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We derive a mesoscopic theory of the Josephson junction from non-relativistic scalar electrodynamics. Our theory reproduces the Josephson relations with the canonical current phase relation acquiring a weak second harmonic term, and it improves the standard lumped-element descriptions employed in circuit quantum electrodynamics by providing spatial resolution of the superconducting order parameter and electromagnetic field. By providing an ab initio derivation of the charge qubit Hamiltonian that relates traditionally free qubit parameters to geometric and material properties, we progress toward the quantum engineering of superconducting circuits at the subnanometer scale.

Model order reduction encompasses mathematical techniques aimed at reducing the complexity of mathematical models in simulations while retaining the essential characteristics and behaviors of the original model. This is particularly useful in the context of large-scale dynamical systems, which can be computationally expensive to analyze and simulate. Here, we present a model order reduction technique to reduce the time complexity of open quantum systems, grounded in the principle of measurement-adapted coarse-graining. This method, governed by a coarse-graining time scale $\tau$ and the spectral band center $\omega_0$, organizes corrections to the lowest-order model which aligns with the RWA Hamiltonian in certain limits, and rigorously justifies the resulting effective quantum master equation (EQME). The focus on calculating to a high degree of accuracy only what can be resolved by the measurement introduces a principled regularization procedure to address singularities and generates low-stiffness models suitable for efficient long-time integration. Furthermore, the availability of the analytical form of the EQME parameters significantly boosts the interpretive capabilities of the method. As a demonstration, we derive the fourth-order EQME for a challenging problem related to the dynamics of a superconducting qubit under high-power dispersive readout in the presence of a continuum of dissipative waveguide modes. This derivation shows that the lowest-order terms align with previous results, while higher-order corrections suggest new phenomena.

Although linear quantum amplification has proven essential to the processing of weak quantum signals, extracting higher-order quantum features such as correlations in principle demands nonlinear operations. However, nonlinear processing of quantum signals is often associated with non-idealities and excess noise, and absent a general framework to harness nonlinearity, such regimes are typically avoided. Here we present a framework to uncover general quantum signal processing principles of a broad class of bosonic quantum nonlinear processors (QNPs), inspired by a remarkably analogous paradigm in nature: the processing of environmental stimuli by nonlinear, noisy neural ensembles, to enable perception. Using a quantum-coherent description of a QNP monitoring a quantum signal source, we show that quantum nonlinearity can be harnessed to calculate higher-order features of an incident quantum signal, concentrating them into linearly-measurable observables, a transduction not possible using linear amplifiers. Secondly, QNPs provide coherent nonlinear control over quantum fluctuations including their own added noise, enabling noise suppression in an observable without suppressing transduced information, a paradigm that bears striking similarities to optimal neural codings that allow perception even under highly stochastic neural dynamics. Unlike the neural case, we show that QNP-engineered noise distributions can exhibit non-classical correlations, providing a new means to harness resources such as entanglement. Finally, we show that even simple QNPs in realistic measurement chains can provide enhancements of signal-to-noise ratio for practical tasks such as quantum state discrimination. Our work provides pathways to utilize nonlinear quantum systems as general computation devices, and enables a new paradigm for nonlinear quantum information processing., Comment: 25+39 pages, 10+7 figures, and 97 references

Many recent advancements in quantum computing leverage strong drives on nonlinear systems for state preparation, signal amplification, or gate operation. However, the interplay within such strongly driven system introduces multi-scale dynamics that affects the long-time behavior of the system in non-trivial ways that are very difficult to model. Therefore, the analysis of these systems often relies on effective Hamiltonian models that introduce additional nonlinear processes which approximate the long-time dynamics so that highly oscillatory terms may be ignored. However, the removal of such high frequency transitions can only be performed rigorously within a systematic framework of time-coarse graining, which is a fundamentally irreversible operation. This implies that standard approaches with unitary effective models cannot accurately capture the long-time behavior of strongly driven nonlinear quantum systems in general. We introduce a systematic perturbation theory for obtaining the complete non-unitary effective model of the time-coarse grained (TCG) dynamics of a driven quantum system to any order in the coupling strengths. We derive a closed-form analytical formula for both unitary and non-unitary contributions, in the form of an effective Hamiltonian and non-unitary (pseudo-)dissipators. Remarkably, even though the effective theory presumes unitary time evolution at the microscopic level, the time-coarse grained dynamics is found to follow a non-unitary time evolution in general. This occurs even when there is no open heat reservoir for the system to become entangled with or dissipate into. We demonstrate the effectiveness of the new method using several typical models of driven nonlinear systems in superconducting circuits, and show that it generalizes and improves on existing methods by providing more accurate results and explaining phenomena that have not been accounted for.

