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Chiral light-matter interactions supported by topological edge modes at the interface of valley photonic crystals provide a robust method to implement the unidirectional spin transfer. The valley topological photonic crystals possess a pair of counterpropagating edge modes. The edge modes are robust against the sharp bend of $60^{\circ}$ and $120^{\circ}$, which can form a resonator with whispering gallery modes. Here, we demonstrate the asymmetric emission of chiral coupling from single quantum dots in a topological resonator by tuning the coupling between a quantum emitter and a resonator mode. Under a magnetic field in Faraday configuration, the exciton state from a single quantum dot splits into two exciton spin states with opposite circularly polarized emissions due to Zeeman effect. Two branches of the quantum dot emissions couple to a resonator mode in different degrees, resulting in an asymmetric chiral emission. Without the demanding of site-control of quantum emitters for chiral quantum optics, an extra degree of freedom to tune the chiral contrast with a topological resonator could be useful for the development of on-chip integrated photonic circuits., Comment: 13 pages, 4 figures

We report the slow-light enhanced spin-resolved in-plane emission from a single quantum dot (QD) in a photonic crystal waveguide (PCW). The slow light dispersions in PCWs are designed to match the emission wavelengths of single QDs. The resonance between two spin states emitted from a single QD and a slow light mode of a waveguide is investigated under a magnetic field with Faraday configuration. Two spin states of a single QD experience different degrees of enhancement as their emission wavelengths are shifted by combining diamagnetic and Zeeman effects with an optical excitation power control. A circular polarization degree up to 0.81 is achieved by changing the off-resonant excitation power. Strongly polarized photon emission enhanced by a slow light mode shows great potential to attain controllable spin-resolved photon sources for integrated optical quantum networks on chip., Comment: 7 pages,5 figures

Single charge control of localized excitons (LXs) in two-dimensional transition metal dichalcogenides (TMDCs) is crucial for potential applications in quantum information processing and storage. However, traditional electrostatic doping method with applying metallic gates onto TMDCs may cause the inhomogeneous charge distribution, optical quench, and energy loss. Here, by locally controlling the ferroelectric polarization of the ferroelectric thin film BiFeO3 (BFO) with a scanning probe, we can deterministically manipulate the doping type of monolayer WSe2 to achieve the p-type and n-type doping. This nonvolatile approach can maintain the doping type and hold the localized excitonic charges for a long time without applied voltage. Our work demonstrated that ferroelectric polarization of BFO can control the charges of LXs effectively. Neutral and charged LXs have been observed in different ferroelectric polarization regions, confirmed by magnetic optical measurement. Highly circular polarization degree about 90 % of the photon emission from these quantum emitters have been achieved in high magnetic fields. Controlling single charge of LXs in a non-volatile way shows a great potential for deterministic photon emission with desired charge states for photonic long-term memory., Comment: 13 pages, 5 figures

Strong exciton-plasmon interaction between the layered two-dimensional (2D) semiconductors and gap plasmons shows a great potential to implement cavity quantum-electrodynamics in ambient condition. However, achieving a robust plasmon-exciton coupling with nanocavity is still very challenging, because the layer area is usually small with conventional approaches. Here, we report on a robust strong exciton-plasmon coupling between the gap mode of bowtie and the excitons in MoS$_2$ layers with gold-assisted mechanical exfoliation and the nondestructive wet transfer techniques for large-area layer. Benefiting from the ultrasmall mode volume and strong in-plane field, the estimated effective exciton number contributing to the coupling is largely reduced. With a corrected exciton transition dipole moment, the exciton numbers are extracted with 40 for the case of monolayer and 48 for 8 layers. Our work paves a way to realize the strong coupling with 2D materials with few excitons at room temperature., Comment: 21 pages, 5 figures

