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To determine the safety of using argon as a deuteron beam stopping material, the

Plastic organic scintillators have been tailored in composition to achieve ultra-fast temporal response, thereby enabling the design and development of fast neutron detection systems with high timing resolution. Eljen Technology's plastic organic scintillators -- EJ-230, EJ-232, and EJ-232Q -- are prospective candidates for use in emerging neutron imaging systems, where fast timing is paramount. To support the neutron response characterization of these materials, the relative proton light yields of EJ-230, EJ-232, and EJ-232Q were measured at the 88-Inch Cyclotron at Lawrence Berkeley National Laboratory. Using a broad-spectrum neutron source and a double time-of-flight technique, the proton light yield relations were obtained over a proton recoil energy range of approximately 300 keV to 4 MeV. The EJ-230, EJ-232, and EJ-232Q scintillators exhibited similar proton light yield relations to each other as well as to other plastic scintillators with the same polymer base material. A comparison of the relative proton light yield of different sized cylindrical EJ-232 and EJ-232Q scintillators also revealed consistent results. This work provides key input data for the realistic computational modeling of neutron detection technologies employing these materials, thereby supporting new capabilities in near-field radionuclide detection for national security applications., Comment: 10 pages, 8 figures

Organic scintillators doped with capture agents provide a detectable signal for neutrons over a broad energy range. This work characterizes the fast and slow neutron response of EJ-254, an organic plastic scintillator with 5% natural boron loading by weight. For fast neutrons, the primary mechanism for light generation in organic scintillators is n-p elastic scattering. To study the fast neutron response, the proton light yield of EJ-254 was measured at the 88-Inch Cyclotron at Lawrence Berkeley National Laboratory. Using a broad-spectrum neutron source and a double time-of-flight technique, the EJ-254 proton light yield was obtained over the energy range of approximately 270 keV to 4.5 MeV and determined to be in agreement with other plastic scintillators comprised of the same polymer base. To isolate the slow neutron response, an AmBe source with polyethylene moderator was made incident on the EJ-254 scintillator surrounded by an array of EJ-309 observation detectors. Events in the EJ-254 target coincident with the signature 477.6 keV $\gamma$ ray (resulting from deexcitation of the residual $^{7}$Li nucleus following boron neutron capture) were identified. Pulse shape discrimination was used to evaluate the temporal differences in the response of EJ-254 scintillation signals arising from $\gamma$-ray and fast/slow neutron interactions. Clear separation between $\gamma$-ray and fast neutrons signals was not achieved and the neutron capture feature was observed to overlap both the $\gamma$-ray and fast neutron bands. Taking into account the electron light nonproportionality, the neutron-capture light yield in EJ-254 was determined to be 89.4$\pm$1.1 keVee., Comment: 9 pages, 10 figures

Background: Organic scintillators are widely used for neutron detection in both basic nuclear physics and applications. While the proton light yield of organic scintillators has been extensively studied, measurements of the light yield from neutron interactions with carbon nuclei are scarce. Purpose: Demonstrate a new approach for the simultaneous measurement of the proton and carbon light yield of organic scintillators. Provide new carbon light yield data for the EJ-309 liquid and EJ-204 plastic organic scintillators. Method: A 33~MeV $^{2}$H$^{+}$ beam from the 88-Inch Cyclotron at Lawrence Berkeley National Laboratory was impinged upon a 3-mm-thick Be target to produce a high-flux, broad-spectrum neutron beam. The double time-of-flight technique was extended to simultaneously measure the proton and carbon light yield of the organic scintillators, wherein the light output associated with the recoil particle was determined using $np$ and $n$C elastic scattering kinematics. Results: The proton and carbon light yield relations of the EJ-309 liquid and EJ-204 plastic organic scintillators were measured over a recoil energy range of approximately 0.3 to 1~MeV and 2 to 5~MeV, respectively for EJ-309, and 0.2 to 0.5~MeV and 1 to 4~MeV, respectively for EJ-204. Conclusions: These data provide new insight into the ionization quenching effect in organic scintillators and key input for simulation of the response of organic scintillators for both basic science and a broad range of applications., Comment: 11 pages, 9 figures

