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We study the impact of mechanical vibrations on the performance of the photonic "hourglass" structure, which is predicted to emit single photons on-demand with near-unity efficiency and indistinguishability. Previous investigations neglected the impact of vibrational modes inherent to this quasi-1D geometry, relying instead on a three-dimensional bulk assumption for the phonon modes. However, it has been shown that phonon decoherence has a much stronger impact in 1D structures as compared with bulk media. Here, we surprisingly demonstrate the robustness of the photonic hourglass design, achieving close-to-unity indistinguishability even by incorporating a detailed description of the vibrational modes. We explain this unexpected result in terms of the large Purcell enhancement of the hourglass single-photon source, which eliminates the negative effect of phonons. Our findings highlight the key role of high-Q optical cavities in mitigating the detrimental effect of phonon decoherence, even for structures of reduced dimensionality., Comment: 11 pages, 6 figures

While the semiconductor quantum dot placed in a solid-state material allows for deterministic emission of single photons, the photon indistinguishability is strongly influenced by the intrinsic coupling to lattice vibrations, phonons, of the solid-state environment. This work investigates the phonon-induced decoherence for a quantum dot placed in the one-dimensional system of a homogeneous cylindrical nanowire. Such a structure supports multiple longitudinal phonon branches, and we consider both a linear and a quadratic coupling of the emitter to these modes. Under a polaron approach, we initially derive an analytical expression for the 1D pure dephasing rate, which leads to a reduced pure dephasing rate compared with bulk. By implementing these results into a full cavity quantum electrodynamic model, we demonstrate that multimode coupling is necessary to correctly predict the indistinguishability in a 1D system, which may otherwise be significantly underestimated., Comment: 21 pages, 14 figures

The swing-up of quantum emitter population (SUPER) scheme allows to populate the excited state of a quantum emitter with near-unity fidelity using two red-detuned laser pulses. Its off-resonant, yet fully coherent nature has attracted significant interest in quantum photonics as a valuable tool for preparing single-photon sources in their excited state on demand, while simultaneously ensuring straightforward spectral filtering of the laser. However, the physical understanding of this mechanism in terms of energy exchange between the electromagnetic field and the emitter is still lacking. Here, we present a fully quantized model of the swing-up excitation and demonstrate that it is in fact a multi-photon process, where one of the modes loses two or more photons while the other gains at least one. Our findings provide an unexpected physical interpretation of the SUPER scheme and unveil a new non-linear interaction between single emitters and multiple field modes., Comment: 15 pages, 6 figures + Supplemental document (4 pages, 2 figures)

The excitation scheme is essential for single-photon sources as it prepares the exciton state, defines the decay dynamics, and influences the spectral diffusion of the emitted single photons. Here, we investigate the impact of different optical excitation strategies on the single-photon emission characteristics of bilayer WSe$_2$ quantum emitters. Under phonon-assisted excitation, we achieve narrow and stable single-photon emission with an excellent purity reaching $ 0.94\pm 0.02\,$. Furthermore, the decay time is reduced by more than an order of magnitude from $(16.65 \pm 2.39)\,$ns for above-band excitation to $(1.33 \pm 0.04)\,$ns for phonon-assisted excitation. Finally, we observe a suppressed spectral wandering along with a two-fold reduction of the spectral linewidth. Our comprehensive investigation highlights the critical role of the excitation method in optimizing the performance of WSe$_2$-based quantum emitters.

Quantum emitters in transition metal dichalcogenides (TMDs) have recently emerged as a promising platform for generating single photons for optical quantum information processing. In this work, we present an approach for deterministically controlling the polarization of fabricated quantum emitters in a tungsten diselenide (WSe$_2$) monolayer. We employ novel nanopillar geometries with long and sharp tips to induce a controlled directional strain in the monolayer, and we report on fabricated WSe$_2$ emitters producing single photons with a high degree of polarization $(99\pm 4 \%)$ and high purity ($g^{(2)}(0) = 0.030 \pm 0.025$). Our work paves the way for the deterministic integration of TMD-based quantum emitters for future photonic quantum technologies.

