Nicholson, Christopher W, Rumo, Maxime, Pulkkinen, Aki, Kremer, Geoffroy, Salzmann, Björn, Mottas, Marie-Laure, Hildebrand, Baptiste, Jaouen, Thomas, Kim, Timur K, Mukherjee, Saumya, Ma, KeYuan, Muntwiler, Matthias, von Rohr, Fabian O, Cacho, Cephise, Monney, Claude, University of Zurich, University of Fribourg, Institut de Physique de Rennes (IPR), Université de Rennes 1 (UR1), Université de Rennes (UNIV-RENNES)-Université de Rennes (UNIV-RENNES)-Centre National de la Recherche Scientifique (CNRS), DIAMOND Light source, Universität Zürich [Zürich] = University of Zurich (UZH), Paul Scherrer Institute (PSI), Université de Fribourg = University of Fribourg (UNIFR), Université de Rennes (UR)-Centre National de la Recherche Scientifique (CNRS), and This project was supported through the Swiss National Science Foundation (SNSF), Grant No. P00P2_170597. We gratefully acknowledge beam time from Diamond light source (proposal SI24880, beamline I05) and the Swiss light source (proposal 20170698, PEARL beamline). A.P. acknowledges the Osk. Huttunen Foundation for financial support, and the CSC–IT Center for Science, Finland, for computational resources. The work at the University of Zurich was supported by the Swiss National Science Foundation under Grant No. PZ00P2_174015.
International audience; Strain is ubiquitous in solid-state materials, but despite its fundamental importance and technological relevance, leveraging externally applied strain to gain control over material properties is still in its infancy. In particular, strain control over the diverse phase transitions and topological states in two-dimensional transition metal dichalcogenides remains an open challenge. Here, we exploit uniaxial strain to stabilize the long-debated structural ground state of the 2D topological semimetal IrTe2, which is hidden in unstrained samples. Combined angle-resolved photoemission spectroscopy and scanning tunneling microscopy data reveal the strain-stabilized phase has a 6 × 1 periodicity and undergoes a Lifshitz transition, granting unprecedented spectroscopic access to previously inaccessible type-II topological Dirac states that dominate the modified inter-layer hopping. Supported by density functional theory calculations, we show that strain induces an Ir to Te charge transfer resulting in strongly weakened inter-layer Te bonds and a reshaped energetic landscape favoring the 6×1 phase. Our results highlight the potential to exploit strain-engineered properties in layered materials, particularly in the context of tuning inter-layer behavior.