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Multidimensional coherent spectroscopy (MDCS) is a highly intriguing field for the unique capacities to unravel quantum pathways of microscopic dynamics and discern different dipole–dipole interactions. These capabilities are not simultaneously accessible through any other techniques. The foundation of MDCS lies in the stable phase and accurate time information of the multi‐pulse sequences involved. Achieving the phase stability has traditionally relied on ingenious geometric optical designs and multiple feedback control systems, albeit at the cost of complexity. In this letter, a phase stability scheme for high‐resolution MDCS is proposed by replacing traditional laser sources with two highly coherent frequency combs. By employing dual‐comb interferometry, the phase distribution across a broad spectral range and the time information of all the excitation pulses are precisely measured, even in setups that lack phase stability. In the experiment, a rephasing MDCS of rubidium atoms is obtained by applying this approach, wherein the comb resolution is utilized to differentiate the couplings of hyperfine energy levels. This scheme simplifies the structure of MDCS and holds potential for applications in other MDCS systems involving many‐body interactions and non‐absorptive resonances. [ABSTRACT FROM AUTHOR]

The impact of geomagnetic storms on the mesosphere temperature has been controversial and lacks direct observational evidence. The intricate chemical and physical processes in the mesosphere, combined with the scarcity of observations, pose challenges to achieving a thorough comprehension of storm‐induced turbulences in this region. Currently, some investigations have characterized temperature responses during geomagnetic storms and the focus has largely been on changes above mesopause (∼90 km). In this work, the responses of temperature in the mesosphere (75–95 km) to the storms on September 8 and 15, 2003 and its causes are studied using observations from the Sounding of the Atmosphere using Broadband Emission Radiometry (SABER) instrument onboard the Thermosphere Ionosphere Mesosphere Energetics and Dynamics (TIMED) satellite. It is found that (a) temperature responses for the moderate storm on September 15 manifest as increases within the latitude range of 80°S to 65°S, with peak values decreasing from approximately 15 K to around 7 K as latitude decreases, while for the minor strom of September 8 temperature changes only occur at ∼80°S with peaks of 7 K and −10 K, (b) the temperature responses can be transmitted down to 76–81 km, depending on the latitude and storm magnitude, and (c) there are significant fluctuations in both ozone (exceed 45%) and atomic oxygen (exceed 90%) after storm onset, highly correlated with temperature temporal and spatial variations. We suggest that the increases in ozone caused by the increases in atomic oxygen concentrations are the major contributor to rising temperature. Plain Language Summary: Geomagnetic storms may have a non‐negligible effect on the atmospheric circulation, neutral temperature, winds, and composition of the mesosphere and lower thermosphere. However, there is a lack of understanding of the perturbations and its chemical and physical processes in the mesosphere during geomagnetic storms. In this paper, we analyze temperature, ozone, and atomic oxygen observations acquired from the SABER instrument aboard the TIMED satellite. Our work demonstrate that variations in mesosphere temperature occur at high latitudes and are correlated with the magnitude of the storm. Additionally, significant disturbances in ozone and atomic oxygen are observed from 80°S to 65°S latitude. We propose that the variations in mesosphere temperature at high latitudes are dominated to changes in ozone caused by the heightened concentrations of atomic oxygen. Key Points: Temperatures of the mesosphere observed by SABER have remarkable responses to the geomagnetic storms of 8 and 15 September 2003The mesosphere temperature variations occur at high latitudes and can be conveyed to 76–81 km, depending on the latitude and storm magnitudeOzone variations are responsible for the mesosphere temperature variations at high latitudes during storms [ABSTRACT FROM AUTHOR]

High-resolution optical multidimensional coherent spectroscopy (MDCS) requires frequency-stable laser sources and high-resolution heterodyne spectra. Fully phase-locked dual-comb spectroscopy (DCS) enables the achievement of high resolution, high accuracy, broad bandwidth, and a rapid multi-heterodyne spectrum, which results in the DCS's potential to replace the spectrometer and phase detection system in MDCS. We verified the phase measurement capability of the MDCS system based on fully phase-locked fiber DCS by studying phase-sensitive photon echoes and double-quantum processes. The accurate phase and frequency of linear and nonlinear signals were obtained simultaneously using a single detector without subsequent frequency drift correction. Subsequently, the acquisition of longtime quantum beat signals demonstrates the high phase coherence between excitation pulses. Additionally, the two-dimensional coherent spectrum (2DCS) with high signal-to-noise-ratio and 100 MHz resolution was obtained via the MDCS system based on fully phase-locked fiber DCS. These results exhibit that fully phase-locked fiber DCS is an effective method for high-resolution 2DCS measurement, which facilitates further research on cold atoms, higher-order nonlinear spectra, and molecular fingerprint vibrational spectroscopy. [ABSTRACT FROM AUTHOR]

Microwave Limb Sounder (MLS) observations showed an obvious variation of ozone concentration during the annular solar eclipse on 21 June 2020 in the mesosphere and upper stratosphere. Ozone concentration slightly reduced near 40 km in the regions of 24°N–36°N, and increased in low latitudes at 40 km. In the heights of 45–60 km, the increase in ozone concentration in most of the regions was obvious. The ozone increases and decreases were more obvious between 60–65 km, where enhancement took the leading role. The nighttime ozone variation was weaker than the daytime in most of the heights of 30–65 km. The variation of HO2 and CO is investigated to study the photochemical and dynamical causes of ozone variation. As HO2 decreased at 1 hPa and increased at 60–65 km, ozone variation shows a mostly reversed relationship to HO2 variation. CO increased at 32–39 km and decreased at 52–60 km, which was related to the upwelling at these heights. The dynamic processes also contributed to the decrease in ozone concentration at 40 km and increase at 50–60 km. [ABSTRACT FROM AUTHOR]

We demonstrate three typical mode-locking processes of a nonlinear amplifying loop mirror (NALM) fiber laser via a general nonlinear Schrödinger equation-based (GNLSE) simulation model. First, the pulse evolutions in the NALM cavity were separately simulated under asymmetric and weakly asymmetric conditions. We found that the splitting ratio and positions of the gain fiber can result in a suitable phase bias between clockwise and counter-clockwise beams, enabling the realization of a self-starting low-threshold operating condition. To assess the roles of the splitting ratio and gain in the mode-locking process, we simulated three pulse formation processes: in the soliton, stretched-pulse, and dissipative soliton mode-locking regimes. The simulation results show that the splitting ratio, gain, and dispersion directly influence the mode-locking condition and pulse characteristics, thereby providing effective quantified guidance for high-quality pulse generation. Finally, an experimental NALM oscillation operating under stretched pulse conditions was established to investigate the impact of the splitting ratio and pump power on the pulse characteristics. The experimental results prove that the splitting ratio, gain, and dispersion can be used to manipulate the mode-locking threshold, self-starting threshold, nonlinear effects, and pulse characteristics.