Practical implementation of many quantum algorithms known today is limited by the coherence time of the executing quantum hardware and quantum sampling noise. Here we present a machine learning algorithm, NISQRC, for qubit-based quantum systems that enables inference on temporal data over durations unconstrained by decoherence. NISQRC leverages mid-circuit measurements and deterministic reset operations to reduce circuit executions, while still maintaining an appropriate length persistent temporal memory in quantum system, confirmed through the proposed Volterra Series analysis. This enables NISQRC to overcome not only limitations imposed by finite coherence, but also information scrambling in monitored circuits and sampling noise, problems that persist even in hypothetical fault-tolerant quantum computers that have yet to be realized. To validate our approach, we consider the channel equalization task to recover test signal symbols that are subject to a distorting channel. Through simulations and experiments on a 7-qubit quantum processor we demonstrate that NISQRC can recover arbitrarily long test signals, not limited by coherence time., Comment: 15+17 pages, 4+7 figures

We develop and demonstrate a trainable temporal post-processor (TPP) harnessing a simple but versatile machine learning algorithm to provide optimal processing of quantum measurement data subject to arbitrary noise processes, for the readout of an arbitrary number of quantum states. We demonstrate the TPP on the essential task of qubit state readout, which has historically relied on temporal processing via matched filters in spite of their applicability only for specific noise conditions. Our results show that the TPP can reliably outperform standard filtering approaches under complex readout conditions, such as high power readout. Using simulations of quantum measurement noise sources, we show that this advantage relies on the TPP's ability to learn optimal linear filters that account for general quantum noise correlations in data, such as those due to quantum jumps, or correlated noise added by a phase-preserving quantum amplifier. Furthermore, we derive an exact analytic form for the optimal TPP weights: this positions the TPP as a linearly-scaling generalization of matched filtering, valid for an arbitrary number of states under the most general readout noise conditions, all while preserving a training complexity that is essentially negligible in comparison to that of training neural networks for processing temporal quantum measurement data. The TPP can be autonomously and reliably trained on measurement data and requires only linear operations, making it ideal for FPGA implementations in cQED for real-time processing of measurement data from general quantum systems., Comment: 15+24 pages, 6+9 figures, and 61 references; updated to published version

The accurate modeling of mode hybridization and calculation of radiative relaxation rates have been crucial to the design and optimization of superconducting quantum devices. In this work, we introduce a spectral theory for the electrohydrodynamics of superconductors that enables the extraction of the relaxation rates of excitations in a general three-dimensional distribution of superconducting bodies. Our approach addresses the long-standing problem of formulating a modal description of open systems that is both efficient and allows for second quantization of the radiative hybridized fields. This is achieved through the implementation of finite but transparent boundaries through which radiation can propagate into and out of the computational domain. The resulting spectral problem is defined within a coarse-grained formulation of the electrohydrodynamical equations that is suitable for the analysis of the non-equilibrium dynamics of multiscale superconducting quantum systems., Comment: 21 pages, 12 figures, journal paper

