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Evidence has emerged for a stochastic signal correlated among 67 pulsars within the 15-year pulsar-timing data set compiled by the NANOGrav collaboration. Similar signals have been found in data from the European, Indian, Parkes, and Chinese PTAs. This signal has been interpreted as indicative of the presence of a nanohertz stochastic gravitational wave background. To explore the internal consistency of this result we investigate how the recovered signal strength changes as we remove the pulsars one by one from the data set. We calculate the signal strength using the (noise-marginalized) optimal statistic, a frequentist metric designed to measure correlated excess power in the residuals of the arrival times of the radio pulses. We identify several features emerging from this analysis that were initially unexpected. The significance of these features, however, can only be assessed by comparing the real data to synthetic data sets. After conducting identical analyses on simulated data sets, we do not find anything inconsistent with the presence of a stochastic gravitational wave background in the NANOGrav 15-year data. The methodologies developed here can offer additional tools for application to future, more sensitive data sets. While this analysis provides an internal consistency check of the NANOGrav results, it does not eliminate the necessity for additional investigations that could identify potential systematics or uncover unmodeled physical phenomena in the data., Comment: 21 pages, 11 figures, 2 tables

Addressing data integrity challenges, such as unlearning the effects of data poisoning after model training, is necessary for the reliable deployment of machine learning models. State-of-the-art influence functions, such as EK-FAC, often fail to accurately attribute abnormal model behavior to the specific poisoned training data responsible for the data poisoning attack. In addition, traditional unlearning algorithms often struggle to effectively remove the influence of poisoned samples, particularly when only a few affected examples can be identified. To address these challenge, we introduce $\Delta$-Influence, a novel approach that leverages influence functions to trace abnormal model behavior back to the responsible poisoned training data using as little as just one poisoned test example. $\Delta$-Influence applies data transformations that sever the link between poisoned training data and compromised test points without significantly affecting clean data. This allows $\Delta$-Influence to detect large negative shifts in influence scores following data transformations, a phenomenon we term as influence collapse, thereby accurately identifying poisoned training data. Unlearning this subset, e.g. through retraining, effectively eliminates the data poisoning. We validate our method across three vision-based poisoning attacks and three datasets, benchmarking against four detection algorithms and five unlearning strategies. We show that $\Delta$-Influence consistently achieves the best unlearning across all settings, showing the promise of influence functions for corrective unlearning. Our code is publicly available at: \url{https://github.com/andyisokay/delta-influence}, Comment: Accepted at NeurIPS Workshop on Attributing Model Behavior at Scale (ATTRIB @ NeurIPS 2024)

Pulsar timing array observations have found evidence for an isotropic gravitational wave background with the Hellings-Downs angular correlations, expected from general relativity. This interpretation hinges on the measured shape of the angular correlations, which is predominately quadrupolar under general relativity. Here we explore a more flexible parameterization: we expand the angular correlations into a sum of Legendre polynomials and use a Bayesian analysis to constrain their coefficients with the 15-year pulsar timing data set collected by the North American Nanohertz Observatory for Gravitational Waves (NANOGrav). When including Legendre polynomials with multipoles $\ell \geq 2$, we only find a significant signal in the quadrupole with an amplitude consistent with general relativity and non-zero at the $\sim 95\%$ confidence level and a Bayes factor of 200. When we include multipoles $\ell \leq 1$, the Bayes factor evidence for quadrupole correlations decreases by more than an order of magnitude due to evidence for a monopolar signal at approximately 4 nHz which has also been noted in previous analyses of the NANOGrav 15-year data. Further work needs to be done in order to better characterize the properties of this monopolar signal and its effect on the evidence for quadrupolar angular correlations., Comment: 15 pages, 6 figures

The detection of a stochastic gravitational wave background by pulsar timing arrays suggests the presence of a supermassive black hole binary population. Although the observed spectrum generally aligns with predictions from orbital evolution driven by gravitational wave emission in circular orbits, there is a discernible preference for a turnover at the lowest observed frequencies. This turnover could indicate a significant hardening phase, transitioning from early environmental influences to later stages predominantly influenced by gravitational wave emission. In the vicinity of these binaries, the ejection of stars or dark matter particles through gravitational three-body slingshots efficiently extracts orbital energy, leading to a low-frequency turnover in the spectrum. By analyzing the NANOGrav 15-year data, we assess how the gravitational wave spectrum depends on the initial inner galactic profile prior to disruption by binary ejections, accounting for a range of initial binary eccentricities. Our findings suggest a parsec-scale galactic center density around $10^6\,M_\odot/\textrm{pc}^3$ across most of the parameter space, offering insights into the environmental effects on black hole evolution and combined matter density near galaxy centers., Comment: 15 pages, 5 figures

One of the most challenging forms of misinformation involves the out-of-context (OOC) use of images paired with misleading text, creating false narratives. Existing AI-driven detection systems lack explainability and require expensive fine-tuning. We address these issues with MAD-Sherlock: a Multi-Agent Debate system for OOC Misinformation Detection. MAD-Sherlock introduces a novel multi-agent debate framework where multimodal agents collaborate to assess contextual consistency and request external information to enhance cross-context reasoning and decision-making. Our framework enables explainable detection with state-of-the-art accuracy even without domain-specific fine-tuning. Extensive ablation studies confirm that external retrieval significantly improves detection accuracy, and user studies demonstrate that MAD-Sherlock boosts performance for both experts and non-experts. These results position MAD-Sherlock as a powerful tool for autonomous and citizen intelligence applications.

