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To assess public exposure to radon, thoron, and their progeny, measurements were conducted in 50 dwellings within the bauxite-rich area of Fongo-Tongo in western Cameroon. Passive integrating radon-thoron discriminative detectors (specifically RADUET) were employed for radon and thoron measurements. Additionally, concentrations of short-lived radon and thoron progeny were estimated using Direct Radon Progeny Sensors (DRPSs) and Direct Thoron Progeny Sensors (DTPSs) based on LR-115 detectors. The findings revealed indoor radon concentrations ranging from 31 to 123 Bq m−3 with a geometric mean (GM) of 62 Bq m−3, and indoor thoron concentrations ranging from 36 to 688 Bq m−3 with a GM of 242 Bq m−3. The Equilibrium Equivalent Radon Concentration (EERC) ranged from 3 to 86 Bq m−3 with a GM of 25 Bq m−3, while the Equilibrium Equivalent Thoron Concentration (EETC) ranged from 1.2 to 12.5 Bq m−3 with a GM of 7.6 Bq m−3. Notably, all dwellings recorded radon concentrations below 100 Bq m−3. Arithmetic means of radon and thoron equilibrium factors were calculated as 0.47 and 0.04, respectively. To assess annual effective doses from radon and thoron inhalation, equilibrium factors were used along with direct measurements of EERC and EETC. The differences observed in annual effective doses were 4.5% for radon and 42.5% for thoron. Furthermore, the contribution of thoron and its decay products to the annual effective dose from radon, thoron, and their progeny ranged from 12 to 94%, with an average contribution of 58%. Thus, this study found that the effective dose due to thoron inhalation in the study area exceeded that due to radon inhalation. It is concluded that, when evaluating radiation doses and health risks, it is crucial to consider both thoron and its progeny alongside radon and its progeny. This underscores the importance of considering direct measurements for accurately estimating radiation doses. [ABSTRACT FROM AUTHOR]

Radiation shielding materials have been researched using Pb and metal oxide particles, and composites of resin and barium sulfate (BaSO4) have been reported. In addition, multiwalled carbon nanotubes (MWCNTs) have often been used as a nanomaterial to improve the mechanical strength of resin–BaSO4 composites. The literature includes no examples of these two materials—BaSO4 and MWCNTs—being used at the interface of composites. We effectively modified the surface of BaSO4 by a simple process involving strong electrostatic interaction between positively charged barium and negatively charged functional groups on the MWCNT surface. The process is simple and can form large amounts of MWCNTs that coat BaSO4 surfaces. As a result, MWCNTs remained on the BaSO4 surface even after the MWCNT‐coated BaSO4 was washed with a solvent and subjected to melt mixing. The physical anchoring of MWCNTs onto the BaSO4 surface improved the interfacial adhesion and mechanical properties of the resultant composites. The originality of this research is that MWCNTs can be coated onto the surface by only electrostatic interaction without using a polymer adhesive. In addition, the x‐ray shielding performance of the MWCNT‐containing composites was the same as that of composites prepared without the MWCNTs. Highlights: MWCNTs were coated onto the surface of BaSO4 by electrostatic interaction.Interfacial adhesion of PS composites was improved by coating MWCNTs.The MWCNTs did not affect the x‐ray shielding performance. [ABSTRACT FROM AUTHOR]

