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1. The Indian-French Trishna Mission: Earth Observation in the Thermal Infrared with High Spatio-Temporal Resolution

Author

Benoit Laignel, Isabelle Dadou, Bimal K. Bhattacharya, Mathieu Gouhier, Xavier Briottet, José A. Sobrino, Albert Olioso, Philippe Gamet, Anil Kumar, Frédéric Jacob, S. K. Singh, G. Boulet, M. Irvine, Muddu Sekhar, Ratheesh Ramakrishnan, K. K. Kumar, Gérard Dedieu, Catherine Ottlé, S. Cherchali, J.-L. Roujean, S. Suresh Babu, C. S. Murthy, Olivier Hagolle, Krishna Mohan Buddhiraju, M. R. Pandya, P. V. Raju, Philippe Crebassol, M. V. Shukla, Kaniska Mallick, Jean-Pierre Lagouarde, Laboratoire de recherche en Hydrodynamique, Énergétique et Environnement Atmosphérique (LHEEA), École Centrale de Nantes (ECN)-Centre National de la Recherche Scientifique (CNRS), Indian Space Research Organisation (ISRO), Centre National d'Études Spatiales [Toulouse] (CNES), Space Physics Laboratory, Centre d'études spatiales de la biosphère (CESBIO), Institut de Recherche pour le Développement (IRD)-Université Toulouse III - Paul Sabatier (UT3), Université Fédérale Toulouse Midi-Pyrénées-Université Fédérale Toulouse Midi-Pyrénées-Observatoire Midi-Pyrénées (OMP), Université Fédérale Toulouse Midi-Pyrénées-Centre National d'Études Spatiales [Toulouse] (CNES)-Centre National de la Recherche Scientifique (CNRS), ONERA / DOTA, Université de Toulouse [Toulouse], ONERA-PRES Université de Toulouse, Space technology cell (ISRO, ITT(B)), DYNBIO LEGOS, Laboratoire d'études en Géophysique et océanographie spatiales (LEGOS), Université Fédérale Toulouse Midi-Pyrénées-Université Fédérale Toulouse Midi-Pyrénées-Centre National d'Études Spatiales [Toulouse] (CNES)-Observatoire Midi-Pyrénées (OMP), Université Fédérale Toulouse Midi-Pyrénées-Centre National de la Recherche Scientifique (CNRS)-Institut de Recherche pour le Développement (IRD)-Université Toulouse III - Paul Sabatier (UT3), Université Fédérale Toulouse Midi-Pyrénées-Centre National de la Recherche Scientifique (CNRS), Observatoire de Physique du Globe de Clermont-Ferrand (OPGC), Centre National de la Recherche Scientifique (CNRS)-Institut national des sciences de l'Univers (INSU - CNRS)-Université Blaise Pascal - Clermont-Ferrand 2 (UBP), Groupe de Recherche en Informatique, Image, Automatique et Instrumentation de Caen (GREYC), Université de Caen Normandie (UNICAEN), Normandie Université (NU)-Normandie Université (NU)-École Nationale Supérieure d'Ingénieurs de Caen (ENSICAEN), Normandie Université (NU)-Centre National de la Recherche Scientifique (CNRS), Laboratoire d'étude des Interactions Sol - Agrosystème - Hydrosystème (UMR LISAH), Institut de Recherche pour le Développement (IRD)-Centre international d'études supérieures en sciences agronomiques (Montpellier SupAgro)-Institut de Recherche pour le Développement (IRD [ Madagascar])-Institut national d’études supérieures agronomiques de Montpellier (Montpellier SupAgro)-Institut National de Recherche pour l’Agriculture, l’Alimentation et l’Environnement (INRAE), School of Medicine and Health Sciences [George Washigton University] (SMHS), George Washington University (GW), Morphodynamique Continentale et Côtière (M2C), Centre National de la Recherche Scientifique (CNRS)-Université de Rouen Normandie (UNIROUEN), Normandie Université (NU)-Normandie Université (NU)-Institut national des sciences de l'Univers (INSU - CNRS)-Université de Caen Normandie (UNICAEN), Normandie Université (NU), Institut de Physique Théorique - UMR CNRS 3681 (IPHT), Centre National de la Recherche Scientifique (CNRS)-Université Paris-Saclay-Commissariat à l'énergie atomique et aux énergies alternatives (CEA), Luxembourg Institute of Science and Technology (LIST), National Remote Sensing Centre [Hyderabad] (NRSC), Environnement Méditerranéen et Modélisation