher than other metal-intercalated bilayer graphenes. By further applying -4\% biaxial compressive strain to C$_{2}$CaC$_{2}$, the $T_{c}$ can be boosted to 26.6 K. Thus, the predicted C$_{2}$CaC$_{2}$ provides a new platform for realizing superconductivity with the highest $T_{c}$ in bilayer graphenes., Comment: 29 pages,11 figures

Portfolio management (PM) is a fundamental financial trading task, which explores the optimal periodical reallocation of capitals into different stocks to pursue long-term profits. Reinforcement learning (RL) has recently shown its potential to train profitable agents for PM through interacting with financial markets. However, existing work mostly focuses on fixed stock pools, which is inconsistent with investors' practical demand. Specifically, the target stock pool of different investors varies dramatically due to their discrepancy on market states and individual investors may temporally adjust stocks they desire to trade (e.g., adding one popular stocks), which lead to customizable stock pools (CSPs). Existing RL methods require to retrain RL agents even with a tiny change of the stock pool, which leads to high computational cost and unstable performance. To tackle this challenge, we propose EarnMore, a rEinforcement leARNing framework with Maskable stOck REpresentation to handle PM with CSPs through one-shot training in a global stock pool (GSP). Specifically, we first introduce a mechanism to mask out the representation of the stocks outside the target pool. Second, we learn meaningful stock representations through a self-supervised masking and reconstruction process. Third, a re-weighting mechanism is designed to make the portfolio concentrate on favorable stocks and neglect the stocks outside the target pool. Through extensive experiments on 8 subset stock pools of the US stock market, we demonstrate that EarnMore significantly outperforms 14 state-of-the-art baselines in terms of 6 popular financial metrics with over 40% improvement on profit.

The discovery of high-temperature superconductivity near 80 K in bilayer nickelate La$_3$Ni$_2$O$_7$ under high pressures has renewed the exploration of superconducting nickelate in bulk materials. The extension of superconductivity in other nickelates in a broader family is also essential. Here, we report the experimental observation of superconducting signature in trilayer nickelate La$_4$Ni$_3$O$_{10}$ under high pressures. By using a modified sol-gel method and post-annealing treatment under high oxygen pressure, we successfully obtained polycrystalline La$_4$Ni$_3$O$_{10}$ samples with different transport behaviors at ambient pressure. Then we performed high-pressure electrical resistance measurements on these samples in a diamond-anvil-cell (DAC) apparatus. Surprisingly, the signature of possible superconducting transition with a maximum transition temperature ($T_\text{c}$) of about 20 K under high pressures is observed, as evidenced by a clear drop of resistance and the suppression of resistance drops under magnetic fields. Although the resistance drop is sample-dependent and relatively small, it appears in all of our measured samples. We argue that the observed superconducting signal is most likely to originate from the main phase of La$_4$Ni$_3$O$_{10}$. Our findings will motivate the exploration of superconductivity in a broader family of nickelates and shed light on the understanding of the underlying mechanisms of high-$T_\text{c}$ superconductivity in nickelates., Comment: 17 pages, 5 figures

We propose a scheme to realize the single-photon transport affected by the temperature. The scheme is composed by a waveguide-atom interacting structure linked to a thermal bath. The single-photon reflection coefficient can be tuned by adjusting the temperature of the thermal bath. This provides a thermal control of the single-photon transport. Moreover, the temperature of the thermal bath can be estimated by measuring the single-photon transport. It is feasible that the estimation on the temperature is sensitive to slight changes of low temperature. This implies an avenue for implementing the optical thermometer with the ability to accurately measure the sample temperature in the low-temperature region., Comment: 7 pages, 4 figures

By applying pressures up to 42 GPa on the nitrogen-doped lutetium hydride (LuH$_{2\pm\text{x}}$N$_y$), we have found a gradual change of color from dark-blue to pink-violet in the pressure region of about 12 GPa to 21 GPa. The temperature dependence of resistivity under pressures up to 50.5 GPa shows progressively optimized metallic behavior with pressure. Interestingly, in the pressure region for the color change, a clear decrease of resistivity is observed with the increase of pressure, which is accompanied by a clear increase of the residual resistivity ratio (RRR). Fitting to the low temperature resistivity gives exponents of about 2, suggesting a Fermi liquid behavior in low temperature region. The general behavior in wide temperature region suggests that the electron-phonon scattering is still the dominant one. The magnetoresistance up to 9 tesla in the state under a pressure of 50.5 GPa shows an almost negligible effect, which suggests that the electric conduction in the pink-violet state is dominated by a single band. It is highly desired to have theoretical efforts in understanding the evolution of color and resistivity in this interesting system., Comment: 15 pages, 4 figures

Recently near-ambient superconductivity was claimed in N-doped lutetium hydride (ref. 1). This induces a worldwide fanaticism about the dream of room temperature superconductivity under low pressures. By using a high pressure and high temperature synthesis technique, we have successfully obtained the nitrogen doped lutetium hydride (LuH$_{2\pm\text{x}}$N$_y$) with a dark-bluish color and a structure with the space group of $Fm\bar{3}m$ evidenced by x-ray diffraction. This structure is the same as that reported in ref. 1. The energy dispersive X-ray spectroscopy (EDS) confirmed the existence of nitrogen in some areas of the samples. At ambient pressure, we witness a kink of resistivity and magnetization at about 300 K, which may correspond to a rearrangement of hydrogen/nitrogen atoms, namely a structural transition. However, by applying a pressure from 1 GPa to 6 GPa, we have seen a progressively optimized metallic behavior without showing superconductivity down to 10 K. Temperature dependence of magnetization shows a roughly flat feature between 100 and 320 K, and the magnetization increases with magnetic field at 100 K, all these are not expected for superconductivity at 100 K. Thus, we conclude the absence of near-ambient superconductivity in this nitrogen-doped lutetium hydride under pressures below 6 GPa., Comment: An updated version with more data was published in Nature online on 11th May 2023 as an Accelerated Article Preview form