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In this contribution we report on further investigations of the recently-evaluated Constant-Fraction Time-over-Threshold (CF-ToT) method for neutron/gamma-ray pulse shape discrimination (PSD). The superiority of the CF-ToT PSD method over the constant-threshold (CT-ToT) method was previously demonstrated, down to low neutron energy thresholds of 100 keVee. Here, we report on a quantitative comparison between the traditionally used Charge Comparison (CC) method and the CF-ToT method using a stilbene scintillator coupled to a silicon photomultiplier, implementing an offline analysis of recorded fast-neutron and gamma-ray waveforms. An optimization of the constant fraction value indicates that a 20%-fraction yields the optimum figure-of-merit (FOM) and gamma-ray peak-to-valley (P/V) ratio. The results obtained for a particle energy threshold of 100 keVee show that the FOM and P/V values achieved with the CF-ToT method are superior to those obtained using the standard CC method. In addition, a first electronic implementation of the CF-ToT method was performed using simple circuitry suitable for multichannel architecture. Initial results obtained with this circuit prototype are presented., Comment: 10 pages, 8 figures. To be submitted to JINST

The use of Time-over-Threshold (TOT) for the discrimination between fast neutrons and gamma-rays is advantageous when large number of detection channels are required due to the simplicity of its implementation. However, the results obtained using the standard, Constant Threshold TOT (CT-TOT) are usually inferior to those obtained using other pulse shape discrimination (PSD) methods, such as Charge Comparison or Zero-Crossing approaches, especially for low amplitude neutron/gamma-ray pulses. We evaluate another TOT approach for fast neutron/gamma-ray PSD using Constant-Fraction Time-over-Threshold (CF-TOT) pulse shape analysis. The CT-TOT and CF-TOT methods were compared quantitatively using digitized waveforms from a liquid scintillator coupled to a photomultiplier tube as well as from a stilbene scintillator coupled to a photomultiplier tube and a silicon photomultiplier. The quality of CF-TOT neutron/gamma-ray discrimination was evaluated using Receiver Operator Characteristics curves and the results obtained with this approach were compared to the that of the standard CT-TOT method. The CF-TOT PSD method results in > 99.9% rejection of gamma-rays with > 80% neutron acceptance, much better than CT-TOT., Comment: Accepted for publication in JINST

In bubble-assisted Liquid HoleMultipliers(LHM), developed for noble-liquid radiation detectors, the stability of the bubble and the electro-mechanical properties of the liquid-to-gas interface play a dominant role in the detector performance. A model is proposed to evaluate the static equilibrium configurations of a bubble sustained underneath a perforated electrode immersed in a liquid. For the first time bubbles were optically observed in LAr; their properties were studied in contact with different material surfaces. This permitted investigating the bubble-electrodynamics via numerical simulations; it was shown that the electric field acts as an additional pressure term on the bubble meniscus. The predictions for the liquid-to-gas interface were successfully validated using X-ray micro-CT in water and in silicone oil at STP. The proposed model and the results of this study are an important milestone towards understanding and optimizing the parameters of LHM-based noble-liquid detectors., Comment: 25 pages, 15 figures

The bubble-assisted Liquid Hole Multiplier (LHM) is a novel concept for the combined detection of ionization electrons and scintillation photons in noble-liquid time projection chambers. It consists of a perforated electrode immersed in the noble liquid, with heating wires generating a stable bubble underneath. Radiation-inducted ionization electrons in the liquid drift into the electrode's holes and cross the liquid-vapor interface into the bubble where they induce electroluminescence (EL). The top surface of the electrode is optionally coated with a CsI photocathode; radiation-induced UV-scintillation photons extract photoelectrons that induce EL in a similar way. EL-photons recorded with an array of photosensors, e.g. SiPMs, provide event localization. We present the basic principles of the LHM and summarize the results obtained in LXe and LAr., Comment: presented at LIDINE 2019; to be published in JINST

