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An assessment of different materials for additive manufacturing (AM) of polymer gears is presented in this research. Experimental testing is carried out for three different materials. Two materials are selected as the most common materials used for gears made by additive manufacturing. These materials are nylon and polycarbonate (PC). The third material is IGUS i180, which is a tribological material specially developed for additive manufacturing of parts with demands for high resistance properties such as resistance to friction, wear, and high temperatures which are essential for the long service life of gears. Gears are experimentally tested to determine service life in the form of operating cycles until failure. In addition, the gear temperature is monitored during the experimental testing. Using the value of maximum temperature at the moment of total gear failure at a specific load level enables the categorization of failure type. Different types of gear failures are categorized and presented. Taking into consideration failure type and the service life in the form of operating cycles, the applicability of analyzed materials for specific applications concerning load, speed, and thermal conditions is presented and discussed at the end of the paper. The main goal of this research was to test IGUS i180 material and compare its mechanical and thermal properties with other commonly used materials for gears manufactured by AM, such as nylon (PA6/66) and polycarbonate (PC). IGUS i180 material showed inferior properties concerning gear design in the case of high loads. This research showed that PA6/66 material is still the best solution for polymer gears production using AM, but the applicability of this material, due to temperature constraints, is still quite limited. [ABSTRACT FROM AUTHOR]