The expressive capacity of physical systems employed for learning is limited by the unavoidable presence of noise in their extracted outputs. Though present in physical systems across both the classical and quantum regimes, the precise impact of noise on learning remains poorly understood. Focusing on supervised learning, we present a mathematical framework for evaluating the resolvable expressive capacity (REC) of general physical systems under finite sampling noise, and provide a methodology for extracting its extrema, the eigentasks. Eigentasks are a native set of functions that a given physical system can approximate with minimal error. We show that the REC of a quantum system is limited by the fundamental theory of quantum measurement, and obtain a tight upper bound for the REC of any finitely-sampled physical system. We then provide empirical evidence that extracting low-noise eigentasks can lead to improved performance for machine learning tasks such as classification, displaying robustness to overfitting. We present analyses suggesting that correlations in the measured quantum system enhance learning capacity by reducing noise in eigentasks. The applicability of these results in practice is demonstrated with experiments on superconducting quantum processors. Our findings have broad implications for quantum machine learning and sensing applications., Comment: 37 pages, 10 figures, 1 table. Significantly expanded version of arXiv:2301.00042 [quant-ph], covering physical systems operating in the classical and quantum regimes

By applying a hydrodynamic representation of non-relativistic scalar electrodynamics to the superconducting order parameter, we predict a negative (attractive) pressure between planar superconducting bodies. For conventional superconductors with London penetration depth $\lambda_\text{L} \approx 100 \text{ nm}$, the pressure reaches tens of $\text{N/mm}^2$ at angstrom separations. The resulting surface energies are in better agreement with experimental values than those predicted by the Hartree-Fock theory, and the emergent electric-field screening length is comparable to that of the Thomas-Fermi theory. The model circumvents the bulk limitations of the Bardeen-Cooper-Schrieffer and Ginzburg-Landau theories to the analysis of superconducting quantum devices., Comment: 8 pages, 1 figure

Coherent multimode instabilities are responsible for several phenomena of recent interest in semiconductor lasers, such as the generation of frequency combs and ultrashort pulses. These techonologies have proven disruptive in optical telecommunications and spectroscopy applications. While the standard Maxwell-Bloch equations encompass such complex lasing phenomena, their integration is computationally expensive and offers limited analytical insight. In this paper, we demonstrate an efficient spectral approach to the simulation of multimode instabilities via a quantitative analysis of the instability of single-frequency lasing in ring lasers, referred to as the Lorenz-Haken (LH) instability or the Risken-Nummedal-Graham-Haken (RNGH) instability in distinct parameter regimes. Our approach, referred to as CFTD, uses generally non-Hermitian Constant Flux modes to obtain projected Time Domain equations. CFTD provides excellent agreement with finite-difference integration of the Maxwell-Bloch equations across a wide range of parameters in regimes of non-stationary inversion, including frequency comb formation and spatiotemporal chaos. We also develop a modal linear stability analysis using CFTD to efficiently predict multimode instabilities in lasers. The combination of numerical accuracy, speedup, and semi-analytic insight across a variety of dynamical regimes make the CFTD approach ideal to analyze multimode instabilities in lasers, especially in more complex geometries or coupled laser arrays., Comment: 20 pages, 11 figures, journal paper

The expressive capacity of quantum systems for machine learning is limited by quantum sampling noise incurred during measurement. Although it is generally believed that noise limits the resolvable capacity of quantum systems, the precise impact of noise on learning is not yet fully understood. We present a mathematical framework for evaluating the available expressive capacity of general quantum systems from a finite number of measurements, and provide a methodology for extracting the extrema of this capacity, its eigentasks. Eigentasks are a native set of functions that a given quantum system can approximate with minimal error. We show that extracting low-noise eigentasks leads to improved performance for machine learning tasks such as classification, displaying robustness to overfitting. We obtain a tight bound on the expressive capacity, and present analyses suggesting that correlations in the measured quantum system enhance learning capacity by reducing noise in eigentasks. These results are supported by experiments on superconducting quantum processors. Our findings have broad implications for quantum machine learning and sensing applications., Comment: 7 + 21 pages, 4 + 12 figures, 1 table

Modeling the behavior of superconducting electronic circuits containing Josephson junctions is crucial for the design of superconducting information processors and devices. In this paper, we introduce DEC-QED, a computational approach for modeling the electrodynamics of superconducting electronic circuits containing Josephson junctions in arbitrary three-dimensional electromagnetic environments. DEC-QED captures the non-linear response and induced currents in BCS superconductors and accurately captures phenomena such as the Meissner effect, flux quantization and Josephson effects. Using a spatial coarse-graining formulation based on Discrete Exterior Calculus (DEC), DEC-QED can accurately simulate transient and long-time dynamics in superconductors. The expression of the entire electrodynamic problem in terms of the gauge-invariant flux field and charges makes the resulting classical field theory suitable for second quantization.

