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2. Self-assembly of bidentate ligands for combinatorial homogeneous catalysis: Asymmetric rhodium-catalyzed hydrogenation

Author

Weis, Martine, Waloch, Christoph, Seiche, Wolfgang, and Breit, Bernhard

Subjects
Ligands -- Research, Hydrogen bonding -- Research, Hydrogenation -- Research, Chemistry
Abstract

The first bidentate phosphorous donor ligand library based on self-assembly through hydrogen bonding was generated and screened from rhodium-catalyzed asymmetric hydrogenation. Bidentate ligand combinations of phosphine/phosphonites as well as diphosphonite systems were identified that furnish excellent catalysts with enantioselectivities of upto 99%.

Published
2006

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