Slow light in topological valley photonic crystal structures offers new possibilities to enhance light-matter interaction. We report a topological cavity based on slow light topological edge mode for broadband Purcell enhancement. The topological edge modes with large group indices over 100 can be realized with a bearded interface between two topologically distinct valley photonic crystals, featuring the greatly enhanced Purcell factor because of the increased local density of states. In the slow light regime, the topological cavity supports much more cavity modes with higher quality factor than that in the fast light regime, which is both demonstrated theoretically and experimentally. We demonstrate the cavity enables the broadband Purcell enhancement together with substantial Purcell factor, benefiting from dense cavity modes with high quality factor in a wide spectral range. It has great benefit to the realization of high-efficiency quantum-dot-based single-photon sources and entangled-photon sources with less restriction on spectral match. Such topological cavity could serve as a significant building block toward the development of photonic integrated circuits with embedded quantum emitters., Comment: 16 pages, 4 figures

Chiral quantum optics has attracted considerable interest in the field of quantum information science. Exploiting the spin-polarization properties of quantum emitters and engineering rational photonic nanostructures has made it possible to transform information from spin to path encoding. Here, compact chiral photonic circuits with deterministic circularly polarized chiral routing and beamsplitting are demonstrated using two laterally adjacent waveguides coupled with quantum dots. Chiral routing arises from the electromagnetic field chirality in waveguide, and beamsplitting is obtained via the evanescent field coupling. The spin- and position-dependent directional spontaneous emission are achieved by spatially selective micro-photoluminescence measurements, with a chiral contrast of up to 0.84 in the chiral photonic circuits. This makes a significant advancement for broadening the application scenarios of chiral quantum optics and developing scalable quantum photonic networks., Comment: 19 pages, 5 figures

We report on controllable cavity modes through controlling the backscattering by two identical scatterers. Periodic changes of the backscattering coupling between two degenerate cavity modes are observed with the angle between two scatterers and elucidated by a theoretical model using two-mode approximation and numerical simulations. The periodically appearing single-peak cavity modes indicate mode degeneracy at diabolical points. Then interactions between single quantum dots and cavity modes are investigated. Enhanced emission of a quantum dot with a six-fold intensity increase is obtained in a microdisk at a diabolical point. This method to control cavity modes allows large-scale integration, high reproducibility and fexible design of the size, location, quantity and shape for scatterers, which can be applied for integrated photonic structures with scatterer-modified light-matter interaction., Comment: 23 pages, 5 figures

Chiral light-matter interaction between photonic nanostructures with quantum emitters shows great potential to implement spin-photon interfaces for quantum information processing. Position-dependent spin momentum locking of the quantum emitter is important for these chiral coupled nanostructures. Here, we report the position-dependent chiral coupling between quantum dots (QDs) and cross waveguides both numerically and experimentally. Four quantum dots distributed at different positions in the cross section are selected to characterize the chiral properties of the device. Directional emission is achieved in a single waveguide as well as in both two waveguides simultaneously. In addition, the QD position can be determined with the chiral contrasts from four outputs. Therefore, the cross waveguide can function as a one-way unidirectional waveguide and a circularly polarized beam splitter by placing the QD in a rational position, which has potential applications in spin-to-path encoding for complex quantum optical networks at the single-photon level., Comment: 13 pages, 4 figures

We report an out-of-plane magnetic field induced large photoluminescence enhancement in WS${}_2$ flakes at $4$ K, in contrast to the photoluminescence enhancement provided by in-plane field in general. Two mechanisms for the enhancement are proposed. One is a larger overlap of electron and hole caused by the magnetic field induced confinement. The other is that the energy difference between $\Lambda$ and K valleys is reduced by magnetic field, and thus enhancing the corresponding indirect-transition trions. Meanwhile, the Land\'e g factor of the trion is measured as $-0.8$, whose absolute value is much smaller than normal exciton, which is around $|-4|$. A model for the trion g factor is presented, confirming that the smaller absolute value of Land\'e g factor is a behavior of this $\Lambda$-K trion. By extending the valley space, we believe this work provides a further understanding of the valleytronics in monolayer transition metal dichalcogenides., Comment: 15 pages, 4 figures