An organic glass scintillator developed by Sandia National Laboratories was characterized in terms of its light output and pulse shape discrimination (PSD) properties and compared to commercial liquid (EJ-309) and plastic (EJ-276) organic scintillators. The electron light output was determined through relative comparison of the $^{137}$Cs Compton edge location. The proton light yield was measured using a double time-of-flight technique at the 88-Inch Cyclotron at Lawrence Berkeley National Laboratory. Using a tunable broad-spectrum neutron source and an array of pulse-shape-discriminating observation scintillators, a continuous measurement of the proton light yield was performed for EJ-309 (200 keV$-$3.2 MeV), EJ-276 (170 keV$-$4.9 MeV), and the organic glass (50 keV$-$20 MeV). Finally, the PSD properties of the organic glass, EJ-309, and EJ-276 were evaluated using an AmBe source and compared via a figure-of-merit metric. The organic glass exhibited a higher electron light output than both EJ-309 and EJ-276. Its proton light yield and PSD performance were comparable to EJ-309 and superior to that of EJ-276. With these performance characteristics, the organic glass scintillator is well poised to replace current state-of-the-art PSD-capable scintillators in a range of fast neutron detection applications., 32 pages, 13 figures, 9 tables

In this paper we present the first systematic analysis of the impact of the populated vs. intrinsic spin distribution on the nuclear level density and γ-ray strength function retrieved through the Oslo Method. We illustrate the effect of the spin distribution on the recently performed 239Pu(d,pγ)240Pu experiment using a 12 MeV deuteron beam performed at the Oslo Cyclotron Lab. In the analysis we couple state-of-the-art calculations for the populated spin-distributions with the Monte-Carlo nuclear decay code RAINIER to compare Oslo Method results to the known input. We find that good knowledge of the populated spin distribution is crucial and show that the populated distribution has a significant impact on the extracted nuclear level density and γ-ray strength function for the 239Pu(d,pγ)240Pu case.

The proton light yield of organic scintillators has been measured extensively in recent years using fast waveform digitizers and large discrepancies exist in the values reported by different authors. In this letter, we address principles of digital signal processing that must be considered when conducting scintillator light yield measurements. Digitized waveform pulse height values are only proportional to the amount of scintillation light if the temporal shape of the scintillation pulse is independent of the amount of energy deposited. This is not the case for scintillation pulses resulting from fast neutron interactions in organic scintillators. Authors measuring proton light yield should therefore report pulse integral values and ensure that the integration length is long enough to capture most of the scintillation light., Comment: 6 pages, 2 figures

Compact neutron imagers using double-scatter kinematic reconstruction are being designed for localization and characterization of special nuclear material. These neutron imaging systems rely on scintillators with a rapid prompt temporal response as the detection medium. As n-p elastic scattering is the primary mechanism for light generation by fast neutron interactions in organic scintillators, proton light yield data are needed for accurate assessment of scintillator performance. The proton light yield of a series of commercial fast plastic organic scintillators---EJ-200, EJ-204, and EJ-208---was measured via a double time-of-flight technique at the 88-Inch Cyclotron at Lawrence Berkeley National Laboratory. Using a tunable deuteron breakup neutron source, target scintillators housed in a dual photomultiplier tube configuration, and an array of pulse-shape-discriminating observation scintillators, the fast plastic scintillator light yield was measured over a broad and continuous energy range down to proton recoil energies of approximately 50 keV. This work provides key input to event reconstruction algorithms required for utilization of these materials in emerging neutron imaging modalities., Comment: 15 pages, 6 figures

In outer space down to the altitudes routinely flown by larger aircrafts, radiation can pose serious issues for microelectronics circuits. The 88-Inch Cyclotron at Lawrence Berkeley National Laboratory is a sector-focused cyclotron and home of the Berkeley Accelerator Space Effects Facility, where the effects of energetic particles on sensitive microelectronics are studied with the goal of designing electronic systems for the space community. This paper describes the flexibility of the facility and its capabilities for testing the bombardment of electronics by heavy ions, light ions, and neutrons. Experimental capabilities for the generation of neutron beams from deuteron breakups and radiation testing of carbon nanotube field effect transistor will be discussed.

