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Plasmonic optical fiber sensors are continuously developed for (bio)chemical sensing purposes. Recently, surface plasmon resonance (SPR) generation was achieved in gold-coated tilted fiber Bragg gratings (TFBGs). These sensors probe the surrounding medium with near-infrared narrowband resonances, which enhances both the penetration depth of the evanescent field in the external medium and the wavelength resolution of the interrogation. They constitute a unique configuration to probe all the fiber cladding modes individually. We use them to analyze the modal distribution of gold-coated telecommunication-grade optical fibers immersed in aqueous solutions. Theoretical investigations with a finite-difference complex mode solver are confirmed by experimental data obtained on TFBGs. We show that the refractometric sensitivity varies with the mode order and that the global SPR envelope shift in response to surrounding refractive index (SRI) changes higher than 1e-2 RIU (refractive index unit) can be ~25% bigger than the local SPR mode shift arising from SRI changes limited to 1e-4 RIU. We bring clear evidence that the optimum gold thickness for SPR generation lies in the range between 50 and 70 nm while a cladding diameter decrease from 125 µm to 80 µm enhances the refractometric sensitivity by ~20%. Finally, we demonstrate that the ultimate refractometric sensitivity of cladding modes is ~550 nm/RIU when they are probed by gold-coated TFBGs.

We demonstrate that the experimental strain-optic coefficients for strong guided modes are not consistent with the accepted photoelastic theory. It is shown that for modes with significant nonparaxial components, such as modes guided by strong refractive index differences or in waveguides with dimensions that are much larger than the wavelengths used, the photoelastic theory should be modified to include the effect of the longitudinal components of the electromagnetic fields of the modes. Moreover, we highlight that the strain-optics coefficients depend on the state of polarization of the mode and provide a formula to calculate the necessary corrections.

A standard single-mode optical fiber, coated with low-index polymer (Cytop), then a thin Au sheath, immersed in fluid, isproposedas a structure for optical (bio)chemical sensing. The highest-order EH1m cladding modes are found to couple strongly to long- or short-range surface plasmons on the Au sheath, forming coupled modes that are sensitive to the refractive index of the fluid or to a biochemical adlayer formed on the outer surface of the Au sheath. Interrogation of the modes can be achieved with the help of a tilted grating photoinduced into the core of the fiber. We demonstrate experimentally, in this manner, the excitation of these modes, and their use for bulk sensing.

The high-order cladding modes of conventional single mode fiber come in semi-degenerate pairs corresponding to mostly radially or mostly azimuthally polarized light. Using tilted fiber Bragg gratings to excite these mode families separately, we show how plasmonic coupling to a thin gold coating on the surface of the fiber modifies the effective indices of the modes differently according to polarization and to mode order. In particular, we show the existence of a single "apolarized" grating resonance, with equal effective index for all input polarization states. This special resonance provides direct evidence of the excitation of a surface plasmon on the metal surface but also an absolute wavelength reference that allows for the precise localization of the most sensitive resonances in refractometric and biochemical sensing applications. Two plasmon interrogation methods are proposed, based on wavelength and amplitude measurements. Finally, we use a biotin-streptavidin biomolecular recognition experiment to demonstrate that differential spectral transmission measurements of a fine comb of cladding mode resonances in the vicinity of the apolarized resonance provide the most accurate method to extract information from plasmon-assisted Tilted fiber Bragg gratings, down to pM concentrations and at least 10-5 refractive index changes.