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Abstract Astronomical precision spectroscopy underpins searches for life beyond Earth, direct observation of the expanding Universe and constraining the potential variability of physical constants on cosmological scales. Laser frequency combs can provide the required accurate and precise calibration to the astronomical spectrographs. For cosmological studies, extending the calibration with such astrocombs to the ultraviolet spectral range is desirable, however, strong material dispersion and large spectral separation from the established infrared laser oscillators have made this challenging. Here, we demonstrate astronomical spectrograph calibration with an astrocomb in the ultraviolet spectral range below 400 nm. This is accomplished via chip-integrated highly nonlinear photonics in periodically-poled, nano-fabricated lithium niobate waveguides in conjunction with a robust infrared electro-optic comb generator, as well as a chip-integrated microresonator comb. These results demonstrate a viable route towards astronomical precision spectroscopy in the ultraviolet and could contribute to unlock the full potential of next-generation ground-based and future space-based instruments.

Abstract Femtosecond laser pulses enable the synthesis of light across the electromagnetic spectrum and provide access to ultrafast phenomena in physics, biology, and chemistry. Chip-integration of femtosecond technology could revolutionize applications such as point-of-care diagnostics, bio-medical imaging, portable chemical sensing, or autonomous navigation. However, current chip-integrated pulse sources lack the required peak power, and on-chip amplification of femtosecond pulses has been an unresolved challenge. Here, addressing this challenge, we report >50-fold amplification of 1 GHz-repetition-rate chirped femtosecond pulses in a CMOS-compatible photonic chip to 800 W peak power with 116 fs pulse duration. This power level is 2–3 orders of magnitude higher compared to those in previously demonstrated on-chip pulse sources and can provide the power needed to address key applications. To achieve this, detrimental nonlinear effects are mitigated through all-normal dispersion, large mode-area and rare-earth-doped gain waveguides. These results offer a pathway to chip-integrated femtosecond technology with peak power levels characteristic of table-top sources.

Abstract Microresonator frequency combs (microcombs) hold great potential for precision metrology within a compact form factor, impacting a wide range of applications such as point-of-care diagnostics, environmental monitoring, time-keeping, navigation and astronomy. Through the principle of self-injection locking, electrically-driven chip-based microcombs with minimal complexity are now feasible. However, phase-stabilisation of such self-injection-locked microcombs—a prerequisite for metrological frequency combs—has not yet been attained. Here, we address this critical need by demonstrating full phase-stabilisation of a self-injection-locked microcomb. The microresonator is implemented in a silicon nitride photonic chip, and by controlling a pump laser diode and a microheater with low voltage signals (less than 1.57 V), we achieve independent control of the comb’s offset and repetition rate frequencies. Both actuators reach a bandwidth of over 100 kHz, enabling phase-locking of the microcomb to external frequency references. These results establish photonic chip-based, self-injection-locked microcombs as low-complexity yet versatile sources for coherent precision metrology in emerging applications.

Frequency combs from continuous-wave-driven Kerr-nonlinear microresonators have evolved into a key photonic technology with applications from optical communication to precision spectroscopy. Essential to many of these applications is the control of the comb’s defining parameters, i.e., carrier-envelope offset frequency and repetition rate. An elegant and all-optical approach to controlling both degrees of freedom is the suitable injection of a secondary continuous-wave laser into the resonator onto which one of the comb lines locks. Here, we experimentally study such sideband injection locking in microresonator soliton combs across a wide optical bandwidth and derive analytic scaling laws for the locking range and repetition rate control. As an application example, we demonstrate optical frequency division and repetition rate phase-noise reduction to three orders of magnitude below the noise of a free-running system. The presented results can guide the design of sideband injection-locked, parametrically generated frequency combs with opportunities for low-noise microwave generation, compact optical clocks with simplified locking schemes, and, more generally, all-optically stabilized frequency combs from Kerr-nonlinear resonators.

Abstract Cavity ring-down spectroscopy is a ubiquitous optical method used to study light-matter interactions with high resolution, sensitivity and accuracy. However, it has never been performed with the multiplexing advantages of direct frequency comb spectroscopy without significantly compromising spectral resolution. We present dual-comb cavity ring-down spectroscopy (DC-CRDS) based on the parallel heterodyne detection of ring-down signals with a local oscillator comb to yield absorption and dispersion spectra. These spectra are obtained from widths and positions of cavity modes. We present two approaches which leverage the dynamic cavity response to coherently or randomly driven changes in the amplitude or frequency of the probe field. Both techniques yield accurate spectra of methane—an important greenhouse gas and breath biomarker. When combined with broadband frequency combs, the high sensitivity, spectral resolution and accuracy of our DC-CRDS technique shows promise for applications like studies of the structure and dynamics of large molecules, multispecies trace gas detection and isotopic composition.

Nonlinear optical frequency conversion is of fundamental importance in photonics and underpins countless of its applications: Sum- and difference-frequency generation in media with quadratic nonlinearity permits reaching otherwise inaccessible wavelength regimes, and the dramatic effect of supercontinuum generation through cubic nonlinearities has resulted in the synthesis of broadband multi-octave spanning spectra, much beyond what can be directly achieved with laser gain media. Chip-integrated waveguides permit to leverage both quadratic and cubic effects at the same time, creating unprecedented opportunities for multi-octave spanning spectra across the entire transparency window of a nonlinear material. Designing such waveguides often relies on numeric modeling of the underlying nonlinear processes, which, however, becomes exceedingly challenging when multiple and cascading nonlinear processes are involved. Here, to address this challenge, we report on a novel numeric simulation tool for mixed and cascaded nonlinearities that uses anti-aliasing strategies to avoid spurious light resulting from a finite simulation bandwidth. A dedicated fifth-order interaction picture Runge–Kutta solver with adaptive step-size permits efficient numeric simulation, as required for design parameter studies. The simulation results are shown to quantitatively agree with experimental data, and the simulation tool is available as an open-source Python package (pychi).

Here, the authors show that the resolution and speed limitations in broadband photo-acoustic spectroscopy can be overcome by combining dual-comb spectroscopy with photo-acoustic detection. This enables broadband detection and allows for rapid and sensitive multi-species molecular analysis across all wavelengths of light.

We present an analysis of Sun-as-a-star observations from four different high-resolution, stabilized spectrographs—HARPS, HARPS-N, EXPRES, and NEID. With simultaneous observations of the Sun from four different instruments, we are able to gain insight into the radial velocity precision and accuracy delivered by each of these instruments and isolate instrumental systematics that differ from true astrophysical signals. With solar observations, we can completely characterize the expected Doppler shift contributed by orbiting Solar System bodies and remove them. This results in a data set with measured velocity variations that purely trace flows on the solar surface. Direct comparisons of the radial velocities measured by each instrument show remarkable agreement with residual intraday scatter of only 15–30 cm s ^−1 . This shows that current ultra-stabilized instruments have broken through to a new level of measurement precision that reveals stellar variability with high fidelity and detail. We end by discussing how radial velocities from different instruments can be combined to provide powerful leverage for testing techniques to mitigate stellar signals.