The fusion Z-pinch experiment (FuZE) is a sheared-flow stabilized Z-pinch designed to study the effects of flow stabilization on deuterium plasmas with densities and temperatures high enough to drive nuclear fusion reactions. Results from FuZE show high pinch currents and neutron emission durations thousands of times longer than instability growth times. While these results are consistent with thermonuclear neutron emission, energetically resolved neutron measurements are a stronger constraint on the origin of the fusion production. This stems from the strong anisotropy in energy created in beam-target fusion, compared to the relatively isotropic emission in thermonuclear fusion. In dense Z-pinch plasmas, a potential and undesirable cause of beam-target fusion reactions is the presence of fast-growing, “sausage” instabilities. This work introduces a new method for characterizing beam instabilities by recording individual neutron interactions in plastic scintillator detectors positioned at two different angles around the device chamber. Histograms of the pulse-integral spectra from the two locations are compared using detailed Monte Carlo simulations. These models infer the deuteron beam energy based on differences in the measured neutron spectra at the two angles, thereby discriminating beam-target from thermonuclear production. An analysis of neutron emission profiles from FuZE precludes the presence of deuteron beams with energies greater than 4.65 keV with a statistical uncertainty of 4.15 keV and a systematic uncertainty of 0.53 keV. This analysis demonstrates that axial, beam-target fusion reactions are not the dominant source of neutron emission from FuZE. These data are promising for scaling FuZE up to fusion reactor conditions.

The Oslo method has been applied to particle-$\ensuremath{\gamma}$ coincidences following the $^{239}\mathrm{Pu}(d,p)$ reaction to obtain the nuclear level density (NLD) and $\ensuremath{\gamma}$-ray strength function ($\ensuremath{\gamma}\mathrm{SF}$) of $^{240}\mathrm{Pu}$. The experiment was conducted with a 12 MeV deuteron beam at the Oslo Cyclotron Laboratory. The low spin transfer of this reaction leads to a spin-parity mismatch between populated and intrinsic levels. This is a challenge for the Oslo method as it can have a significant impact on the extracted NLD and $\ensuremath{\gamma}\mathrm{SF}$. We have developed an iterative approach to ensure consistent results even for cases with a large spin-parity mismatch, in which we couple Green's function transfer calculations of the spin-parity dependent population cross-section to the nuclear decay code rainier. The resulting $\ensuremath{\gamma}\mathrm{SF}$ shows a pronounced enhancement between 2--4 MeV that is consistent with the location of the low-energy orbital $M1$ scissors mode.

Herein we report the progress towards an organic glass scintillator with fast and thermal neutron sensitivity providing “triple” pulse shape discrimination (PSD) through the inclusion of a boron-incorporated aromatic molecule. The commercially available molecule 2-(p-tolyl)-1,3,2-dioxaborinane (TDB) can be readily synthesized in one step using inexpensive materials and incorporated into the organic glass scintillator at 20% by weight or 0.25% 10B by mass. In addition, we demonstrate that TDB can be easily scaled up and formulated into organic glass scintillator samples to produce a thermal neutron capture signal with a light yield equivalent to 120.4 ± 3.7 keVee, which is the highest value reported in the literature to date.

Author(s): Rose, SJ; Zeiser, F; Wilson, JN; Oberstedt, A; Oberstedt, S; Siem, S; Tveten, GM; Bernstein, LA; Bleuel, DL; Brown, JA; Crespo Campo, L; Giacoppo, F; Gorgen, A; Guttormsen, M; Hadynska, K; Hafreager, A; Hagen, TW; Klintefjord, M; Laplace, TA; Larsen, AC; Renstrom, T; Sahin, E; Schmitt, C; Tornyi, TG; Wiedeking, M | Abstract: Prompt-fission γ rays are responsible for approximately 5% of the total energy released in fission, and therefore important to understand when modeling nuclear reactors. In this work we present prompt γ-ray emission characteristics in fission as a function of the nuclear excitation energy of the fissioning system. Emitted γ-ray spectra were measured, and γ-ray multiplicities and average and total γ energies per fission were determined for the U(d,pf)233 reaction for excitation energies between 4.8 and 10 MeV, and for the Pu(d,pf)239 reaction between 4.5 and 9 MeV. The spectral characteristics show no significant change as a function of excitation energy above the fission barrier, despite the fact that an extra ∼5 MeV of energy is potentially available in the excited fragments for γ decay. The measured results are compared with model calculations made for prompt γ-ray emission with the fission model code gef. Further comparison with previously obtained results from thermal neutron induced fission is made to characterize possible differences arising from using the surrogate (d,p) reaction.

In the outer space down to the altitudes routinely flown by the larger commercial aircrafts, radiation is a serious problem for the microelectronics circuits. The 88-Inch Cyclotron at Lawrence Berkeley National Laboratory is a sector-focused cyclotron and is the home of the Berkeley Accelerator Space Effects Facility, where the effects of energetic particles on sensitive microelectronics are studied with the goal of designing electronic systems for the space community. The paper will describe the flexibility of the facility and its capabilities for testing the bombardment of the electronics by heavy ions, light ions, and neutrons.