des Agro-Hydrosystèmes (EMMAH), Avignon Université (AU)-Institut National de Recherche pour l’Agriculture, l’Alimentation et l’Environnement (INRAE), Laboratoire des Sciences du Climat et de l'Environnement [Gif-sur-Yvette] (LSCE), Université Paris-Saclay-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Centre National de la Recherche Scientifique (CNRS), Groupe d'étude de l'atmosphère météorologique (CNRM-GAME), Institut national des sciences de l'Univers (INSU - CNRS)-Météo France-Centre National de la Recherche Scientifique (CNRS), Indian Institute of Science, Foundation for Innovation and Technology Transfer (FITT), Indian Institute of Technology Delhi (IIT Delhi), Global Change Unit, University of Valencia, Universitat de València (UV), Centre National de la Recherche Scientifique (CNRS)-Institut de Recherche pour le Développement (IRD)-Institut National de Recherche pour l’Agriculture, l’Alimentation et l’Environnement (INRAE)-Université Toulouse III - Paul Sabatier (UT3), Université Fédérale Toulouse Midi-Pyrénées-Université Fédérale Toulouse Midi-Pyrénées-Institut national des sciences de l'Univers (INSU - CNRS)-Observatoire Midi-Pyrénées (OMP), Météo France-Centre National d'Études Spatiales [Toulouse] (CNES)-Université Fédérale Toulouse Midi-Pyrénées-Centre National de la Recherche Scientifique (CNRS)-Institut de Recherche pour le Développement (IRD)-Météo France-Centre National d'Études Spatiales [Toulouse] (CNES)-Centre National de la Recherche Scientifique (CNRS), Météo France-Centre National d'Études Spatiales [Toulouse] (CNES)-Université Fédérale Toulouse Midi-Pyrénées-Centre National de la Recherche Scientifique (CNRS)-Institut de Recherche pour le Développement (IRD)-Météo France-Centre National d'Études Spatiales [Toulouse] (CNES)-Centre National de la Recherche Scientifique (CNRS)-Institut de Recherche pour le Développement (IRD)-Centre National de la Recherche Scientifique (CNRS)-Institut de Recherche pour le Développement (IRD)-Université Toulouse III - Paul Sabatier (UT3), Météo France-Centre National d'Études Spatiales [Toulouse] (CNES)-Université Fédérale Toulouse Midi-Pyrénées-Centre National de la Recherche Scientifique (CNRS)-Institut de Recherche pour le Développement (IRD)-Météo France-Centre National d'Études Spatiales [Toulouse] (CNES)-Centre National de la Recherche Scientifique (CNRS)-Institut de Recherche pour le Développement (IRD)-Centre National de la Recherche Scientifique (CNRS), Institut de Recherche pour le Développement (IRD)-Institut National de la Recherche Agronomique (INRA)-Centre international d'études supérieures en sciences agronomiques (Montpellier SupAgro)-Institut national d’études supérieures agronomiques de Montpellier (Montpellier SupAgro), Institut national d'enseignement supérieur pour l'agriculture, l'alimentation et l'environnement (Institut Agro)-Institut national d'enseignement supérieur pour l'agriculture, l'alimentation et l'environnement (Institut Agro), The George Washington University (GW), Normandie Université (NU)-Normandie Université (NU)-Institut national des sciences de l'Univers (INSU - CNRS)-Université de Rouen Normandie (UNIROUEN), Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Université Paris-Saclay-Centre National de la Recherche Scientifique (CNRS), Institut national des sciences de l'Univers (INSU - CNRS)-Université Paris-Saclay-Centre National de la Recherche Scientifique (CNRS)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ), Modélisation des Surfaces et Interfaces Continentales (MOSAIC), Institut national des sciences de l'Univers (INSU - CNRS)-Université Paris-Saclay-Centre National de la Recherche Scientifique (CNRS)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Institut national des sciences de l'Univers (INSU - CNRS)-Université Paris-Saclay-Centre National de la