Chiang Mai province of Thailand is known for having the highest natural background radiation in the country, as well as being recognized as one of the world's most polluted cities for air quality. This represents the major contributor to the development of lung cancer. This research aims to estimate the comprehensive dose of both internal and external exposure due to natural background radiation and related health perspectives in the highly polluted area of Chiang Mai. The average values of indoor radon and thoron concentrations in 99 houses over 6 months were 40.8 ± 22.6 and 17.8 ± 16.3 Bq/m3, respectively. These results exceed the worldwide value for indoor radon and thoron (40 and 10 Bq/m3), respectively. During burning season, the average values of indoor radon (56.7 ± 20 Bq/m3) and thoron (20.8 ± 20.4 Bq/m3) concentrations were higher than the world-wide averages. The radon concentration in drinking water (56 samples) varied from 0.1 to 91.9 Bq/L, with an average value of 9.1 ± 22.8 Bq/L. Most of the drinking water samples (87%) fell below the recommended maximum contamination limit of 11.1 Bq/L. The average values of natural radionuclide (226Ra, 232Th and 40K) in 48 soil samples were 47 ± 20.9, 77.9 ± 29.7 and 700.1 ± 233 Bq/kg, respectively. All values were higher than the worldwide average of 35, 30 and 400 Bq/kg, respectively. The average value of outdoor absorbed gamma dose rate (98 ± 32.5 nGy/h) exceeded the worldwide average of 59 nGy/h. Meanwhile, the average activity concentrations of 226Ra, 232Th and 40K in 25 plant food samples were 2.7 ± 0.1, 3.2 ± 1.6 and 1000.7 ± 1.9 Bq/kg, respectively. The 40K concentration was the most predominant in plant foods. The highest concentrations of 226Ra, 232Th and 40K were found in Chinese cabbage, celery and cilantro, respectively. The total annual effective dose for residents in the study area varied from 0.6 to 4.3 mSv, with an average value of 1.4 mSv. This indicates a significant long-term public health hazard due to natural background radiation and suggests a heightened radiation risk for the residents. The excess lifetime cancer risk value (5.4) associated with natural background radiation was found to be higher than the recommended value. Moreover, the number of lung cancer cases per year per million average of 25.2 per million persons per year was in the limit range 170–230 per million people. Overall, our results will be used for future decision making in the prevention of lung cancer risk associated with natural background radiation. [ABSTRACT FROM AUTHOR]

The exposure from radon, thoron, and thoron progeny was measured for 45 dwellings in high background radiation area in Takandeang, Indonesia with ambient dose equivalent rate ranging from 0.34 μSv h−1 to 1.90 μSv h−1. The measurement was taken using passive radon and thoron discriminative detector and thoron progeny detector. This measurement was taken from November 2018 to October 2019, and within one month the detector would be replaced with a new detector. The concentrations of radon, thoron, and thoron progeny were calculated as 42–490 Bq m−3, 20–618 Bq m−3, and 4–40 Bq m−3, respectively. The concentrations for outdoor were 49–435 Bq m−3, 23–457 Bq m−3, and 4–37 Bq m−3, respectively, and the annual effective dose was 9.8–28.6 mSv y−1. Based on the result of Spearman’s correlations analysis between the indoor radon and thoron concentrations and between the indoor thoron progeny and thoron concentrations, we suggest that exposure to thoron cannot be predicted from exposure to radon, and the equilibrium equivalent thoron concentration has a large uncertainty when it is estimated from thoron concentration assuming a single thoron equilibrium factor.

The deposition-based direct indoor 222Rn and 220Rn progeny measurement techniques are mostly affected by the indoor environmental conditions, such as the ventilation, concentration of condensation nuclei, and reactions with the structure and its furnishings. In this study, a theoretical model of a direct 222Rn and 220Rn progeny monitor based on allyl diglycol carbonate (ADC or CR-39) was established to analyse the factors that influence the detection process by using the parameter sensitivity analysis. The aerosol parameters contributed the highest to the variance, followed by the aerodynamic parameters. With respect to the result of the Spearman’s correlation analysis, the aerosol-related and the room-related parameters are positive, whereas the aerodynamic parameters – which affect the turbulence of indoor deposition – are negative. It means that both the attachment process and the deposition process of 222Rn and 220Rn progenies are important to the performance of the progeny monitor.

In this study, the activity concentrations of radon (222Rn), thoron (220Rn) and thoron progeny were measured simultaneously in Djeno (Pointe-Noire, Republic of Congo) using RADUET detectors to evaluate the air quality and the radiological risks due to the inhalation of these radionuclides. Activity concentrations of radon progeny were calculated from those of radon. Indoor radon, thoron and progenies followed a lognormal distribution ranging between 20 and 40, 6 and 62, 8 and 17.6 and 0.4 and 19.6 Bq m−3 for radon, thoron, radon progeny and thoron progeny, respectively. Mean values for radon were lower than the worldwide values estimated by the United Nation Scientific Committee on the Effects of Atomic Radiation (UNSCEAR), which are 40 Bq m−3 (arithmetic mean) and 45 Bq m−3 (geometric mean). Radon concentrations in the dwellings under study were below the World Health Organization and the International Commission on Radiological Protection recommended reference levels, which are, respectively, 100 and 300 Bq m−3. The mean concentration of thoron was twice the world average value of 10 Bq m−3 estimated by UNSCEAR. Thoron progeny mean concentration was sharply greater than the typical value (0.3 Bq m−3) for indoor atmosphere provided by UNSCEAR. Annual effective dose ranges were 0.40–0.87 mSv (arithmetic mean, 0.57 ± 0.11 mSv) for radon and 0.10–4.14 mSv (arithmetic mean, 0.55 ± 0.77 mSv) for thoron. The mean value for radon was lower than the value (1.15 mSv) estimated by UNSCEAR, while the mean value for thoron was five times higher than the UNSCEAR value (0.10 mSv). The study showed that the use of the typical equilibrium factor value given by UNSCEAR to compute effective dose led to an error above 80%. Finally, the results of this study showed that the excess relative risk of radon-induced cancer was low, below 2% for the population under 55 y. The results presented in the present study prove that the population of Djeno is exposed to a relatively low potential risk of radon- and thoron-induced cancer. [ABSTRACT FROM AUTHOR]