We report a high-resolution photocurrent (PC) spectroscopy of a single self-assembled InAs/GaAs quantum dot (QD) embedded in an n-i-Schottky device with an applied vector magnetic field. The PC spectra of positively charged exciton (X$^+$) and neutral exciton (X$^0$) are obtained by two-color resonant excitation. With an applied magnetic field in Voigt geometry, the double $\Lambda$ energy level structure of X$^+$ and the dark states of X$^0$ are observed in PC spectra clearly. In Faraday geometry, the PC amplitude of X$^+$ decreases and then quenches with the increasing of the magnetic field, which provides a new way to determine the relative sign of the electron and the hole g-factors. With an applied vector magnetic field, the electron and the hole g-factor tensors of X$^+$ and X$^0$ are obtained. The anisotropy of the hole g-factors of both X$^+$ and X$^0$ is larger than that of the electron., Comment: 21 pages, 5 figures

Topological photonics provides a new paradigm in studying cavity quantum electrodynamics with robustness to disorder. In this work, we demonstrate the coupling between single quantum dots and the second-order topological corner state. Based on the second-order topological corner state, a topological photonic crystal cavity is designed and fabricated into GaAs slabs with quantum dots embedded. The coexistence of corner state and edge state with high quality factor close to 2000 is observed. The enhancement of photoluminescence intensity and emission rate are both observed when the quantum dot is on resonance with the corner state. This result enables the application of topology into cavity quantum electrodynamics, offering an approach to topological devices for quantum information processing., Comment: 17 pages, 3 figures

Monolayer transition metal dichalcogenides have recently attracted great interests because the quantum dots embedded in monolayer can serve as optically active single photon emitters. Here, we provide an interpretation of the recombination mechanisms of these quantum emitters through polarization-resolved and magneto-optical spectroscopy at low temperature. Three types of defect-related quantum emitters in monolayer tungsten diselenide (WSe$_2$) are observed, with different exciton g factors of 2.02, 9.36 and unobservable Zeeman shift, respectively. The various magnetic response of the spatially localized excitons strongly indicate that the radiative recombination stems from the different transitions between defect-induced energy levels, valance and conduction bands. Furthermore, the different g factors and zero-field splittings of the three types of emitters strongly show that quantum dots embedded in monolayer have various types of confining potentials for localized excitons, resulting in electron-hole exchange interaction with a range of values in the presence of anisotropy. Our work further sheds light on the recombination mechanisms of defect-related quantum emitters and paves a way toward understanding the role of defects in single photon emitters in atomically thin semiconductors., Comment: 14 pages, 4 Figures

Hybrid Perovskites have shown a great potential for applications in photovoltaics and light-emitting devices with high efficiency. Interaction between defect-induced trapped excitons and phonons plays an important role in understanding the emerging phenomena for such an excellent figure-of-merit. Here we demonstrate hot polarons with narrow linewidth in $\mathrm{CH_{3}NH_{3}PbBr_{3}}$ nanowires, which originate from the interaction between trapped excitons and octahedra-twist phonons. The observation of hot polarons in photoluminescence without gain methods indicates the large interaction strength between excitons and phonons. The multiple hot polarons are further confirmed by magneto-optical spectra with a Zeeman splitting of the trapped excitons and a phonon energy increase with diamagnetic effect. Furthermore, the phonons participating in the interaction are demonstrated to be the octahedra-twist vibrations which are transverse optical phonons, while the interaction between trapped excitons and longitudinal optical phonons is weak. Our work demonstrates that trapped excitons in perovskites prefer to interact with transverse rather than longitudinal optical phonons. Since bulk materials usually interact with longitudinal optical phonons, this result provides a physical explanation of the high tolerance of defects in perovskites., Comment: 16 pages, 4 figures

Transition metal dichalcogenide monolayers provide an emerging material system to implement quantum photonics with intrinsic two-dimensional excitons or embedded zero-dimensional localized states. Here we demonstrate the mesoscopic localized states between two- and zero- dimensions, which is a many-body system with electron-electron Coulomb interactions. A fine structure splitting is observed, which is similar to quantum dots. Meanwhile the polarization is changed by the magnetic field, due to the nature of two-dimensional monolayers. Furthermore, a large quadratic diamagnetism with a coefficient of around $100\ \mathrm{\mu eV/T^2}$ is observed, as a unique consequence of the mesoscopic scale. The many-body effect also results in the emission energy variation and linewidth narrowing in the spectrum, which corresponds well to the theoretical analysis. These unique properties indicate the great potential of mesoscopic localized states in many-body physics and quantum photonics., Comment: 14 pages, 4 figures