Recherche Scientifique (CNRS)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ), Institute of Electrical and Electronics Engineers (IEEE). USA., Université de Toulouse (UT)-Université de Toulouse (UT)-Institut national des sciences de l'Univers (INSU - CNRS)-Observatoire Midi-Pyrénées (OMP), Université de Toulouse (UT)-Université de Toulouse (UT)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National d'Études Spatiales [Toulouse] (CNES)-Centre National de la Recherche Scientifique (CNRS)-Météo-France -Institut national des sciences de l'Univers (INSU - CNRS)-Centre National d'Études Spatiales [Toulouse] (CNES)-Centre National de la Recherche Scientifique (CNRS)-Météo-France -Centre National de la Recherche Scientifique (CNRS)-Institut National de Recherche pour l’Agriculture, l’Alimentation et l’Environnement (INRAE), Université de Toulouse (UT)-Université de Toulouse (UT)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National d'Études Spatiales [Toulouse] (CNES)-Centre National de la Recherche Scientifique (CNRS)-Météo-France -Institut de Recherche pour le Développement (IRD)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National d'Études Spatiales [Toulouse] (CNES)-Centre National de la Recherche Scientifique (CNRS)-Météo-France -Centre National de la Recherche Scientifique (CNRS)-Institut de Recherche pour le Développement (IRD)-Université Toulouse III - Paul Sabatier (UT3), Université de Toulouse (UT)-Université de Toulouse (UT)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National d'Études Spatiales [Toulouse] (CNES)-Centre National de la Recherche Scientifique (CNRS)-Météo-France -Institut de Recherche pour le Développement (IRD)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National d'Études Spatiales [Toulouse] (CNES)-Centre National de la Recherche Scientifique (CNRS)-Météo-France -Centre National de la Recherche Scientifique (CNRS), Université Blaise Pascal - Clermont-Ferrand 2 (UBP)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS), Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Institut national des sciences de l'Univers (INSU - CNRS)-Université Paris-Saclay-Centre National de la Recherche Scientifique (CNRS), Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Institut national des sciences de l'Univers (INSU - CNRS)-Université Paris-Saclay-Centre National de la Recherche Scientifique (CNRS)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Institut national des sciences de l'Univers (INSU - CNRS)-Université Paris-Saclay-Centre National de la Recherche Scientifique (CNRS), Centre national de recherches météorologiques (CNRM), Institut national des sciences de l'Univers (INSU - CNRS)-Observatoire Midi-Pyrénées (OMP), Université de Toulouse (UT)-Université de Toulouse (UT)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National d'Études Spatiales [Toulouse] (CNES)-Centre National de la Recherche Scientifique (CNRS)-Météo-France -Institut de Recherche pour le Développement (IRD)-Université Toulouse III - Paul Sabatier (UT3), Université de Toulouse (UT)-Université de Toulouse (UT)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National d'Études Spatiales [Toulouse] (CNES)-Centre National de la Recherche Scientifique (CNRS)-Météo-France -Centre National de la Recherche Scientifique (CNRS), Interactions Sol Plante Atmosphère (ISPA), Ecole Nationale Supérieure des Sciences Agronomiques de Bordeaux-Aquitaine (Bordeaux Sciences Agro)-Institut National de la Recherche Agronomique (INRA), ISRO, Centre National d’Etudes Spatiales, Space Phys Lab, Vikram Sarabhai Space Ctr, Institut de Recherche pour le Développement (IRD [Réunion]), Université de Toulouse, Institut de Recherche pour le Développement (IRD), Université de Rouen Normandie (UNIROUEN), and Commissariat à l'énergie atomique et aux énergies alternatives (CEA)