We present for the first time, discharge-free operation at cryogenic conditions of a Resistive-Plate WELL (RPWELL) detector. It is a single-sided Thick Gaseous Electron Multiplier (THGEM) coupled to a readout anode via a plate of high bulk resistivity. The results of single- and double-stage RPWELL detectors operated in stable conditions in Ne/5$\%$CH$_{4}$ at 163 K are summarized. The RPWELL comprised a ferric-based (Fe$^{3+}$) ceramic composite ("Fe-ceramic") as the resistive plate, of volume resistivity $\sim$$10^{11}$ $\Omega$$\cdot$cm at this temperature. Gains of $\sim$$10^{4}$ and $\sim$$10^{5}$ were reached with the single-stage RPWELL, with 6 keV X-rays and single UV-photons, respectively. The double-stage detector, a THGEM followed by the RPWELL, reached gains $\sim$$10^{5}$ and $\sim$$10^{6}$ with X-rays and single UV-photons, respectively. The results were obtained with and without a CsI photocathode on the first multiplying element. Potential applications at these cryogenic conditions are discussed., Comment: 14 pages, 8 figures, to be submitted to JINST

First imaging results in liquid xenon of a Liquid Hole Multiplier (LHM) coupled to a Quad-Silicon Photomultiplier (SiPM) array are presented. Ionization electrons deposited in the noble liquid by 5.5 MeV alpha particles, are collected into the holes of a Thick Gas Electron Multiplier (THGEM) electrode having a xenon gas bubble trapped underneath. They drift through the liquid-gas interface, inducing electroluminescence within the bubble. The resulting photons are detected with a Hamamatsu VUV4 quad-SiPM array - providing the deposited energy with a charge-only RMS resolution of 6.6%. The image reconstruction resolution was estimated to be ~200 um (RMS).

We report on recent advances in the operation of bubble-assisted Liquid Hole Multipliers (LHM). By confining a vapor bubble under or adjacent to a perforated electrode immersed in liquid xenon, we could record both radiation-induced ionization electrons and primary scintillation photons in the noble liquid. Four types of LHM electrodes were investigated: a THGEM, standard double-conical GEM, 50 $\mu$m-thick single-conical GEM (SC-GEM) and 125 $\mu$m-thick SC-GEM - all coated with CsI photocathodes. The 125 $\mu$m-thick SC-GEM provided the highest electroluminescence (EL) yields, up to ~400 photons per electron over 4$\pi$ with an RMS pulse-height resolution reaching 5.5% for events comprising ~7000 primary electrons. Applying a high transfer field across the bubble, the EL yield was further increased by a factor of ~5. The feasibility of a vertical-mode LHM, with the bubble confined between two vertical electrodes, and the operation of a two-stage LHM configuration were demonstrated for the first time. We combine electrostatic simulations with observed signals to draw conclusions regarding the location of the liquid-gas interface and suggest an explanation for the observed differences in EL yield between the investigated electrodes., Comment: 27 pages, 22 figures. Submitted to JINST

Gamma-ray and fast-neutron imaging was performed with a novel liquid xenon (LXe) scintillation detector read out by a Gaseous Photomultiplier (GPM). The 100 mm diameter detector prototype comprised a capillary-filled LXe converter/scintillator, coupled to a triple-THGEM imaging-GPM, with its first electrode coated by a CsI UV-photocathode, operated in Ne/5%CH4 cryogenic temperatures. Radiation localization in 2D was derived from scintillation-induced photoelectron avalanches, measured on the GPM's segmented anode. The localization properties of Co-60 gamma-rays and a mixed fast-neutron/gamma-ray field from an AmBe neutron source were derived from irradiation of a Pb edge absorber. Spatial resolutions of 12+/-2 mm and 10+/-2 mm (FWHM) were reached with Co-60 and AmBe sources, respectively. The experimental results are in good agreement with GEANT4 simulations. The calculated ultimate expected resolutions for our application-relevant 4.4 and 15.1 MeV gamma-rays and 1-15 MeV neutrons are 2-4 mm and ~2 mm (FWHM), respectively. These results indicate the potential applicability of the new detector concept to Fast-Neutron Resonance Radiography (FNRR) and Dual-Discrete-Energy Gamma Radiography (DDEGR) of large objects., Comment: 27 pages, 17 figures. Submitted to JINST