Within optical quantum information processing, single-photon sources based on a two-level system in a semiconductor material allow for on-demand generation of single photons. To initiate the spontaneous emission process, it is necessary to efficiently populate the excited state. However, reconciling the requirement for on-demand excitation with both high efficiency and high photon indistinguishability remains a challenge due to the presence of charge noise and phonon-induced decoherence in the solid-state environment. Here, we propose a method for reconstructing the phonon spectral density experienced by WSe$_{2}$ quantum emitters in the emission process. Using the reconstructed phonon spectral density, we analyze the performance of the resonant, phonon-assisted, and Swing-UP of the quantum EmitteR population (SUPER) swing-up excitation schemes. Under resonant excitation, we obtain an exciton preparation fidelity limited to $\sim$0.80 by the strong phonon coupling, which improves to 0.96 for the SUPER scheme (or 0.89, depending on the type of emitter considered). Under near-resonant phonon-assisted excitation, we observe near-unity excitation fidelity up to 0.976 (0.997). Additionally, we demonstrate that, assuming the suppression of the phonon sidebands, residual dephasing mechanisms such as charge/spin fluctuations are the dominating decoherence mechanisms undermining the photon indistinguishability., Comment: 13 pages, 5 figures

In this paper, we demonstrate that a few-period circular Bragg reflector around an infinite nanowire can increase the $\beta$ factor of the fundamental mode up to 0.999 due to further suppression of the emission into radiation modes caused by a photonic band gap effect. We then apply this strategy in the practically relevant case of the finite-sized SPS based on tapered nanowires and demonstrate that the collection efficiency can be further increased. Additionally, we also show the beneficial effects of adding optimized high-index rings around the micropillar SPS.

We present a detailed analysis of the physics governing the collection efficiency and the Purcell enhancement of the nanopost single-photon source. We show that a standard single-mode Fabry-P\'erot model is insufficient to describe the device performance, which benefits significantly from scattering from the fundamental mode to radiation modes. We show how the scattering mechanism decouples the collection efficiency from the Purcell enhancement, such that maximum collection efficiency is obtained off-resonance. Finally, we discuss how this scattering mechanism can be beneficial for future single-photon source designs.

Single-photon sources with near-unity efficiency and indistinguishability play a major role in the development of quantum technologies. However, on-demand excitation of the emitter imposes substantial limitations to the source performance. Here, we show that coherent two-color pumping allows for population inversion arbitrarily close to unity in bulk quantum dots thanks to a decoupling effect between the emitter and its phonon bath. Driving a micropillar single-photon source with this scheme, we calculate very high photon emission into the cavity mode (0.95 photons per pulse) together with excellent indistinguishability (0.975) in a realistic configuration, thereby removing the limitations imposed by the excitation scheme on single-photon source engineering., Comment: Replacement of a previous version entitled "Phonon-decoupled di-chromatic pumping scheme for highly efficient and indistinguishable single-photon sources"

We report a numerical design procedure for pursuing a near-unity coupling efficiency in quantum dot-cavity ridge waveguide single-photon sources by performing simulations with the finite element method. Our optimum design which is based on a 1D nanobeam cavity, achieves a high source efficiency $\epsilon_{xy}$ of 97.7$\%$ for an isotropic in-plane dipole, together with a remarkable Purcell factor of 38.6. Such a good performance is mainly attributed to the high index contrast of GaAs/SiO$_2$ and a careful cavity design achieving constructive interference and low scattering losses. Furthermore, we analyze the bottleneck of the proposed platform, which is the mode mismatch between the cavity mode and the Bloch mode in the nanobeam. Accordingly, we present the optimization recipe of an arbitrarily high-efficiency on-chip single-photon source by implementing a taper section, whose high smoothness is beneficial to gradually overcoming the mode mismatch, and therefore leading to a higher Purcell factor and source efficiency. Finally, we see good robustness of the source properties in the taper-nanobeam system under the consideration of realistic fabrication imperfections on the hole variation.