Subjects
Earth observation, 010504 meteorology & atmospheric sciences, INFRAROUGE, CLIMATE CHANGE, WATER MANAGEMENT, 0211 other engineering and technologies, Climate change, 02 engineering and technology, 01 natural sciences, [SDV.BV]Life Sciences [q-bio]/Vegetal Biology, WATER STRESS, Water cycle, Thermal infrared, Baseline (configuration management), SATELLITE, 021101 geological & geomatics engineering, 0105 earth and related environmental sciences, Remote sensing, THERMAL, [SDE.IE]Environmental Sciences/Environmental Engineering, INFRARED, Spectral bands, MISSION SPATIALE, Natural resource, 13. Climate action, Temporal resolution, [SDE]Environmental Sciences, Environmental science, Satellite
Abstract

International audience; The monitoring of the water cycle at the Earth surface which tightly interacts with the climate change processes as well as a number of practical applications (agriculture, soil and water quality assessment, irrigation and water resource management, etc...) requires surface temperature measurements at local scale. Such is the goal of the Indian-French high spatio-temporal TRISHNA mission (Thermal infraRed Imaging Satellite for High-resolution Natural resource Assessment). The scientific objectives of the mission and research work conducted to consolidate the mission specifications are presented. Progress in modelling of surface fluxes is then discussed. The main specifications of the mission such as the revisit, the spatial resolution, the overpass time, the spectral bands and the orbit are analyzed and justified. The resulting baseline of the mission is given.

Published
2018

2. A European aerosol phenomenology – 6: scattering properties of atmospheric aerosol particles from 28 ACTRIS sites

Author

M. Pandolfi, L. Alados-Arboledas, A. Alastuey, M. Andrade, C. Angelov, B. Artiñano, J. Backman, U. Baltensperger, P. Bonasoni, N. Bukowiecki, M. Collaud Coen, S. Conil, E. Coz, V. Crenn, V. Dudoitis, M. Ealo, K. Eleftheriadis, O. Favez, P. Fetfatzis, M. Fiebig, H. Flentje, P. Ginot, M. Gysel, B. Henzing, A. Hoffer, A. Holubova Smejkalova, I. Kalapov, N. Kalivitis, G. Kouvarakis, A. Kristensson, M. Kulmala, H. Lihavainen, C. Lunder, K. Luoma, H. Lyamani, A. Marinoni, N. Mihalopoulos, M. Moerman, J. Nicolas, C. O'Dowd, T. Petäjä, J.-E. Petit, J. M. Pichon, N. Prokopciuk, J.-P. Putaud, S. Rodríguez, J. Sciare, K. Sellegri, E. Swietlicki, G. Titos, T. Tuch, P. Tunved, V. Ulevicius, A. Vaishya, M. Vana, A. Virkkula, S. Vratolis, E. Weingartner, A. Wiedensohler, P. Laj, Institute of Environmental Assessment and Water Research (IDAEA), Consejo Superior de Investigaciones Científicas [Madrid] (CSIC), Universidad de Granada = University of Granada (UGR), Universidad Mayor de San Andrés (UMSA), Bulgarian Academy of Sciences (BAS), Centro de Investigaciones Energéticas Medioambientales y Tecnológicas [Madrid] (CIEMAT), Helsingin yliopisto = Helsingfors universitet = University of Helsinki, Finnish Meteorological Institute (FMI), Laboratory of Atmospheric Chemistry [Paul Scherrer Institute] (LAC), Paul Scherrer Institute (PSI), CNR