A novel method utilizing Fast Neutron Resonance Transmission Radiography is proposed for rapid, non-destructive and quantitative determination of the weight fractions of oil and water in cores taken from subterranean or underwater geological formations. Its ability to distinguish water from oil stems from the unambiguously-specific energy-dependence of the neutron cross-sections for the principal elemental constituents. Furthermore, the fluid weight fractions permit determining core porosity and oil and water saturations. In this article we show results of experimental determination of oil and water weight fractions in 10 cm thick samples of Berea Sandstone and Indiana Limestone formations, followed by calculation of their porosity and fluid saturations. The technique may ultimately permit rapid, accurate and non-destructive evaluation of relevant petro-physical properties in thick intact cores. It is suitable for all types of formations including tight shales, clays and oil sands., Comment: 11 pages, 7 figures. arXiv admin note: text overlap with arXiv:1602.06533

The bubble-assisted Liquid Hole-Multiplier (LHM) is a recently-introduced detection concept for noble-liquid time projection chambers. In this "local dual-phase" detection element, a gas bubble is supported underneath a perforated electrode (e.g., Thick Gas Electron Multiplier - THGEM, or Gas Electron Multiplier - GEM). Electrons drifting through the holes induce large electroluminescence signals as they pass into the bubble. In this work we report on recent results of THGEM and GEM electrodes coated with cesium iodide and immersed in liquid xenon, allowing - for the first time - the detection of primary VUV scintillation photons in addition to ionization electrons using LHMs., Comment: Presented at the 2016 Vienna Conference on Instrumentation. Submitted to the conference proceedings in NIM A

A novel method based on Fast Neutron Resonance Transmission Radiography is proposed for non-destructive, quantitative determination of the weight percentages of oil and water in cores taken from subterranean or underwater geological formations. The ability of the method to distinguish water from oil stems from the unambiguously-specific energy dependence of the neutron cross-sections for the principal elemental constituents. Monte-Carlo simulations and initial results of experimental investigations indicate that the technique may provide a rapid, accurate and non-destructive method for quantitative evaluation of core fluids in thick intact cores, including those of tight shales for which the use of conventional core analytical approaches appears to be questionable., Comment: 16 pages, 10 figures, patent pending

Bubble formation in liquid xenon underneath a Thick Gaseous Electron Multiplier (THGEM) electrode immersed in liquid xenon was observed with a CCD camera. With voltage across the THGEM, the appearance of bubbles was correlated with that of electroluminescence signals induced by ionization electrons from alpha-particle tracks. This confirms recent indirect evidence that the observed photons are due to electroluminescence within a xenon vapor layer trapped under the electrode. The bubbles seem to emerge spontaneously due to heat flow from 300K into the liquid, or in a controlled manner, by locally boiling the liquid with resistive wires. Controlled bubble formation resulted in energy resolution of {\sigma}/E~7.5% for ~6,000 ionization electrons. The phenomenon could pave ways towards the conception of large-volume 'local dual-phase' noble-liquid TPCs., Comment: Submitted to JINST

We discuss recent advances in the development of cryogenic gaseous photomultipliers (GPM), for possible use in dark matter and other rare-event searches using noble-liquid targets. We present results from a 10 cm diameter GPM coupled to a dual-phase liquid xenon (LXe) TPC, demonstrating - for the first time - the feasibility of recording both primary ("S1") and secondary ("S2") scintillation signals. The detector comprised a triple Thick Gas Electron Multiplier (THGEM) structure with cesium iodide photocathode on the first element; it was shown to operate stably at 180 K with gains above 10^5, providing high single-photon detection efficiency even in the presence of large alpha particle-induced S2 signals comprising thousands of photoelectrons. S1 scintillation signals were recorded with a time resolution of 1.2 ns (RMS). The energy resolution ({\sigma}/E) for S2 electroluminescence of 5.5 MeV alpha particles was ~9%, which is comparable to that obtained in the XENON100 TPC with PMTs. The results are discussed within the context of potential GPM deployment in future multi-ton noble-liquid detectors., Comment: Submitted to JINST

