1. Nonlinear spectroscopy of semiconductor moir\'e materials
- Author
-
Evrard, B., Adlong, H. S., Ghita, A. A., Uto, T., Ciorciaro, L., Watanabe, K., Taniguchi, T., Kroner, M., and İmamoğlu, A.
- Subjects
Condensed Matter - Strongly Correlated Electrons ,Physics - Optics ,Quantum Physics - Abstract
We use time-resolved nonlinear pump--probe measurements to reveal features of semiconductor moir\'e materials not accessible to linear spectroscopy. With an intense, red-detuned pump pulse, we generate a high density of virtual excitons or exciton--polarons in various moir\'e minibands. A broadband probe pulse in turn measures the response of all optical resonances induced by the pump-generated excitations. We generically observe a coherent blue shift originating from contact-like exciton--exciton interactions. At charge neutrality, these measurements allow us to assess the spatial overlap between different optical excitations and to observe signatures of a bound biexciton state between two different moir\'e exciton modes. In contrast to electron doped monolayers, spatially confined moir\'e attractive polarons behave as an ensemble of non-interacting two-level emitters, exhibiting an electron-density-independent ac-Stark effect. Tuning the pump laser into resonance with the attractive polaron, we demonstrate the filling of the moir\'e lattice with localized polarons and thereby realize a nonequilibrium Bose--Fermi mixture in moir\'e flat bands.
- Published
- 2024