Institute of Atmospheric Sciences and Climate (ISAC), National Research Council of Italy | Consiglio Nazionale delle Ricerche (CNR), Federal Office of Meteorology and Climatology MeteoSwiss, Observatoire Pérenne de l'Environnement, Agence Nationale pour la Gestion des Déchets Radioactifs (ANDRA), Laboratoire des Sciences du Climat et de l'Environnement [Gif-sur-Yvette] (LSCE), Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Institut national des sciences de l'Univers (INSU - CNRS)-Université Paris-Saclay-Centre National de la Recherche Scientifique (CNRS), ADDAIR Sté (France), Center for Physical Sciences and Technology [Vilnius] (FTMC), National Centre for Scientific Research Demokritos, Institut National de l'Environnement Industriel et des Risques (INERIS), Norwegian Institute for Air Research (NILU), Institut des Géosciences de l’Environnement (IGE), Institut de Recherche pour le Développement (IRD)-Institut polytechnique de Grenoble - Grenoble Institute of Technology (Grenoble INP )-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS)-Université Grenoble Alpes [2016-2019] (UGA [2016-2019]), The Netherlands Organisation for Applied Scientific Research (TNO), University of Crete [Heraklion] (UOC), National Observatory of Athens (NOA), Lund University [Lund], Laboratoire de Météorologie Physique (LaMP), Institut national des sciences de l'Univers (INSU - CNRS)-Université Clermont Auvergne [2017-2020] (UCA [2017-2020])-Centre National de la Recherche Scientifique (CNRS), Chimie Atmosphérique Expérimentale (CAE), Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Institut national des sciences de l'Univers (INSU - CNRS)-Université Paris-Saclay-Centre National de la Recherche Scientifique (CNRS)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Institut national des sciences de l'Univers (INSU - CNRS)-Université Paris-Saclay-Centre National de la Recherche Scientifique (CNRS), JRC Institute for Environment and Sustainability (IES), European Commission - Joint Research Centre [Ispra] (JRC), Leibniz Institute for Tropospheric Research (TROPOS), Vikram Sarabhai Space Ctr, European Commission, University of Granada [Granada], University of Helsinki, Consiglio Nazionale delle Ricerche (CNR), Institut national des sciences de l'Univers (INSU - CNRS)-Université Paris-Saclay-Centre National de la Recherche Scientifique (CNRS)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ), Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS)-Institut polytechnique de Grenoble - Grenoble Institute of Technology (Grenoble INP )-Institut de Recherche pour le Développement (IRD)-Université Grenoble Alpes [2016-2019] (UGA [2016-2019]), Institut national des sciences de l'Univers (INSU - CNRS)-Université Paris-Saclay-Centre National de la Recherche Scientifique (CNRS)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Institut national des sciences de l'Univers (INSU - CNRS)-Université Paris-Saclay-Centre National de la Recherche Scientifique (CNRS)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ), INAR Physics, and Department of Physics