We study the radiative properties -- the Lamb shift, Purcell decay rate and the spontaneous emission dynamics -- of an artificial atom coupled to a long, multimode cavity formed by an array of Josephson junctions. Introducing a tunable coupling element between the atom and the array, we demonstrate that such a system can exhibit a crossover from a perturbative to non-perturbative regime of light-matter interaction as one strengthens the coupling between the atom and the Josephson junction array (JJA). As a consequence, the concept of spontaneous emission as the occupation of the local atomic site being governed by a single complex-valued exponent breaks down. This breakdown, we show, can be interpreted in terms of formation of hybrid atom-resonator modes with radiative losses that are non-trivially related to the effective coupling between individual modes. We develop a singular function expansion approach for the description of the open quantum system dynamics in such a multimode non-perturbative regime. This modal framework generalizes the normal mode description of quantum fields in a finite volume, incorporating exact radiative losses and incident quantum noise at the delimiting surface. Our results are pertinent to recent experiments with Josephson atoms coupled to high impedance Josephson junction arrays.

The paradigm of reservoir computing exploits the nonlinear dynamics of a physical reservoir to perform complex time-series processing tasks such as speech recognition and forecasting. Unlike other machine-learning approaches, reservoir computing relaxes the need for optimization of intra-network parameters, and is thus particularly attractive for near-term hardware-efficient quantum implementations. However, the complete description of practical quantum reservoir computers requires accounting for their placement in a quantum measurement chain, and its conditional evolution under measurement. Consequently, training and inference has to be performed using finite samples from obtained measurement records. Here we describe a framework for reservoir computing with nonlinear quantum reservoirs under continuous heterodyne measurement. Using an efficient truncated-cumulants representation of the complete measurement chain enables us to sample stochastic measurement trajectories from reservoirs of several coupled nonlinear bosonic modes under strong excitation. This description also offers a mathematical basis to directly compare the computational capabilities of a given physical reservoir operated across classical and quantum regimes. Applying this framework to the classification of quantum states of systems that are part of the same measurement chain as the quantum reservoir computer, we assess and explain measurement-contingent advantages and disadvantages of reservoir processing in quantum regimes. Our results also identify the vicinity of bifurcation points as presenting optimal nonlinear processing regimes of an oscillator-based quantum reservoir. The considered models are directly realizable in modern circuit QED experiments, while the framework is applicable to more general quantum nonlinear reservoirs., Comment: 22+16 pages, 11+5 figures, and 80 references

Efficient quantum state measurement is important for maximizing the extracted information from a quantum system. For multi-qubit quantum processors in particular, the development of a scalable architecture for rapid and high-fidelity readout remains a critical unresolved problem. Here we propose reservoir computing as a resource-efficient solution to quantum measurement of superconducting multi-qubit systems. We consider a small network of Josephson parametric oscillators, which can be implemented with minimal device overhead and in the same platform as the measured quantum system. We theoretically analyze the operation of this Kerr network as a reservoir computer to classify stochastic time-dependent signals subject to quantum statistical features. We apply this reservoir computer to the task of multinomial classification of measurement trajectories from joint multi-qubit readout. For a two-qubit dispersive measurement under realistic conditions we demonstrate a classification fidelity reliably exceeding that of an optimal linear filter using only two to five reservoir nodes, while simultaneously requiring far less calibration data \textendash{} as little as a single measurement per state. We understand this remarkable performance through an analysis of the network dynamics and develop an intuitive picture of reservoir processing generally. Finally, we demonstrate how to operate this device to perform two-qubit state tomography and continuous parity monitoring with equal effectiveness and ease of calibration. This reservoir processor avoids computationally intensive training common to other deep learning frameworks and can be implemented as an integrated cryogenic superconducting device for low-latency processing of quantum signals on the computational edge., Comment: 17 pages, 9 figures, and 57 references