The Zirconium (Z = 40) isotopic chain has attracted interest for more than four decades. The abrupt lowering of the energy of the first $2^+$ state and the increase in the transition strength B(E2; $2_1^\rightarrow 0_1^+$ going from $^{98}$Zr to $^{100}$Zr has been the first example of "quantum phase transition" in nuclear shapes, which has few equivalents in the nuclear chart. Although a multitude of experiments have been performed to measure nuclear properties related to nuclear shapes and collectivity in the region, none of the measured lifetimes were obtained using the Recoil Distance Doppler Shift method in the $\gamma\gamma$-coincidence mode where a gate on the direct feeding transition of the state of interest allows a strict control of systematical errors. This work reports the results of lifetime measurements for the first yrast excited states in $^{98-104}$Zr carried out to extract reduced transition probabilities. The new lifetime values in $\gamma\gamma$-coincidence and $\gamma$-single mode are compared with the results of former experiments. Recent predictions of the Interacting Boson Model with Configuration Mixing, the Symmetry Conserving Configuration Mixing model based on the Hartree-Fock-Bogoliubov approach and the Monte Carlo Shell Model are presented and compared with the experimental data.

The Workflows Community Summit gathered 111 participants from 18 countries to discuss emerging trends and challenges in scientific workflows, focusing on six key areas: time-sensitive workflows, AI-HPC convergence, multi-facility workflows, heterogeneous HPC environments, user experience, and FAIR computational workflows. The integration of AI and exascale computing has revolutionized scientific workflows, enabling higher-fidelity models and complex, time-sensitive processes, while introducing challenges in managing heterogeneous environments and multi-facility data dependencies. The rise of large language models is driving computational demands to zettaflop scales, necessitating modular, adaptable systems and cloud-service models to optimize resource utilization and ensure reproducibility. Multi-facility workflows present challenges in data movement, curation, and overcoming institutional silos, while diverse hardware architectures require integrating workflow considerations into early system design and developing standardized resource management tools. The summit emphasized improving user experience in workflow systems and ensuring FAIR workflows to enhance collaboration and accelerate scientific discovery. Key recommendations include developing standardized metrics for time-sensitive workflows, creating frameworks for cloud-HPC integration, implementing distributed-by-design workflow modeling, establishing multi-facility authentication protocols, and accelerating AI integration in HPC workflow management. The summit also called for comprehensive workflow benchmarks, workflow-specific UX principles, and a FAIR workflow maturity model, highlighting the need for continued collaboration in addressing the complex challenges posed by the convergence of AI, HPC, and multi-facility research environments.

Sparse autoencoders (SAEs) are a recent technique for decomposing neural network activations into human-interpretable features. However, in order for SAEs to identify all features represented in frontier models, it will be necessary to scale them up to very high width, posing a computational challenge. In this work, we introduce Switch Sparse Autoencoders, a novel SAE architecture aimed at reducing the compute cost of training SAEs. Inspired by sparse mixture of experts models, Switch SAEs route activation vectors between smaller "expert" SAEs, enabling SAEs to efficiently scale to many more features. We present experiments comparing Switch SAEs with other SAE architectures, and find that Switch SAEs deliver a substantial Pareto improvement in the reconstruction vs. sparsity frontier for a given fixed training compute budget. We also study the geometry of features across experts, analyze features duplicated across experts, and verify that Switch SAE features are as interpretable as features found by other SAE architectures., Comment: Code available at https://github.com/amudide/switch_sae

A key challenge in interpretability is to decompose model activations into meaningful features. Sparse autoencoders (SAEs) have emerged as a promising tool for this task. However, a central problem in evaluating the quality of SAEs is the absence of ground truth features to serve as an evaluation gold standard. Current evaluation methods for SAEs are therefore confronted with a significant trade-off: SAEs can either leverage toy models or other proxies with predefined ground truth features; or they use extensive prior knowledge of realistic task circuits. The former limits the generalizability of the evaluation results, while the latter limits the range of models and tasks that can be used for evaluations. We introduce SAGE: Scalable Autoencoder Ground-truth Evaluation, a ground truth evaluation framework for SAEs that scales to large state-of-the-art SAEs and models. We demonstrate that our method can automatically identify task-specific activations and compute ground truth features at these points. Compared to previous methods we reduce the training overhead by introducing a novel reconstruction method that allows to apply residual stream SAEs to sublayer activations. This eliminates the need for SAEs trained on every task-specific activation location. Then we validate the scalability of our framework, by evaluating SAEs on novel tasks on Pythia70M, GPT-2 Small, and Gemma-2-2. Our framework therefore paves the way for generalizable, large-scale evaluations of SAEs in interpretability research.