In this work we discuss the mechanism behind the large electroluminescence signals observed at relatively low electric fields in the holes of a Thick Gas Electron Multiplier (THGEM) electrode immersed in liquid xenon. We present strong evidence that the scintillation light is generated in xenon bubbles trapped below the THGEM holes. The process is shown to be remarkably stable over months of operation, providing - under specific thermodynamic conditions - energy resolution similar to that of present dual-phase liquid xenon experiments. The observed mechanism may serve as the basis for the development of Liquid Hole Multipliers (LHMs), capable of producing local charge-induced electroluminescence signals in large-volume single-phase noble-liquid detectors for dark matter and neutrino physics experiments., Comment: Submitted to JINST

Recently, a new detector concept, for combined imaging and spectroscopy of fast-neutrons and gamma was presented. It encompasses a liquid-xenon (LXe) converter-scintillator coupled to a UV-sensitive gaseous Thick Gas Electron Multiplier (THGEM)-based imaging photomultiplier (GPM). In this work we present and discuss the results of a systematic computer-simulation study aiming at optimizing the type and performance of LXe converter. We have evaluated the detector spectral response, detection efficiency and spatial resolution for gamma-rays and neutrons in the energy range of 2-15 MeV for 50 mm thick converters consisting of plain LXe volume and LXe-filled capillaries, of Teflon, Polyethylene or hydrogen-containing Teflon (Tefzel). Neutron detection efficiencies for plain LXe, Teflon-capillaries and Tefzel-capillaries converters were about 20% over the entire energy range. In polyethylene capillaries converters the neutron detection efficiency was about 10% at 2 MeV and increased up to about 20% at 14 MeV. Detection efficiencies of gammas in Teflon, Tefzel and polyethylene converters were ~35%. The plain-LXe converter provided the highest gamma-ray detection efficiency, of ~40-50% for 2-15 MeV energy range. Optimization of LXe-filled Tefzel capillary dimensions resulted in spatial resolution of ~1.5mm (FWHM) for neutrons and up to 3.5 mm (FWHM) for gamma-rays. Simulations of radiographic images of various materials using two discrete energy gamma-rays (4.4 MeV and 15.1 MeV) and neutrons in broad energy range (2-10 MeV) were performed in order to evaluate the potential of elemental discrimination., Comment: 29 pages, 17 figures

The Time-Resolved Integrative Optical Neutron (TRION) detector was developed for Fast Neutron Resonance Radiography (FNRR), a fast-neutron transmission imaging method that exploits characteristic energy-variations of the total scattering cross-section in the En = 1-10 MeV range to detect specific elements within a radiographed object. As opposed to classical event-counting time of flight (ECTOF), it integrates the detector signal during a well-defined neutron Time of Flight window corresponding to a pre-selected energy bin, e.g., the energy-interval spanning a cross-section resonance of an element such as C, O and N. The integrative characteristic of the detector permits loss-free operation at very intense, pulsed neutron fluxes, at a cost however, of recorded temporal resolution degradation. This work presents a theoretical and experimental evaluation of detector related parameters which affect temporal resolution of the TRION system., Comment: Pre-print, also appears at JINST KEYWORDS: Fast neutron detectors; Plastic scintillator; Neutron radiography; Time-of-flight spectroscopy; Detection of explosives; Image intensifier; Pulsed Fast Neutron Transmission Spectroscopy (PFNTS); Fast Neutron Resonance Radiography (FNRR); Simulation

Radiation-induced proportional-electroluminescence UV signals, emitted from the holes of a Thick Gas Electron Multiplier (THGEM) electrode immersed in liquid xenon, were recorded with a PMT for the first time. Significant photon yields were observed using a 0.4 mm thick electrode with 0.3 mm diameter holes; at 2 kV across the THGEM the photon yield was estimated to be ~600 UV photons/electron over 4pi This may pave the way towards the realization of novel single-phase noble-liquid radiation detectors incorporating liquid hole-multipliers (LHM); their concept is presented., Comment: To be published in the MPGD2013 JINST proceedings

Optical recording of avalanche-induced photons is an interesting tool for studying basic physics processes in gaseous detectors. In this work we demonstrate the potential of optical readout in avalanche-propagation investigations in Thick Gas Electron Multipliers (THGEMs) operated with Ne/CF4 (95/5). We present the results of direct measurements, with single- and cascaded-THGEM detectors irradiated with soft x-rays, of the hole-multiplicity and avalanche asymmetry within holes, as a function of detector parameters. Further study directions are discussed.