Subjects
Atmospheric Science, Angstrom exponent, 010504 meteorology & atmospheric sciences, Mass concentrations, Seasonal variation, NUMBER CONCENTRATIONS, Aerosol sources, radiative properties, 010501 environmental sciences, black carbon, western mediterranean basin, 01 natural sciences, lcsh:Chemistry, free troposphere, saharan dust, Factorization, Physics::Atmospheric and Oceanic Physics, Positive matrix, Particle size, Particulates, lcsh:QC1-999, LIGHT-SCATTERING, optical-properties, in-situ, Climatology, [SDE]Environmental Sciences, MEDITERRANEAN BASIN, Phenomenology, Environment & Sustainability, Particle light scattering, Atmospheric aerosol, Scattering properties, Aerosol particle, Backscatter, Urbanisation, Mineral dust, Environment, 114 Physical sciences, Aerosol formation, medicine, Aerosol, 1172 Environmental sciences, 0105 earth and related environmental sciences, particulate matter, Scattering, Aerosol properties, integrating nephelometer, Seasonality, medicine.disease, Concentration (composition), lcsh:QD1-999, Arctic, 13. Climate action, regional background sites, Environmental science, Particulate matter, Aerosol property, lcsh:Physics
Abstract

This paper presents the light-scattering properties of atmospheric aerosol particles measured over the past decade at 28 ACTRIS observatories, which are located mainly in Europe. The data include particle light scattering (σsp) and hemispheric backscattering (σbsp) coefficients, scattering Ångström exponent (SAE), backscatter fraction (BF) and asymmetry parameter (g). An increasing gradient of σsp is observed when moving from remote environments (arctic/mountain) to regional and to urban environments. At a regional level in Europe, σsp also increases when moving from Nordic and Baltic countries and from western Europe to central/eastern Europe, whereas no clear spatial gradient is observed for other station environments. The SAE does not show a clear gradient as a function of the placement of the station. However, a west-to-east-increasing gradient is observed for both regional and mountain placements, suggesting a lower fraction of fine-mode particle in western/south-western Europe compared to central and eastern Europe, where the fine-mode particles dominate the scattering. The g does not show any clear gradient by station placement or geographical location reflecting the complex relationship of this parameter with the physical properties of the aerosol particles. Both the station placement and the geographical location are important factors affecting the intraannual variability. At mountain sites, higher σsp and SAE values are measured in the summer due to the enhanced boundary layer influence and/or new particle-formation episodes. Conversely, the lower horizontal and vertical dispersion during winter leads to higher σsp values at all low-altitude sites in central and eastern Europe compared to summer. These sites also show SAE maxima in the summer (with corresponding g minima). At all sites, both SAE and g show a strong variation with aerosol particle loading. The lowest values of g are always observed together with low σsp values, indicating a larger contribution from particles in the smaller accumulation mode. During periods of high σsp values, the variation of g is less pronounced, whereas the SAE increases or decreases, suggesting changes mostly in the coarse aerosol particle mode rather than in the fine mode. Statistically significant decreasing trends of σsp are observed at 5 out of the 13 stations included in the trend analyses. The total reductions of σsp are consistent with those reported for PM2.5 and PM10 mass concentrations over similar periods across Europe. © Author(s) 2018., Acknowledgements. This project has received funding from the European Union’s Horizon 2020 research and innovation programme under grant agreement no. 654109, ACTRIS (project no. 262254), ACTRIS-PPP (project no. 739530). We thank the International Foundation High Altitude Research Stations JFJ (Jungfraujoch) and Gornergrat (HFSJG), which made it possible to carry out the experiments at the High Altitude Research JFJ Station and the support of MeteoSwiss within the Swiss programme of the Global Atmosphere Watch (GAW) of the WMO. The MAD (Madrid) station is co-financed by the PROACLIM (CGL2014-52877-R) project. The SMR (Hyytiälä) station acknowledges BACCHUS (project no. 603445), CRAICC (project no. 26060) and the Academy of Finland (project no. 3073314). The UGR (Granada) station is co-financed by the Spanish Ministry of Economy and Competitiveness through project CGL2016-81092-R. Measurements at MSY (Montseny) and MSA (Montsec) stations were supported by the MINECO (Spanish Ministry of Economy, Industry and Competitiveness) and FEDER funds under the PRISMA project (CGL2012-39623-C02/00) and under the HOUSE project (CGL2016-78594-R), by the MAGRAMA (Spanish Ministry of Agriculture, Food and Environment) and by the Generalitat de Catalunya (AGAUR 2014 SGR33, AGAUR 2017 SGR41 and the DGQA). Measurements at IZO (Izaña) were supported by the AEROATLAN project (CGL2015-17 66229-P), co-funded by the Ministry of Economy and Competitiveness of Spain and the European Regional Development Fund. Station KOS (Košetice) is supported by the Ministry of Education, Youth and Sports of the Czech Republic within the project to support the national research infrastructure ACTRIS – participation of the Czech Republic (ACTRIS-CZ – LM2015037). Measurements at PUY (Puy de Dôme) were partly supported by CNRS-INSU, University Clermont-Auvergne, OPGC and the french CLAP programme. The PAL (Pallas) station acknowledges KONE Foundation, Academy of Finland (project no. 269095 and no. 296302). CHC (Mt Chacaltaya) station received support from Institut de Recherche pour le Développement (IRD) under both Jeune Equipe programme attributed to LFA and support to ACTRIS-FR programme. CHC received grants from Labex OSUG@2020 (Investissements d’avenir – ANR10 LABX56). Marco Pandolfi is funded by a Ramón y Cajal Fellowship (RYC-2013-14036) awarded by the Spanish Ministry of Economy and Competitiveness. The authors would like to express their gratitude to David Carslaw and Karl Ropkins for providing the OpenAir software used in this paper (Carslaw and Ropkins, 2012; Carslaw, 2012). We also thank the co-editor Andreas Petzold and two anonymous reviewers for their constructive comments.