The rapid proliferation of AI-manipulated or generated audio deepfakes poses serious challenges to media integrity and election security. Current AI-driven detection solutions lack explainability and underperform in real-world settings. In this paper, we introduce novel explainability methods for state-of-the-art transformer-based audio deepfake detectors and open-source a novel benchmark for real-world generalizability. By narrowing the explainability gap between transformer-based audio deepfake detectors and traditional methods, our results not only build trust with human experts, but also pave the way for unlocking the potential of citizen intelligence to overcome the scalability issue in audio deepfake detection.

As a powerful and rapidly advancing dual-use technology, AI offers both immense benefits and worrisome risks. In response, governing bodies around the world are developing a range of regulatory AI laws and policies. This paper compares three distinct approaches taken by the EU, China and the US. Within the US, we explore AI regulation at both the federal and state level, with a focus on California's pending Senate Bill 1047. Each regulatory system reflects distinct cultural, political and economic perspectives. Each also highlights differing regional perspectives on regulatory risk-benefit tradeoffs, with divergent judgments on the balance between safety versus innovation and cooperation versus competition. Finally, differences between regulatory frameworks reflect contrastive stances in regards to trust in centralized authority versus trust in a more decentralized free market of self-interested stakeholders. Taken together, these varied approaches to AI innovation and regulation influence each other, the broader international community, and the future of AI regulation., Comment: 36 pages, 11 figures and tables

The application of average Hamiltonian theory (AHT) to magnetic resonance and quantum sensing informs pulse sequence design, for example, by providing efficient approximations of spin dynamics while retaining important physical characteristics of system evolution. However, AHT predictions break down in many common experimental conditions, including for sensing with solid-state spins. Here we establish that certain symmetries, such as rapid echos, allow AHT to remain accurate well beyond the perturbative limit. An exact method is presented to determine the sensor response to a target signal, which stays valid beyond the regime of AHT convergence. This beyond AHT approach enables new opportunities in quantum control techniques that leverage complementary analytical and numerical methods, with applications in a variety of quantum sensing platforms, Hamiltonian engineering, and probes of quantum many-body phenomena., Comment: 6 pages, 4 figures

The rapid proliferation of frontier model agents promises significant societal advances but also raises concerns about systemic risks arising from unsafe interactions. Collusion to the disadvantage of others has been identified as a central form of undesirable agent cooperation. The use of information hiding (steganography) in agent communications could render collusion practically undetectable. This underscores the need for evaluation frameworks to monitor and mitigate steganographic collusion capabilities. We address a crucial gap in the literature by demonstrating, for the first time, that robust steganographic collusion in LLMs can arise indirectly from optimization pressure. To investigate this problem we design two approaches -- a gradient-based reinforcement learning (GBRL) method and an in-context reinforcement learning (ICRL) method -- for reliably eliciting sophisticated LLM-generated linguistic text steganography. Importantly, we find that emergent steganographic collusion can be robust to both passive steganalytic oversight of model outputs and active mitigation through communication paraphrasing. We contribute a novel model evaluation framework and discuss limitations and future work. Our findings imply that effective risk mitigation from steganographic collusion post-deployment requires innovation in passive and active oversight techniques.

We introduce and investigate a generalization of the Hele-Shaw flow with injection where several droplets compete for space as they try to expand due to internal pressure while still preserving their topology. Droplets are described by their closed non-crossing interface curves in $\mathbb{C}$ or more generally in a Riemann surface of finite type. Our main focus is on stationary solutions which we show correspond to the critical vertical trajectories of a particular quadratic differential with second order poles at the source points. The quadratic differentials that arise in this way have a simple description in terms of their associated half-translation surfaces. Existence of stationary solutions is proved in some generality by solving an extremal problem involving an electrostatic energy functional, generalizing a classic problem studied by Teichm\"uller, Jenkins, Strebel and others. We study several special cases, including stationary Jordan curves on the Riemann sphere. We also introduce a discrete random version of the dynamics closely related to Propp's competitive erosion model, and conjecture that realizations of the lattice model will converge towards a corresponding solution to the competitive Hele-Shaw problem as the mesh size tends to zero., Comment: 34 pages, 13 figures

Global expansion of the Event Horizon Telescope (EHT) will see the strategic addition of antennas at new geographical locations, transforming the sensitivity and imaging fidelity of the $\lambda \sim 1\,$mm EHT array. A possible South African EHT station would leverage a strong geographical advantage, local infrastructure, and radio astronomy expertise, and have strong synergies with the Africa Millimetre Telescope in Namibia. We assessed three South African candidate millimetre sites using climatological simulations and found at least two promising sites. These sites are comparable to some existing EHT stations during the typical April EHT observing window and outperform them during most of the year, especially the southern hemisphere winter. Interferometric simulations of Africa-enhanced EHT arrays under the simulated atmospheric conditions demonstrate the improved array performance. In typical weather, the number of reliable visibility detections increased considerably, especially at $(u, v)$-distances corresponding to the angular sizes of the Sagittarius A$^*$ and Messier 87$^*$ black hole shadow diameters ($\sim40\,\mathrm{\mu}$as to $50\,\mathrm{\mu}$as). The simulation results underscore the sizable, positive impact of a strategically placed South African EHT station on ngEHT objectives and the resulting black hole science., Comment: 6 pages, 3 figures, 1 table. Submitted to URSI RSL