An air cargo inspection system combining two nuclear reaction based techniques, namely Fast-Neutron Resonance Radiography and Dual-Discrete-Energy Gamma Radiography is currently being developed. This system is expected to allow detection of standard and improvised explosives as well as special nuclear materials. An important aspect for the applicability of nuclear techniques in an airport inspection facility is the inventory and lifetimes of radioactive isotopes produced by the neutron and gamma radiation inside the cargo, as well as the dose delivered by these isotopes to people in contact with the cargo during and following the interrogation procedure. Using MCNPX and CINDER90 we have calculated the activation levels for several typical inspection scenarios. One example is the activation of various metal samples embedded in a cotton-filled container. To validate the simulation results, a benchmark experiment was performed, in which metal samples were activated by fast-neutrons in a water-filled glass jar. The induced activity was determined by analyzing the gamma spectra. Based on the calculated radioactive inventory in the container, the dose levels due to the induced gamma radiation were calculated at several distances from the container and in relevant time windows after the irradiation, in order to evaluate the radiation exposure of the cargo handling staff, air crew and passengers during flight. The possibility of remanent long-lived radioactive inventory after cargo is delivered to the client is also of concern and was evaluated., Comment: Proceedings of FNDA 2011

The development of a mm-spatial-resolution, resonant-response detector based on a micrometric glass capillary array filled with liquid scintillator is described. This detector was developed for Gamma Resonance Absorption (GRA) in 14N. GRA is an automatic-decision radiographic screening technique that combines high radiation penetration (the probe is a 9.17 MeV gamma ray) with very good sensitivity and specificity to nitrogenous explosives. Detailed simulation of the detector response to electrons and protons generated by the 9.17 MeV gamma-rays was followed by a proof-of-principle experiment, using a mixed gamma-ray and neutron source. Towards this, a prototype capillary detector was assembled, including the associated filling and readout systems. Simulations and experimental results indeed show that proton tracks are distinguishable from electron tracks at relevant energies, on the basis of a criterion that combines track length and light intensity per unit length., Comment: 18 pages, 16 figures

A stable reference light source based on an LED (Light Emission Diode) is presented for stabilizing the conversion gain of the opto-electronic system of a gamma- and fast-neutron radiographic and tomographic imaging device. A constant fraction of the LED light is transported to the image plane of the camera and provides a stable reference exposure. This is used to normalize the images during off-line image processing. We have investigated parameters influencing the stability of LEDs and developed procedures and criteria to prepare and select LEDs suitable for delivering stable light outputs for several 100 h of operation.

A dual-purpose ion-accelerator concept, capable of serving as radiation source in a versatile, nuclear-reaction-based cargo inspection system, is presented. The system will automatically and reliably detect small, operationally-relevant quantities of concealed explosives and special nuclear materials (SNM). It will be cost-effective, employing largely-common hardware, but different reactions/DAQ-modes. Typical expected throughput is 10-20 aviation containers/hr. PACS: 25.20.Dc; 25.40.Ny; 27.20.+n; 29.27.Fh; 79.77.+g; 89.20.Bb; 89.20.Dd Keywords: Cargo inspection; Nuclear-reaction-based methods; Explosives detection; SNM detection

Two generations of a novel detector for high-resolution transmission imaging and spectrometry of fast-neutrons are presented. These devices are based on a hydrogenous fiber scintillator screen and single- or multiple-gated intensified camera systems (ICCD). This detector is designed for energy-selective neutron radiography with nanosecond-pulsed broad-energy (1 - 10 MeV) neutron beams. Utilizing the Time-of-Flight (TOF) method, such a detector is capable of simultaneously capturing several images, each at a different neutron energy (TOF). In addition, a gamma-ray image can also be simultaneously registered, allowing combined neutron/gamma inspection of objects. This permits combining the sensitivity of the fast-neutron resonance method to low-Z elements with that of gamma radiography to high-Z materials., Comment: Also published in JINST: http://www.iop.org/EJ/abstract/1748-0221/4/05/P05016