Background: The Cd isotopes are well studied, but experimental data for the rare isotopes are sparse. At energies above the Coulomb barrier, higher states become accessible.Purpose: Remeasure and supplement existing lifetimes and magnetic moments of low-lying states in $^{106}\mathrm{Cd}$.Methods: In an inverse kinematics reaction, a $^{106}\mathrm{Cd}$ beam impinging on a $^{12}\mathrm{C}$ target was used to Coulomb excite the projectiles. The high recoil velocities provide a unique opportunity to measure $g$ factors with the transient-field technique and to determine lifetimes from lineshapes by using the Doppler-shift-attenuation method. Large-scale shell-model calculations were carried out for $^{106}\mathrm{Cd}$.Results: The $g$ factors of the ${2}_{1}^{+}$ and ${4}_{1}^{+}$ states in $^{106}\mathrm{Cd}$ were measured to be $g({2}_{1}^{+})=+0.398(22)$ and $g({4}_{1}^{+})=+0.23(5)$. A lineshape analysis yielded lifetimes in disagreement with published values. The new results are $\ensuremath{\tau}(^{106}\mathrm{Cd};{2}_{1}^{+})=7.0(3)\phantom{\rule{4.pt}{0ex}}\mathrm{ps}$ and $\ensuremath{\tau}(^{106}\mathrm{Cd};{4}_{1}^{+})=2.5(2)\phantom{\rule{4.pt}{0ex}}\mathrm{ps}$. The mean life $\ensuremath{\tau}(^{106}\mathrm{Cd};{2}_{2}^{+})=0.28(2)\phantom{\rule{4.pt}{0ex}}\mathrm{ps}$ was determined from the fully-Doppler-shifted $\ensuremath{\gamma}$ line. Mean lives of $\ensuremath{\tau}(^{106}\mathrm{Cd};{4}_{3}^{+})=1.1(1)\phantom{\rule{4.pt}{0ex}}\mathrm{ps}$ and $\ensuremath{\tau}(^{106}\mathrm{Cd};{3}_{1}^{\ensuremath{-}})=0.16(1)\phantom{\rule{4.pt}{0ex}}\mathrm{ps}$ were determined for the first time.Conclusions: The newly measured $g({4}_{1}^{+})$ of $^{106}\mathrm{Cd}$ is found to be only 59% of the $g({2}_{1}^{+})$. This difference cannot be explained by either shell-model or collective-model calculations.

In this study, the structure of the semimagic Sn50 isotopes were previously studied via measurements of B(E2;21+ → 01+) and g factors of 21+ states. The values of the B(E2;21+) in the isotopes below midshell at N = 66 show an enhancement in collectivity, contrary to predictions from shell-model calculations. This work presents the first measurement of the 21+ and 41+ states' magnetic moments in the unstable neutron-deficient 110Sn. The g factors provide complementary structure information to the interpretation of the observed B(E2) values.

The level density and gamma-ray strength function (gammaSF) of 243Pu have been measured in the quasi-continuum using the Oslo method. Excited states in 243Pu were populated using the 242Pu(d,p) reaction. The level density closely follows the constant-temperature level density formula for excitation energies above the pairing gap. The gammaSF displays a double-humped resonance at low energy as also seen in previous investigations of actinide isotopes. The structure is interpreted as the scissors resonance and has a centroid of omega_{SR}=2.42(5)MeV and a total strength of B_{SR}=10.1(15)mu_N^2, which is in excellent agreement with sum-rule estimates. The measured level density and gammaSF were used to calculate the 242Pu(n,gamma) cross section in a neutron energy range for which there were previously no measured data.

Recent progress in the development of novel organic scintillators necessitates modern characterization capabilities. As the primary means of energy deposition by neutrons in these materials is n-p elastic scattering, knowledge of the proton light yield is paramount. This work establishes a new model-independent method to continuously measure proton light yield in organic scintillators over a broad energy range. Using a deuteron breakup neutron source at the 88-Inch Cyclotron at Lawrence Berkeley National Laboratory and an array of organic scintillators, the proton light yield of EJ-301 and EJ-309, commercially available organic liquid scintillators from Eljen Technology, were measured via a double time-of-flight technique. The light yield was determined using a kinematically over-constrained system in the proton energy range of 1-20 MeV. The effect of pulse integration length on the magnitude and shape of the proton light yield relation was also explored. This work enables accurate simulation of the performance of advanced neutron detectors and supports the development of next-generation neutron imaging systems., 18 pages, 10 figures