The NANOGrav 15-year data provides compelling evidence for a stochastic gravitational-wave (GW) background at nanohertz frequencies. The simplest model-independent approach to characterizing the frequency spectrum of this signal consists in a simple power-law fit involving two parameters: an amplitude A and a spectral index \gamma. In this paper, we consider the next logical step beyond this minimal spectral model, allowing for a running (i.e., logarithmic frequency dependence) of the spectral index, \gamma_run(f) = \gamma + \beta \ln(f/f_ref). We fit this running-power-law (RPL) model to the NANOGrav 15-year data and perform a Bayesian model comparison with the minimal constant-power-law (CPL) model, which results in a 95% credible interval for the parameter \beta consistent with no running, \beta \in [-0.80,2.96], and an inconclusive Bayes factor, B(RPL vs. CPL) = 0.69 +- 0.01. We thus conclude that, at present, the minimal CPL model still suffices to adequately describe the NANOGrav signal; however, future data sets may well lead to a measurement of nonzero \beta. Finally, we interpret the RPL model as a description of primordial GWs generated during cosmic inflation, which allows us to combine our results with upper limits from big-bang nucleosynthesis, the cosmic microwave background, and LIGO-Virgo-KAGRA., Comment: 17 pages, 4 figures, 2 tables

We present here the current state of a collection of promising ultraviolet technologies in preparation for the Habitable Worlds Observatory. Working with experts representing a significant number of groups working in the ultraviolet, we summarize some of the leading science drivers, present an argument for a 100 nm blue wavelength cutoff, and gather current state of the art of UV technologies. We present the state of the art of contamination control, a crucial piece of the UV instrument plan. We explore next steps with individual technologies, as well as present paths forward with systems level testing and development.

Elasmobranchs (shark sand rays) represent a critical component of marine ecosystems. Yet, they are experiencing global population declines and effective monitoring of populations is essential to their protection. Underwater stationary videos, such as those from Baited Remote Underwater Video Stations (BRUVS), are critical for understanding elasmobranch spatial ecology and abundance. However, processing these videos requires time-consuming manual analysis that can delay conservation. To address this challenge, we developed SharkTrack, a semi-automatic underwater video analysis software. SharkTrack uses Convolutional Neural Networks (CNN) and Multi-Object Tracking to automatically detect and track elasmobranchs and provides an annotation pipeline to manually classify elasmobranch species and compute species-specific MaxN (ssMaxN), the standard metric of relative abundance. When tested on BRUVS footage from locations unseen by the CNN model during training, SharkTrack computed ssMaxN with 89% accuracy over 207 hours of footage. The semi-automatic SharkTrack pipeline required two minutes of manual classification per hour of video, an estimated 95% reduction of manual analysis time compared to traditional methods. Furthermore, we demonstrate SharkTrack accuracy across diverse marine ecosystems and elasmobranch species, an advancement compared to previous models, which were limited to specific species or locations. SharkTrack applications extend beyond BRUVS, facilitating the analysis of any underwater stationary video. By making video analysis faster and more accessible, SharkTrack enables research and conservation organisations to monitor elasmobranch populations more efficiently, thereby improving conservation efforts. To further support these goals, we provide public access to the SharkTrack software.

Pulsar-timing-array experiments have reported evidence for a stochastic background of nanohertz gravitational waves consistent with the signal expected from a population of supermassive--black-hole binaries. Those analyses assume power-law spectra for intrinsic pulsar noise and for the background, as well as a Hellings--Downs cross-correlation pattern among the gravitational-wave--induced residuals across pulsars. These assumptions are idealizations that may not be realized in actuality. We test them in the NANOGrav 15 yr data set using Bayesian posterior predictive checks: after fitting our fiducial model to real data, we generate a population of simulated data-set replications, and use them to assess whether the optimal-statistic significance, inter-pulsar correlations, and spectral coefficients assume extreme values for the real data when compared to the replications. We confirm that the NANOGrav 15 yr data set is consistent with power-law and Hellings--Downs assumptions. We also evaluate the evidence for the stochastic background using posterior-predictive versions of the frequentist optimal statistic and of Bayesian model comparison, and find comparable significance (3.2\ $\sigma$ and 3\ $\sigma$ respectively) to what was previously reported for the standard statistics. We conclude with novel visualizations of the reconstructed gravitational waveforms that enter the residuals for each pulsar. Our analysis strengthens confidence in the identification and characterization of the gravitational-wave background as reported by NANOGrav., Comment: 20 pages, 14 Figures