TRION is a sub-mm spatial resolution fast neutron imaging detector, which employs an integrative optical time-of-flight technique. The detector was developed for fast neutron resonance radiography, a method capable of detecting a broad range of conventional and improvised explosives. In this study we have analyzed in detail, using Monte-Carlo calculations and experimentally determined parameters, all the processes that influence the signal and noise in the TRION detector. In contrast to event-counting detectors where the signal-to-noise ratio is dependent only on the number of detected events (quantum noise), in an energy-integrating detector additional factors, such as the fluctuations in imparted energy, number of photoelectrons, system gain and other factors will contribute to the noise. The excess noise factor (over the quantum noise) due to these processes was 4.3, 2.7, 2.1, 1.9 and 1.9 for incident neutron energies of 2, 4, 7.5, 10 and 14 MeV, respectively. It is shown that, even under ideal light collection conditions, a fast neutron detection system operating in an integrative mode cannot be quantum-noise-limited due to the relatively large variance in the imparted proton energy and the resulting scintillation light distributions., Comment: 18 pages

We present the results of our recent studies on a Thick Gas Electron Multiplier (THGEM)-based imaging detector prototype. It consists of two 100x100 mm^2 THGEM electrodes in cascade, coupled to a resistive anode. The event location is recorded with a 2D double-sided readout electrode equipped with discrete delay-lines and dedicated electronics. The THGEM electrodes, produced by standard printed-circuit board and mechanical drilling techniques, a 0.4 mm thick with 0.5 mm diameter holes spaced by 1 mm. Localization resolutions of about 0.7 mm (FWHM) were measured with soft x-rays, in a detector operated with atmospheric-pressure Ar/CH4; good linearity and homogeneity were achieved. We describe the imaging-detector layout, the resistive-anode 2D readout system and the imaging properties. The THGEM has numerous potential applications that require large-area imaging detectors, with high-rate capability, single-electron sensitivity and moderate (sub-mm) localization resolution., Comment: Published in JINST, 22 pages, 18 figures

Thick GEM-like (THGEM) electrodes are robust, high gain gaseous electron multipliers, economically-manufactured by standard drilling and etching of thin printed circuit board or other materials. Their operation and structure are similar to that of standard GEMs but with 5 to 20-fold expanded dimensions. Due to the larger hole dimensions they provide up to 10^5 and 10^7 charge multiplication, in a single- and in two-electrode cascade, respectively. The signal rise time is of a few ns and the counting-rate capability approaches 10 MHz/mm^2 at 10^4 gains. Sub-mm localization precision was demonstrated with a simple, delay-line based 2D readout scheme. These multipliers may be produced in a variety of shapes and sizes and can operate in many gases. They may replace the standard GEMs in many applications requiring very large area, robust, flat, thin detectors, with good timing and counting-rate properties and modest localization. The properties of these multipliers are presented in short and possible applications are discussed., Comment: 3 pages, 6 figures, SNIC Symposium, Stanford, California, 3-6 April 2006

We have analyzed and compared the performance of two novel fast-neutron imaging methods with time-of-flight spectroscopy capability. Using MCNP and GEANT code simulations of neutron and charged-particle transport in the detectors, key parameters such as detection efficiency, the amount of energy deposited in the converter and the spatial resolution of both detector variants have been evaluated.

One of our two methods for fast-neutron imaging with spectrometric capability is presented here. It is a neutron-counting technique based on a hydrogenous neutron converter coupled to Gaseous Electron Multipliers (GEM). The principles of the detection techniques and the optimization of the converter, electron amplification and the readout are described. Evaluation of the properties are derived from a experiment in a pulsed neutron beam of spectral distribution between 2 and 10 MeV

Two detectors for energy-resolved fast-neutron imaging in pulsed broad-energy neutron beams are presented. The first one is a neutron-counting detector based on a solid neutron converter coupled to a gaseous electron multiplier (GEM). The second is an integrating imaging technique, based on a scintillator for neutron conversion and an optical imaging system with fast framing capability.