Published
2018

3. Exciting Wide NMR Spectra of Static Solid Samples with Weak Radiofrequency Fields

Author

Diego Carnevale, Geoffrey Bodenhausen, Srinivas Chinthalapalli, Neuchâtel Platform of Analytical Chemistry (NPAC), Université de Neuchâtel (UNINE), Institut des Sciences et Ingénierie Chimiques (ISIC), Ecole Polytechnique Fédérale de Lausanne (EPFL), Vikram Sarabhai Space Ctr, Structure et Dynamique des Biomolécules (LBM-E3), Laboratoire des biomolécules (LBM UMR 7203), Institut de Chimie du CNRS (INC)-Centre National de la Recherche Scientifique (CNRS)-Institut National de la Santé et de la Recherche Médicale (INSERM)-Département de Chimie - ENS Paris, École normale supérieure - Paris (ENS Paris), Université Paris sciences et lettres (PSL)-Université Paris sciences et lettres (PSL)-École normale supérieure - Paris (ENS Paris), Université Paris sciences et lettres (PSL)-Université Paris sciences et lettres (PSL)-Université Pierre et Marie Curie - Paris 6 (UPMC)-Institut de Chimie du CNRS (INC)-Centre National de la Recherche Scientifique (CNRS)-Institut National de la Santé et de la Recherche Médicale (INSERM)-Département de Chimie - ENS Paris, Université Paris sciences et lettres (PSL)-Université Paris sciences et lettres (PSL)-Université Pierre et Marie Curie - Paris 6 (UPMC), Université Pierre et Marie Curie - Paris 6 (UPMC)-Département de Chimie - ENS Paris, École normale supérieure - Paris (ENS-PSL), Université Paris sciences et lettres (PSL)-Université Paris sciences et lettres (PSL)-École normale supérieure - Paris (ENS-PSL), Université Paris sciences et lettres (PSL)-Université Paris sciences et lettres (PSL)-Institut National de la Santé et de la Recherche Médicale (INSERM)-Institut de Chimie du CNRS (INC)-Centre National de la Recherche Scientifique (CNRS)-Université Pierre et Marie Curie - Paris 6 (UPMC)-Département de Chimie - ENS Paris, and Université Paris sciences et lettres (PSL)-Université Paris sciences et lettres (PSL)-Institut National de la Santé et de la Recherche Médicale (INSERM)-Institut de Chimie du CNRS (INC)-Centre National de la Recherche Scientifique (CNRS)

Subjects
Analytical chemistry, 02 engineering and technology, dipolar echoes, 010402 general chemistry, 01 natural sciences, Molecular physics, Spectral line, Homonuclear molecule, NMR spectroscopy, [CHIM]Chemical Sciences, Physical and Theoretical Chemistry, Anisotropy, hydration water, solid echoes, dipolar interactions, quadrupolar interactions, Chemistry, Chemical shift, 021001 nanoscience & nanotechnology, 0104 chemical sciences, NMR spectra database, quadrupolar echoes, solid-state NMR of static samples, Dipole, DANTE, Crystallite, 0210 nano-technology, Excitation
Abstract

Trains of short pulses in the manner of ‘delays alternating with nutations for tailored excitation’ (DANTE) have been applied to the Pake patterns of protons of water molecules trapped in a static powdered sample of barium chlorate monohydrate. The spin dynamics in the course of such experiments have been investigated by means of numerical simulations and compared with the ideal refocusing that can be achieved under magic-angle spinning (MAS). Solid echoes yield essentially undistorted lineshapes, in contrast to direct excitation without refocusing that leads to severe dispersions of the phases because of inhomogeneous interactions such as homonuclear dipolar couplings and anisotropic chemical shifts. The selectivity of DANTE sequences allows one to access ‘slices’ of the Pake pattern that can be related to particular crystallite orientations. Single-crystal spectra can therefore be extracted from powder spectra. A similar behavior is expected for both dipolar and quadrupolar echoes.