Electrochemical Impedance Spectroscopy (EIS) is a crucial technique for assessing corrosion of a metallic materials. The analysis of EIS hinges on the selection of an appropriate equivalent circuit model (ECM) that accurately characterizes the system under study. In this work, we systematically examined the applicability of three commonly used ECMs across several typical material degradation scenarios. By applying Bayesian Inference to simulated corrosion EIS data, we assessed the suitability of these ECMs under different corrosion conditions and identified regions where the EIS data lacks sufficient information to statistically substantiate the ECM structure. Additionally, we posit that the traditional approach to EIS analysis, which often requires measurements to very low frequencies, might not be always necessary to correctly model the appropriate ECM. Our study assesses the impact of omitting data from low to medium-frequency ranges on inference results and reveals that a significant portion of low-frequency measurements can be excluded without substantially compromising the accuracy of extracting system parameters. Further, we propose simple checks to the posterior distributions of the ECM components and posterior predictions, which can be used to quantitatively evaluate the suitability of a particular ECM and the minimum frequency required to be measured. This framework points to a pathway for expediting EIS acquisition by intelligently reducing low-frequency data collection and permitting on-the-fly EIS measurements

Using the full potential of LLMs in higher education is hindered by challenges with access to LLMs. The two main access modes currently discussed are paying for a cloud-based LLM or providing a locally maintained open LLM. In this paper, we describe the current state of establishing an open LLM infrastructure at FernUniversit\"at in Hagen under the project name FLEXI (FernUni LLM Experimental Infrastructure). FLEXI enables experimentation within teaching and research with the goal of generating strongly needed evidence in favor (or against) the use of locally maintained open LLMs in higher education. The paper will provide some practical guidance for everyone trying to decide whether to run their own LLM server.

AI systems are increasingly pervasive, yet information needed to decide whether and how to engage with them may not exist or be accessible. A user may not be able to verify whether a system has certain safety certifications. An investigator may not know whom to investigate when a system causes an incident. It may not be clear whom to contact to shut down a malfunctioning system. Across a number of domains, IDs address analogous problems by identifying particular entities (e.g., a particular Boeing 747) and providing information about other entities of the same class (e.g., some or all Boeing 747s). We propose a framework in which IDs are ascribed to instances of AI systems (e.g., a particular chat session with Claude 3), and associated information is accessible to parties seeking to interact with that system. We characterize IDs for AI systems, provide concrete examples where IDs could be useful, argue that there could be significant demand for IDs from key actors, analyze how those actors could incentivize ID adoption, explore a potential implementation of our framework for deployers of AI systems, and highlight limitations and risks. IDs seem most warranted in settings where AI systems could have a large impact upon the world, such as in making financial transactions or contacting real humans. With further study, IDs could help to manage a world where AI systems pervade society., Comment: Under review; accepted to RegML workshop at NeurIPS 2024

Constrained single-objective problems have been frequently tackled by evolutionary multi-objective algorithms where the constraint is relaxed into an additional objective. Recently, it has been shown that Pareto optimization approaches using bi-objective models can be significantly sped up using sliding windows (Neumann and Witt, ECAI 2023). In this paper, we extend the sliding window approach to $3$-objective formulations for tackling chance constrained problems. On the theoretical side, we show that our new sliding window approach improves previous runtime bounds obtained in (Neumann and Witt, GECCO 2023) while maintaining the same approximation guarantees. Our experimental investigations for the chance constrained dominating set problem show that our new sliding window approach allows one to solve much larger instances in a much more efficient way than the 3-objective approach presented in (Neumann and Witt, GECCO 2023)., Comment: To appear at PPSN 2024

The rapid proliferation of open-source language models significantly increases the risks of downstream backdoor attacks. These backdoors can introduce dangerous behaviours during model deployment and can evade detection by conventional cybersecurity monitoring systems. In this paper, we introduce a novel class of backdoors in autoregressive transformer models, that, in contrast to prior art, are unelicitable in nature. Unelicitability prevents the defender from triggering the backdoor, making it impossible to evaluate or detect ahead of deployment even if given full white-box access and using automated techniques, such as red-teaming or certain formal verification methods. We show that our novel construction is not only unelicitable thanks to using cryptographic techniques, but also has favourable robustness properties. We confirm these properties in empirical investigations, and provide evidence that our backdoors can withstand state-of-the-art mitigation strategies. Additionally, we expand on previous work by showing that our universal backdoors, while not completely undetectable in white-box settings, can be harder to detect than some existing designs. By demonstrating the feasibility of seamlessly integrating backdoors into transformer models, this paper fundamentally questions the efficacy of pre-deployment detection strategies. This offers new insights into the offence-defence balance in AI safety and security., Comment: 10 pages, 5 figures

Minimum-entropy coupling (MEC) -- the process of finding a joint distribution with minimum entropy for given marginals -- has applications in areas such as causality and steganography. However, existing algorithms are either computationally intractable for large-support distributions or limited to specific distribution types and sensitive to hyperparameter choices. This work addresses these limitations by unifying a prior family of iterative MEC (IMEC) approaches into a generalized partition-based formalism. From this framework, we derive a novel IMEC algorithm called ARIMEC, capable of handling arbitrary discrete distributions, and introduce a method to make IMEC robust to suboptimal hyperparameter settings. These innovations facilitate the application of IMEC to high-throughput steganography with language models, among other settings. Our codebase is available at https://github.com/ssokota/mec .

Blockchain technology and Artificial Intelligence (AI) have emerged as transformative forces in their respective domains. This paper explores synergies and challenges between these two technologies. Our research analyses the biggest projects combining blockchain and AI, based on market capitalization, and derives a novel framework to categorize contemporary and future use cases. Despite the theoretical compatibility, current real-world applications combining blockchain and AI remain in their infancy.

