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We report here on results of experimental-theoretical investigation of high-order harmonic generation (HHG) in layers of CdSe semiconductor quantum dots of different sizes and a reference bulk CdSe thin film. We observe a strong decrease in the efficiency, up to complete suppression of HHG with energies of quanta above the bandgap for the smallest dots, whereas the intensity of below bandgap harmonics remains weakly affected by the dot size. In addition, it is observed that the ratio between suppression of above gap harmonics versus below gap harmonics increases with driving wavelength. We suggest that the reduction in the dot size below the classical electron oscillatory radius and the corresponding off the dots wall scattering limits the maximum acceleration by the laser field. Moreover, this scattering leads to a chaotization of motion, causing dephasing and a loss of coherence, therefore suppressing the efficiency of the emission of highest-order harmonics. Our results demonstrate a new regime of intense laser-nanoscale solid interaction, intermediate between the bulk and single molecule response., Comment: 32 pages, 19 Figures

We report on experimental results in a new regime of a relativistic light-matter interaction employing mid-infrared (3.9-micrometer wavelength) high-intensity femtosecond laser pulses. In the laser generated plasma, the electrons reach relativistic energies already at rather low intensities due to the fortunate lambda^2-scaling of the kinetic energy with the laser wavelength. The lower intensity suppresses optical field ionization and creation of the pre-plasma at the rising edge of the laser pulse efficiently, enabling an enhanced efficient vacuum heating of the plasma. The lower critical plasma density for long-wavelength radiation can be surmounted by using nanowires instead of flat targets. In our experiments about 80% of the incident laser energy has been absorbed resulting in a long living, keV-temperature, high-charge state plasma with a density of more than three orders of magnitude above the critical value. Our results pave the way to laser-driven experiments on laboratory astrophysics and nuclear physics at a high repetition rate.

We present experimental evidence of ultra-high energy density plasma states with the keV bulk electron temperatures and near-solid electron densities generated during the interaction of high contrast, relativistically intense laser pulses with planar metallic foils. The bulk electron temperature and density have been measured using x-ray spectroscopy tools; the temperature of supra-thermal electrons traversing the target was determined from measured bremsstrahlung spectra; run-away electrons were detected using magnet spectrometers. The measured electron energy distribution was in a good agreement with results of Particle-in-Cell (PIC) simulations. Analysis of the bremsstrahlung spectra and results on measurements of the run-away electrons showed a suppression of the hot electrons production in the case of the high laser contrast. By application of Ti-foils covered with nm-thin Fe-layers we demonstrated that the thickness of the created keV hot dense plasma does not exceed 150 nm. Results of the pilot hydro-dynamic simulations that are based on a wide-range two-temperature EOS, wide-range description of all transport and optical properties, ionization, electron and radiative heating, plasma expansion, and Maxwell equations (with a wide-range permittivity) for description of the laser absorption are in excellent agreement with experimental results. According to these simulations, the generation of keV-hot bulk electrons is caused by the collisional mechanism of the laser pulse absorption in plasmas with a near solid step-like electron density profile. The laser energy firstly deposited into the nm-thin skin-layer is then transported into the target depth by the electron heat conductivity. This scenario is opposite to the volumetric character of the energy deposition produced by supra-thermal electrons., Comment: 15 pages, 10 figures

Accurate spectroscopy of highly charged high-Z ions in a storage ring is demonstrated to be feasible by the use of specially adapted crystal optics. The method has been applied for the measurement of the 1s Lamb shift in hydrogen-like gold (Au 78+) in a storage ring through spectroscopy of the Lyman x rays. This measurement represents the first result obtained for a high-Z element using high-resolution wavelength-dispersive spectroscopy in the hard x-ray regime, paving the way for sensitivity to higher-order QED effects.

Group velocity control is demonstrated for x-ray photons of 14.4 keV energy via a direct measurement of the temporal delay imposed on spectrally narrow x-ray pulses. Sub-luminal light propagation is achieved by inducing a steep positive linear dispersion in the optical response of ${}^{57}$Fe M\"ossbauer nuclei embedded in a thin film planar x-ray cavity. The direct detection of the temporal pulse delay is enabled by generating frequency-tunable spectrally narrow x-ray pulses from broadband pulsed synchrotron radiation. Our theoretical model is in good agreement with the experimental data., Comment: 8 pages, 4 figures

The properties of high energy density plasma are under increasing scrutiny in recent years due to their importance to our understanding of stellar interiors, the cores of giant planets$^{1}$, and the properties of hot plasma in inertial confinement fusion devices$^2$. When matter is heated by X-rays, electrons in the inner shells are ionized before the valence electrons. Ionization from the inside out creates atoms or ions with empty internal electron shells, which are known as hollow atoms (or ions)$^{3,4,5}$. Recent advances in free-electron laser (FEL) technology$^{6,7,8,9}$ have made possible the creation of condensed matter consisting predominantly of hollow atoms. In this Letter, we demonstrate that such exotic states of matter, which are very far from equilibrium, can also be formed by more conventional optical laser technology when the laser intensity approaches the radiation dominant regime$^{10}$. Such photon-dominated systems are relevant to studies of photoionized plasmas found in active galactic nuclei and X-ray binaries$^{11}$. Our results promote laser-produced plasma as a unique ultra-bright x-ray source for future studies of matter in extreme conditions as well as for radiography of biological systems and for material science studies$^{12,13,14,15}$.