Published
2017

4. WRF/ARPEGE-CLIMAT simulated climate trends over West Africa

Author

S. Sijikumar, Pascal Roucou, S. Tyteca, Nicolas Vigaud, Bernard Fontaine, Centre de Recherches de Climatologie ( CRC ), Université de Bourgogne ( UB ) -Centre National de la Recherche Scientifique ( CNRS ), Space Physics Laboratory, Indian Space Research Organisation ( ISRO ), Groupe d'étude de l'atmosphère météorologique ( CNRM-GAME ), Institut national des sciences de l'Univers ( INSU - CNRS ) -Météo France-Centre National de la Recherche Scientifique ( CNRS ), ANR-06-VULN-0017,RESSAC,Vulnérabilité des ressources en eau superficielle au Sahel aux évolutions anthropiques et climatiques à moyen term ( 2006 ), Centre de Recherches de Climatologie (CRC), Université de Bourgogne (UB)-Centre National de la Recherche Scientifique (CNRS), Space Phys Lab, Vikram Sarabhai Space Ctr, Groupe d'étude de l'atmosphère météorologique (CNRM-GAME), Institut national des sciences de l'Univers (INSU - CNRS)-Météo France-Centre National de la Recherche Scientifique (CNRS), Indian Space Research Organisation (ISRO), and ANR-06-VULN-0017,RESSAC,Vulnérabilité des ressources en eau superficielle au Sahel aux évolutions anthropiques et climatiques à moyen term(2006)

Subjects
Atmospheric Science, 010504 meteorology & atmospheric sciences, [SDE.MCG]Environmental Sciences/Global Changes, WRF, 0207 environmental engineering, Regional model, Climate change, 02 engineering and technology, Monsoon, 01 natural sciences, West Africa, 020701 environmental engineering, 0105 earth and related environmental sciences, Tropical wave, Moisture advection, African easterly jet, [ SDE.MCG ] Environmental Sciences/Global Changes, 13. Climate action, [SDU.STU.CL]Sciences of the Universe [physics]/Earth Sciences/Climatology, Climatology, Weather Research and Forecasting Model, Environmental science, Climate model, [ SDU.STU.CL ] Sciences of the Universe [physics]/Earth Sciences/Climatology, Downscaling
Abstract

20 pages; International audience; The Weather Regional Forecast (WRF) model is used in this study to downscale low-resolution data over West Africa. First, the performance of the regional model is estimated through contemporary period experiments (1981-1990) forced by ARPEGE-CLIMAT GCM output (ARPEGE) and ERA-40 re-analyses. Key features of the West African monsoon circulation are reasonably well represented. WRF atmospheric dynamics and summer rainfall compare better to observations than ARPEGE forcing data. WRF simulated moisture transport over West Africa is also consistent in both structure and variability with re-analyses, emphasizing the substantial role played by the West African Monsoon (WAM) and African Easterly Jet (AEJ) flows. The statistical significance of potential climate changes for the A2 scenario between 2032 and 2041 is enhanced in the downscaling from ARPEGE by the regional experiments, with substantial rainfall increases over the Guinea Gulf and eastern Sahel. Future scenario WRF simulations are characterized by higher temperatures over the eastern Tropical Atlantic suggesting more evaporation available locally. This leads to increased moisture advection towards eastern regions of the Guinea Gulf where rainfall is enhanced through a strengthened WAM flow, supporting surface moisture convergence over West Africa. Warmer conditions over both the Mediterranean region and northeastern Sahel could also participate in enhancing moisture transport within the AEJ. The strengthening of the thermal gradient between the Sahara and Guinean regions, particularly pronounced north of 10A degrees N, would support an intensification of the AEJ northwards, given the dependance of the jet to the position/intensity of the meridional gradient. In turn, mid-tropospheric moisture divergence tends to be favored within the AEJ region supporting southwards deflection of moist air and contributing to deep moist convection over the Sahel where late summer rainfall regimes are sustained in the context of the A2 scenario regional projections. In conclusion, WRF proved to be a valuable and efficient tool to help downscaling GCM projections over West Africa, and thus assessing issues such as water resources vulnerability locally.

Published
2009

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