Organic electro-optic materials have demonstrated promising performance in developing electro-optic phase shifters. Their integration with other silicon photonic processes, nanofabrication complexities, and durability remain to be developed. While the required poling step in electro-optic polymers limits their potential and utilization on a large scale, devices made of paraelectric nematic liquid crystals suffer from slow bandwidth. In ferroelectric nematic liquid crystals, we report an additional GHz-fast phase shift that ultimately allows for significant second-order nonlinear optical coefficients and the related Pockels effect. It avoids poling issues and can pave the way for hybrid silicon-organic systems with CMOS-foundry compatibility. We report DC and AC modulation efficiencies of $\approx$0.25 V$\cdot$mm and $\approx$25.7 V$\cdot$mm, respectively, an on-chip insertion loss of $\approx$2.1 dB, and an electro-optic bandwidth of $f_{-6dB}$>4.18 GHz, employing improved light-matter interaction in a waveguide architecture that calls for only one lithography step., Comment: 25 pages, 5 figures

Intercalation of epitaxial graphene on SiC(0001) with Sn results in a well-ordered 2D metallic Sn phase with a $(1\times1)$ structure at the interface between SiC substrate and quasi-freestanding graphene. The 2D\,Sn phase exhibits exotic electronic properties with Dirac-like and flat bands coexisting close to the Fermi level that exhibit both Zeeman- and Rashba-type spin splittings. Possible inter-layer interactions between the 2D\,Sn layer and graphene that may result in emerging electronic properties remain unexplored. We use time- and angle-resolved photoemission spectroscopy to reveal a surprisingly short-lived non-equilibrium carrier distribution inside the Dirac cone of graphene. Further, we find that the graphene $\pi$-band exhibits a transient down-shift that we attribute to charging of the graphene layer with holes. We interpret our results with support from density functional theory calculations of the graphene - 2D\,Sn heterostructure that reveal a substantial hybridization between graphene $\pi$-band and Sn $p_z$-states that opens up a $\sim230$\,meV band gap inside the Dirac cone and delocalizes the charge carriers over both the graphene and 2D\,Sn layers. Our results have important implications for the design of future ultrafast optoelectronic devices that may find applications in the fields of light harvesting and detection, as supercapacitors, or in novel quantum computing technologies., Comment: 19 pages, 5 figures

In the next few years, applications of Generative AI are expected to revolutionize a number of different areas, ranging from science & medicine to education. The potential for these seismic changes has triggered a lively debate about potential risks and resulted in calls for tighter regulation, in particular from some of the major tech companies who are leading in AI development. This regulation is likely to put at risk the budding field of open-source Generative AI. We argue for the responsible open sourcing of generative AI models in the near and medium term. To set the stage, we first introduce an AI openness taxonomy system and apply it to 40 current large language models. We then outline differential benefits and risks of open versus closed source AI and present potential risk mitigation, ranging from best practices to calls for technical and scientific contributions. We hope that this report will add a much needed missing voice to the current public discourse on near to mid-term AI safety and other societal impact., Comment: Accepted to ICML'24 as a position paper

The JWST has captured the sharpest IR images ever taken of the Horsehead nebula, a prototypical moderately irradiated PDR that is fully representative of most of the UV-illuminated molecular gas in the Milky Way and star-forming galaxies. We investigate the impact of FUV radiation of a molecular cloud and constrain the structure of the edge of the PDR and its illumination conditions. We used NIRCam and MIRI to obtain 17 broadband and 6 narrowband maps from 0.7 to 28 $\mu$m. We mapped the dust emission, scattered light, and several gas phase lines. We also used HST-WFC3 maps at 1.1 and 1. 6 $\mu$m, along with HST-STIS spectroscopic observations of the H$\alpha$ line. We probed the structure of the edge of the Horsehead and resolved its spatial complexity. We detected a network of faint striated features extending perpendicularly to the PDR front into the H\,II region in filters sensitive to nano-grain emission and light scattered by larger grains. This may indeed figure as the first detection of the entrainment of dust particles in the evaporative flow. The map of the 1-0 S(1) line of H$_2$ presents sharp sub-structures on scales as small as 1.5 arcsec. The ionization and dissociation fronts appear at distances 1-2 arcsec behind the edge of the PDR and seem to spatially coincide, indicating a thickness of the neutral atomic layer below 100 au. All broadband maps present strong color variations which can be explained by dust attenuation. Deviations of the emissions in the H$\alpha$, Pa$\alpha,$ and Br$\alpha$ lines also indicate dust attenuation. With a very simple model, we derive the main features of the extinction curve. A small excess of extinction at 3 $\mu$m may be attributed to icy H$_2$O mantles onto grains. In all lines of sight crossing the inner regions of the Horsehead, it appears that dust attenuation is non-negligible over the entire spectral range., Comment: 25 pages, 17 figures