While coherently-driven Kerr microcavities have rapidly matured as a platform for frequency comb formation, such microresonators generally possess weak Kerr coefficients; consequently, triggering comb generation requires millions of photons to be circulating inside the cavity. This suppresses the role of quantum fluctuations in the comb's dynamics. In this paper, we realize a minimal version of coherently-driven Kerr-mediated microwave frequency combs in the circuit QED architecture, where the quantum vacuum's fluctuations are the primary limitation on comb coherence. We achieve a comb phase coherence of up to 35~$\mu$s, approaching the theoretical device quantum limit of 55~$\mu$s, and vastly longer than the modes' inherent lifetimes of 13~ns. The ability within cQED to engineer stronger nonlinearities than optical microresonators, together with operation at cryogenic temperatures, and excellent agreement of comb dynamics with quantum theory indicates a promising platform for the study of complex dynamics of quantum nonlinear systems

Recent experiments in superconducting qubit systems have shown an unexpectedly strong dependence of the qubit relaxation rate on the readout drive power. This phenomenon limits the maximum measurement strength and thus the achievable readout speed and fidelity. We address this problem here and provide a plausible mechanism for drive-power dependence of relaxation rates. To this end we introduce a two-parameter perturbative expansion in qubit anharmonicity and the drive amplitude through a unitary transformation technique introduced in Part I. This approach naturally reveals number non-conserving terms in the Josephson potential as a fundamental mechanism through which applied microwave drives can activate additional relaxation mechanisms. We present our results in terms of an effective master equation with renormalized state- and drive-dependent transition frequency and relaxation rates. Comparison of numerical results from this effective master equation to those obtained from a Lindblad master equation which only includes number-conserving terms (i.e. Kerr interactions) shows that number non-conserving terms can lead to significant drive-power dependence of the relaxation rates. The systematic expansion technique introduced here is of general applicability to obtaining effective master equations for driven-dissipative quantum systems that contain weakly non-linear degrees of freedom., Comment: 28 pages, 6 figures, 4 tables

The dynamics of a weakly anharmonic superconducting qubit in a complex electromagnetic environment is generally well-described by an effective multimode Kerr Hamiltonian at sufficiently weak excitation. This Hamiltonian can be embedded in a master equation with losses determined by the details of the electromagnetic environment. Recent experiments indicate, however, that when a superconducting circuit is driven with microwave signals the observed relaxation rates appear to be substantially different from expectations based on the electromagnetic environment of the qubit alone. This issue is a limiting factor in the optimization of superconducting qubit readout schemes. We claim here that an effective master equation with drive-power dependent parameters is an efficient approach to model such quantum dynamics. In this sequence of papers, we derive effective master equations, whose parameters exhibit nonlinear dependence on the excitation level of the circuit as well as the electromagnetic environment of the qubit. We show that the number non-conserving terms in the qubit nonlinearity generally lead to a renormalization of dissipative parameters of the effective master equation, while the number conserving terms give rise to a renormalization of the system frequencies. Here, in Part I, we consider the excitation-relaxation dynamics of a transmon qubit that is prepared in a certain initial state, but is not driven otherwise. A unitary transformation technique is introduced to study the renormalization of i) qubit relaxation due to coupling to a generic bath and ii) Purcell decay. Analytic expressions are provided for the dependence of the nonlinear dissipative terms on the details of the electromagnetic environment of the qubit. The perturbation technique based on unitary transformations developed here is generalized to the continuously driven case in Part II., Comment: 20 pages, 5 figures, 4 tables and 38 references

Long-lived fluxon excitations can be trapped inside a superinductor ring, which is divided into an array of loops by a periodic sequence of Josephson junctions in the quantum regime, thereby allowing fluxons to tunnel between neighboring sites. By tuning the Josephson couplings, and implicitly the fluxon tunneling probability amplitudes, a wide class of 1D tight-binding lattice models may be implemented and populated with a stable number of fluxons. We illustrate the use of this quantum simulation platform by discussing the Su-Schrieffer-Heeger model in the 1-fluxon subspace, which hosts a symmetry protected topological phase with fractionally charged bound states at the edges. This pair of localized edge states could be used to implement a superconducting qubit increasingly decoupled from decoherence mechanisms., Comment: 13 pages, 7 figures