An on-going challenge within scalable optical quantum information processing is to increase the collection efficiency $\varepsilon$ and the photon indistinguishability $\eta$ of the single-photon source towards unity. Within quantum dot-based sources, the prospect of increasing the product $\varepsilon \eta$ arbitrarily close to unity was recently questioned. In this work, we discuss the influence of the trade-off between efficiency and indistinguishability in the presence of phonon-induced decoherence, and we show that the photonic "hourglass" design allows for improving $\varepsilon \eta$ beyond the predicted maximum for the standard micropillar design subject to this trade-off. This circumvention of the trade-off is possible thanks to control of the spontaneous emission into background radiation modes, and our work highlights the importance of engineering of the background emission in future pursuits of near-unity performance of quantum dot single-photon sources., Comment: Added some small sections discussing possible reduction in indistinguishability due to charge noise, the possibility of electrical pumping, and some additional excitation schemes. Added small clarifications regarding the indistinguishability of QDs in bulk, the usage of dielectric screening in photonic crystals, and on the strong coupling regime

We report on the design of nanohole/nanobeam cavities in ridge waveguides for on-chip, quantum-dot-based single-photon generation. Our design overcomes limitations of a low-refractive-index-contrast material platform in terms of emitter-mode coupling efficiency and yields an outcoupling efficiency of 0.73 to the output ridge waveguide. Importantly, this high coupling efficiency is combined with broadband operation of 9 nm full-width half-maximum. We provide an explicit design procedure for identifying the optimum geometrical parameters according to the developed design. Besides, we fabricate and optically characterize a proof-of-concept waveguide structure. The results of the microphotoluminescence measurements provide evidence for cavity-enhanced spontaneous emission from the quantum dot, thus supporting the potential of our design for on-chip single-photon sources applications.

We analyze the occurrence of in-plane anisotropy in the electronic, magnetic, elastic and transport properties of more than one thousand 2D materials from the C2DB database. We identify hundreds of anisotropic materials and classify them according to their point group symmetry and degree of anisotropy. A statistical analysis reveals that a lower point group symmetry and a larger amount of different elements in the structure favour all types of anisotropies, which could be relevant for future materials design approaches. Besides, we identify novel compounds, predicted to be easily exfoliable from a parent bulk compound, with anisotropies that largely outscore those of already known 2D materials. Our findings provide a comprehensive reference for future studies of anisotropic response in atomically-thin crystals and point to new previously unexplored materials for the next generation of anisotropic 2D devices., Comment: 19 pages, 8 figures

The outstanding transport properties expected at the edge of two-dimensional time-reversal invariant topological insulators have proven to be challenging to realize experimentally, and have so far only been demonstrated in very short devices. In search for an explanation to this puzzling observation, we here report a full first-principles calculation of topologically protected transport at the edge of novel quantum spin Hall insulators - specifically, Bismuth and Antimony halides - based on the non-equilibrium Green's functions formalism. Our calculations unravel two different scattering mechanisms that may affect two-dimensional topological insulators, namely time-reversal symmetry breaking at vacancy defects and inter-edge scattering mediated by multiple co-operating impurities, possibly non-magnetic. We discuss their drastic consequences for typical non-local transport measurements as well as strategies to mitigate their negative impact. Finally, we provide an instructive comparison of the transport properties of topologically protected edge states to those of the trivial edge states in MoS$_2$ ribbons. Although we focus on a few specific cases (in terms of materials and defect types) our results should be representative for the general case and thus have significance beyond the systems studied here., Comment: 12 pages, 7 figures + Supplemental Material

We investigate heat current fluctuations induced by a periodic train of Lorentzian-shaped pulses, carrying an integer number of electronic charges, in a Hong-Ou-Mandel interferometer implemented in a quantum Hall bar in the Laughlin sequence. We demonstrate that the noise in this collisional experiment cannot be reproduced in a setup with a single drive, in contrast to what is observed in the charge noise case. Nevertheless, the simultaneous collision of two identical levitons always leads to a total suppression even for the Hong-Ou-Mandel heat noise at all filling factors, despite the presence of emergent anyonic quasi-particle excitations in the fractional regime. Interestingly, the strong correlations characterizing the fractional phase are responsible for a remarkable oscillating pattern in the HOM heat noise, which is completely absent in the integer case. These oscillations can be related to the recently predicted crystallization of levitons in the fractional quantum Hall regime., Comment: 18 pages, 4 figures