Indoor radon, thoron and thoron progeny concentrations, along with the equilibrium factor for thoron progeny and soil gas radon concentrations, have been measured to assess radiological risks in the centre and south regions of Cameroon. Indoor radon and thoron concentrations were estimated using radon–thoron discriminative detectors (RADUET), while thoron progeny monitors measured the equilibrium equivalent thoron concentration (EETC). Radon concentrations in the soil were determined using a MARKUS 10 detector. It was found that radon, thoron and thoron progeny concentrations range between 19 and 62 Bq m−3, 10 and 394 Bq m−3 and 0.05 and 21.8 Bq m−3, with geometric means of 32 Bq m−3, 98 Bq m−3 and 4.9 Bq m−3, respectively. The thoron equilibrium factor ranges between 0.007 and 0.24, with an arithmetic mean of 0.06 ± 0.03; this is higher than the world average value of 0.02 provided by the United Nations Scientific Commission on the Effects of Atomic Radiation(UNSCEAR, New York, USA). The level of the soil radon concentration ranges from 4.8 to 57.3 kBq m−3, with a geometric mean of 12.1 kBq m−3 at a depth of 0.7 m. Of the sampling points, 66% fall within normal radon risk areas, and 3% of the sampling areas are high radon risk areas exceeding 50 kBq m−3. The annual effective dose was found to be 0.03 ± 0.01 mSv for radon, 0.08 ± 0.05 mSv for thoron, 0.63 ± 0.12 mSv for radon progeny and 1.40 ± 0.84 mSv for thoron progeny. The total dose is estimated to be 2.14 mSv y−1. The mean estimated indoor excess lifetime cancer risk values due to radon, thoron, radon progeny and thoron progeny are 0.12 × 10−3, 0.31 × 10−3, 2.51 × 10−3 and 5.58 × 10−3, respectively. Thoron progeny contributed 60% to the effective dose. Thus, thoron progeny cannot be neglected in dose assessments, in order to avoid biased results in radio-epidemiological studies. [ABSTRACT FROM AUTHOR]

Mamuju is an area of high natural radiation in Indonesia with high natural radiation levels (average 613 nSv h−1). Mamuju is anomalous due to its high average 238U and 232Th concentrations of 22,882 and 33,549 Bq kg−1, respectively, in laterite and rock. High natural radionuclide concentrations of 238U, 232Th, and 40K have also been reported in soil samples from several locations in Mamuju, including Botteng, Northern Botteng, Takandeang, Ahu, and Taan. High radiation levels are related to radioactive mineral occurrences in the Adang volcanic complex, comprised of phonolitoid and foiditoid lithologies. According to the International Atomic Energy Agency (IAEA), uranium deposits can be classified into several types, among them a volcanic-related deposits, which include three sub-types: stratabound, structure-bound, and volcano-sedimentary deposits. This study aims to characterize volcanic rock deposit sub-types in the Mamuju area based on uranium radioisotope measurements. The uranium isotopes were measured using a tandem quadrupole inductively coupled plasma mass spectrometer combined with chemical separation by extraction chromatography using UTEVA resin. The analytical results for the 234U/238U ratios are used to determine the formation characteristics of minerals in each deposit sub-type based on mineral formation age, post-formation processes, and disturbances that affected the formation processes. Based on geochronological calculations using 234U/238U mineralization age, the deposits in the Mamuju area are 0.914–1.11 million years old and are classified as recent mineralization. These data have important implications for tracing uranium source rocks in the Mamuju area and may explain the anomalously high radiation levels in the Mamuju area. [ABSTRACT FROM AUTHOR]