A class of metaheuristic techniques called estimation-of-distribution algorithms (EDAs) are employed in optimization as more sophisticated substitutes for traditional strategies like evolutionary algorithms. EDAs generally drive the search for the optimum by creating explicit probabilistic models of potential candidate solutions through repeated sampling and selection from the underlying search space. Most theoretical research on EDAs has focused on pseudo-Boolean optimization. Jedidia et al. (GECCO 2023) proposed the first EDAs for optimizing problems involving multi-valued decision variables. By building a framework, they have analyzed the runtime of a multi-valued UMDA on the r-valued LeadingOnes function. Using their framework, here we focus on the multi-valued compact genetic algorithm (r-cGA) and provide a first runtime analysis of a generalized OneMax function. To prove our results, we investigate the effect of genetic drift and progress of the probabilistic model towards the optimum. After finding the right algorithm parameters, we prove that the r-cGA solves this r-valued OneMax problem efficiently. We show that with high probability, the runtime bound is O(r2 n log2 r log3 n). At the end of experiments, we state one conjecture related to the expected runtime of another variant of multi-valued OneMax function.

This work identifies 18 foundational challenges in assuring the alignment and safety of large language models (LLMs). These challenges are organized into three different categories: scientific understanding of LLMs, development and deployment methods, and sociotechnical challenges. Based on the identified challenges, we pose $200+$ concrete research questions.

With the STAR experiment at the BNL Relativisic Heavy Ion Collider, we characterize $\sqrt{s_\mathrm{NN}}$ = 200 GeV p+Au collisions by event activity (EA) measured within the pseudorapidity range $eta$ $in$ [-5, -3.4] in the Au-going direction and report correlations between this EA and hard- and soft- scale particle production at midrapidity ($\eta$ $\in$ [-1, 1]). At the soft scale, charged particle production in low-EA p+Au collisions is comparable to that in p+p collisions and increases monotonically with increasing EA. At the hard scale, we report measurements of high transverse momentum (pT) jets in events of different EAs. In contrast with the soft particle production, high-pT particle production and EA are found to be inversely related. To investigate whether this is a signal of jet quenching in high-EA events, we also report ratios of pT imbalance and azimuthal separation of dijets in high- and low-EA events. Within our measurement precision, no significant differences are observed, disfavoring the presence of jet quenching in the highest 30% EA p+Au collisions at $\sqrt{s_\mathrm{NN}}$ = 200 GeV., Comment: 12 page, 9 figures

We study poly-crystalline spherical drops of an aqueous suspension of highly charged colloidal spheres exposed to a colloid-free aqueous environment. Crystal contours were obtained from standard optical imaging. The crystal spheres first expand to nearly four times their initial volume before slowly shrinking due to dilution-induced melting. Exploiting coherent multiple-scattering by (110) Bragg reflecting crystals, time-dependent density profiles were recorded deep within the drop interior. These show a continuously flattening radial density gradient and a decreasing central density. Expansion curves and density profiles are qualitatively consistent with theoretical expectations based on dynamical density functional theory for the expansion of a spherical crystallite made of charged Brownian spheres. We anticipate that our study opens novel experimental access to densi-ty determination in turbid crystals., Comment: Thoroughly revised version. now 23 pages with 9 figures and 57 references; supplementary materials 15 pages with 11 figures and 22 references. Accepted for publication in Soft Matter in August 2024

While reinforcement learning (RL) algorithms have been successfully applied across numerous sequential decision-making problems, their generalization to unforeseen testing environments remains a significant concern. In this paper, we study the problem of out-of-distribution (OOD) detection in RL, which focuses on identifying situations at test time that RL agents have not encountered in their training environments. We first propose a clarification of terminology for OOD detection in RL, which aligns it with the literature from other machine learning domains. We then present new benchmark scenarios for OOD detection, which introduce anomalies with temporal autocorrelation into different components of the agent-environment loop. We argue that such scenarios have been understudied in the current literature, despite their relevance to real-world situations. Confirming our theoretical predictions, our experimental results suggest that state-of-the-art OOD detectors are not able to identify such anomalies. To address this problem, we propose a novel method for OOD detection, which we call DEXTER (Detection via Extraction of Time Series Representations). By treating environment observations as time series data, DEXTER extracts salient time series features, and then leverages an ensemble of isolation forest algorithms to detect anomalies. We find that DEXTER can reliably identify anomalies across benchmark scenarios, exhibiting superior performance compared to both state-of-the-art OOD detectors and high-dimensional changepoint detectors adopted from statistics., Comment: Accepted as a full paper to the 23rd International Conference on Autonomous Agents and Multiagent Systems (AAMAS 2024)