Using a periodic train of Lorentzian voltage pulses, which generates soliton-like electronic excitations called Levitons, we investigate the charge density backscattered off a quantum point contact in the fractional quantum Hall regime. We find a regular pattern of peaks and valleys, reminiscent of analogous self-organization recently observed for optical solitons in non-linear environments. This crystallization phenomenon is confirmed by additional side dips in the Hong-Ou-Mandel noise, a feature that can be observed in nowadays electron quantum optics experiments., Comment: 9 pages, 4 figures

We study the photoassisted shot noise generated by a periodic voltage in the fractional quantum Hall regime. Fluctuations of the current are due to the presence of a quantum point contact operating in the weak backscattering regime. We show how to reconstruct the photoassisted absorption and emission probabilities by varying independently the dc and ac contributions to the voltage drive. This is made possible by the peculiar power-law behavior of the tunneling rates in the chiral Luttinger liquid theory, which allow to approximate the typical infinite sums of the photoassisted transport formalism in a simple and particularly convenient way., Comment: 6 pages, 2 figures, Proceedings of LT28 (Gothenburg, Sweden)

We investigate minimal excitation states for heat transport into a fractional quantum Hall system driven out of equilibrium by means of time-periodic voltage pulses. A quantum point contact allows for tunneling of fractional quasi-particles between opposite edge states, thus acting as a beam splitter in the framework of the electron quantum optics. Excitations are then studied through heat and mixed noise generated by the random partitioning at the barrier. It is shown that levitons, the single-particle excitations of a filled Fermi sea recently observed in experiments, represent the cleanest states for heat transport, since excess heat and mixed shot noise both vanish only when Lorentzian voltage pulses carrying integer electric charge are applied to the conductor. This happens in the integer quantum Hall regime and for Laughlin fractional states as well, with no influence of fractional physics on the conditions for clean energy pulses. In addition, we demonstrate the robustness of such excitations to the overlap of Lorentzian wavepackets. Even though mixed and heat noise have nonlinear dependence on the voltage bias, and despite the non-integer power-law behavior arising from the fractional quantum Hall physics, an arbitrary superposition of levitons always generates minimal excitation states., Comment: 15 pages, 7 figures

We consider thermoelectric transport properties of the edge states of a two dimensional topological insulator in a double quantum point contact geometry coupled to two thermally biased reservoirs. Both spin-preserving and spin-flipping tunneling processes between opposite edges are analyzed in the presence of electron-electron interactions. We demonstrate that the simultaneous presence of spin-flipping processes and interactions gives rise to a finite longitudinal spin current. Moreover, its sign and amplitude can be tuned by means of gate voltages with the possibility to generate a pure spin current, with a vanishing charge current., Comment: 9 pages, 7 figures

Interference represents one of the most striking manifestation of quantum physics in low-dimensional systems. Despite evidences of quantum interference in charge transport have been known for a long time, only recently signatures of interference induced thermal properties have been reported, paving the way for the phase-coherent manipulation of heat in mesoscopic devices. In this work we show that anomalous thermoelectric properties and efficient heat rectification can be achieved by exploiting the phase-coherent edge states of quantum Hall systems. By considering a tunneling geometry with multiple quantum point contacts, we demonstrate that the interference paths effectively break the electron-hole symmetry, allowing for a thermoelectric charge current flowing either from hot to cold or viceversa, depending on the details of the tunnel junction. Correspondingly, an interference induced heat current is predicted, and we are able to explain these results in terms of an intuitive physical picture. Moreover, we show that heat rectification can be achieved by coupling two quantum Hall systems with different filling factors, and that this effect can be enhanced by exploiting the interference properties of the tunnel junction., Comment: 9 pages, 7 figures

We analyze the backscattering current induced by a time dependent constriction as a tool to probe fractional topological insulators. We demonstrate an enhancement of the total current for a fractional topological insulator induced by the dominant tunneling excitation, contrary to the decreasing present in the integer case for not too strong interactions. This feature allows to unambiguously identify fractional quasiparticles. Furthermore, the dominant tunneling processes, which may involve one or two quasiparticles depending on the interactions, can be clearly determined., Comment: 6 pages, 3 figures