The cosmic merger history of supermassive black hole binaries (SMBHBs) is expected to produce a low-frequency gravitational wave background (GWB). Here we investigate how signs of the discrete nature of this GWB can manifest in pulsar timing arrays through excursions from, and breaks in, the expected $f_{\mathrm{GW}}^{-2/3}$ power-law of the GWB strain spectrum. To do this, we create a semi-analytic SMBHB population model, fit to NANOGrav's 15 yr GWB amplitude, and with 1,000 realizations we study the populations' characteristic strain and residual spectra. Comparing our models to the NANOGrav 15 yr spectrum, we find two interesting excursions from the power-law. The first, at $2 \; \mathrm{nHz}$, is below our GWB realizations with $p$-value significance $p = 0.05$ to $0.06$ ($\approx 1.8 \sigma - 1.9 \sigma$). The second, at $16 \; \mathrm{nHz}$, is above our GWB realizations with $p = 0.04$ to $0.15$ ($\approx 1.4 \sigma - 2.1 \sigma$). We explore the properties of a loud SMBHB which could cause such an excursion. Our simulations also show that the expected number of SMBHBs decreases by three orders of magnitude, from $\sim 10^6$ to $\sim 10^3$, between $2\; \mathrm{nHz}$ and $20 \; \mathrm{nHz}$. This causes a break in the strain spectrum as the stochasticity of the background breaks down at $26^{+28}_{-19} \; \mathrm{nHz}$, consistent with predictions pre-dating GWB measurements. The diminished GWB signal from SMBHBs at frequencies above the $26~\mathrm{nHz}$ break opens a window for PTAs to detect continuous GWs from individual SMBHBs or GWs from the early universe., Comment: 13 pages, 8 figures, 2 appendices, in press at ApJ

The emerging technology of quantum computing has the potential to change the way how problems will be solved in the future. This work presents a centralized network control algorithm executable on already existing quantum computer which are based on the principle of quantum annealing like the D-Wave Advantage. We introduce a resource reoccupation algorithm for traffic engineering in wide-area networks. The proposed optimization algorithm changes traffic steering and resource allocation in case of overloaded transceivers. Settings of active components like fiber amplifiers and transceivers are not changed for the reason of stability. This algorithm is beneficial in situations when the network traffic is fluctuating in time scales of seconds or spontaneous bursts occur. Further, we developed a discrete-time flow simulator to study the algorithm's performance in wide-area networks. Our network simulator considers backlog and loss modeling of buffered transmission lines. Concurring flows are handled equally in case of a backlog. This work provides an ILP-based network configuring algorithm that is applicable on quantum annealing computers. We showcase, that traffic losses can be reduced significantly by a factor of 2 if a resource reoccupation algorithm is applied in a network with bursty traffic. As resources are used more efficiently by reoccupation in heavy load situations, overprovisioning of networks can be reduced. Thus, this new form of network operation leads toward a zero-margin network. We show that our newly introduced network simulator enables analyses of short-time effects like buffering within fat-pipe networks. As the calculation of network configurations in real-sized networks is typically time-consuming, quantum computing can enable the proposed network configuration algorithm for application in real-sized wide-area networks., Comment: 7 pages, 9 figures, accepted for publication at "IEEE International Conference on High Performance Switching and Routing 2024"

We propose a new, flexible approach for dynamically maintaining successful mutation rates in evolutionary algorithms using $k$-bit flip mutations. The algorithm adds successful mutation rates to an archive of promising rates that are favored in subsequent steps. Rates expire when their number of unsuccessful trials has exceeded a threshold, while rates currently not present in the archive can enter it in two ways: (i) via user-defined minimum selection probabilities for rates combined with a successful step or (ii) via a stagnation detection mechanism increasing the value for a promising rate after the current bit-flip neighborhood has been explored with high probability. For the minimum selection probabilities, we suggest different options, including heavy-tailed distributions. We conduct rigorous runtime analysis of the flexible evolutionary algorithm on the OneMax and Jump functions, on general unimodal functions, on minimum spanning trees, and on a class of hurdle-like functions with varying hurdle width that benefit particularly from the archive of promising mutation rates. In all cases, the runtime bounds are close to or even outperform the best known results for both stagnation detection and heavy-tailed mutations.

Mid-infrared emission features probe the properties of ionized gas, and hot or warm molecular gas. The Orion Bar is a frequently studied photodissociation region (PDR) containing large amounts of gas under these conditions, and was observed with the MIRI IFU aboard JWST as part of the "PDRs4All" program. The resulting IR spectroscopic images of high angular resolution (0.2") reveal a rich observational inventory of mid-IR emission lines, and spatially resolve the substructure of the PDR, with a mosaic cutting perpendicularly across the ionization front and three dissociation fronts. We extracted five spectra that represent the ionized, atomic, and molecular gas layers, and measured the most prominent gas emission lines. An initial analysis summarizes the physical conditions of the gas and the potential of these data. We identified around 100 lines, report an additional 18 lines that remain unidentified, and measured the line intensities and central wavelengths. The H I recombination lines originating from the ionized gas layer bordering the PDR, have intensity ratios that are well matched by emissivity coefficients from H recombination theory, but deviate up to 10% due contamination by He I lines. We report the observed emission lines of various ionization stages of Ne, P, S, Cl, Ar, Fe, and Ni, and show how certain line ratios vary between the five regions. We observe the pure-rotational H$_2$ lines in the vibrational ground state from 0-0 S(1) to 0-0 S(8), and in the first vibrationally excited state from 1-1 S(5) to 1-1 S(9). We derive H$_2$ excitation diagrams, and approximate the excitation with one thermal (~700 K) component representative of an average gas temperature, and one non-thermal component (~2700 K) probing the effect of UV pumping. We compare these results to an existing model for the Orion Bar PDR and highlight the differences with the observations., Comment: 26 pages, 12 figures, 3 tables. Submitted to A&A, under review (1st revision)