We investigate the dynamics of a microwave-driven Josephson junction capacitively coupled to a lumped element LC oscillator. In the regime of driving where the Josephson junction can be approximated as a Kerr oscillator, this minimal nonlinear system has been previously shown to exhibit a bistability in phase and amplitude. In the present study, we characterize the full phase diagram and show that besides a parameter regime exhibiting bistability, there is also a regime of self-oscillations characterized by a frequency comb in its spectrum. We discuss the mechanism of comb generation which appears to be different from those studied in microcavity frequency combs and mode-locked lasers. We then address the fate of the comb-like spectrum in the regime of strong quantum fluctuations, reached when nonlinearity becomes the dominant scale with respect to dissipation. We find that the nonlinearity responsible for the emergence of the frequency combs also leads to its dephasing, leading to broadening and ultimate disappearance of sharp spectral peaks. Our study explores the fundamental question of the impact of quantum fluctuations for quantum systems which do not possess a stable fixed point in the classical limit., Comment: 5+17 pages, 4+9 figures; updated to published version

The process of photosynthesis, the main source of energy in the animate world, converts sunlight into chemical energy. The surprisingly high efficiency of this process is believed to be enabled by an intricate interplay between the quantum nature of molecular structures in photosynthetic complexes and their interaction with the environment. Investigating these effects in biological samples is challenging due to their complex and disordered structure. Here we experimentally demonstrate a new approach for studying photosynthetic models based on superconducting quantum circuits. In particular, we demonstrate the unprecedented versatility and control of our method in an engineered three-site model of a pigment protein complex with realistic parameters scaled down in energy by a factor of $10^5$. With this system we show that the excitation transport between quantum coherent sites disordered in energy can be enabled through the interaction with environmental noise. We also show that the efficiency of the process is maximized for structured noise resembling intramolecular phononic environments found in photosynthetic complexes., Comment: 8+12 pages, 4+12 figures

Any quantum-confined electronic system coupled to the electromagnetic continuum is subject to radiative decay and renormalization of its energy levels. When coupled to a cavity, these quantities can be strongly modified with respect to their values in vacuum. Generally, this modification can be accurately captured by including only the closest resonant mode of the cavity. In the circuit quantum electrodynamics architecture, where the coupling strengths can be substantial, it is however found that the radiative decay rates are strongly influenced by far off-resonant modes. A multimode calculation accounting for the infinite set of cavity modes leads to divergences unless a cutoff is imposed. It has so far not been identified what the source of divergence is. We show here that unless gauge invariance is respected, any attempt at the calculation of circuit QED quantities is bound to diverge. We then present a theoretical approach to the calculation of a finite spontaneous emission rate and the Lamb shift that is free of cutoff., Comment: 13 pages, 3 figures. Revised sections I,II and IV of the Supplementary Material rely on and summarize formalism developed in 1609.00359

We present a theoretical study of synchronization dynamics in incoherently pumped exciton-polariton condensates in coupled polariton traps. Our analysis is based on a coupled-mode theory for the generalized Gross-Pitaevskii equation, which employs an expansion in non-Hermitian, pump-dependent modes appropriate for the pumped geometry. We find that polariton-polariton and reservoir-polariton interactions play competing roles and lead to qualitatively different synchronized phases of the coupled polariton modes as pumping power is increased. Crucially, these interactions can also act against each other to hinder synchronization. We map out a phase diagram and discuss the general characteristics of these phases using a generalized Adler equation., Comment: 16 pages, 10 figures, updated to published version

We study the dynamics of a transmon qubit that is capacitively coupled to an open multimode superconducting resonator. Our effective equations are derived by eliminating resonator degrees of freedom while encoding their effect in the Green's function of the electromagnetic background. We account for the dissipation of the resonator exactly by employing a spectral representation for the Green's function in terms of a set of non-Hermitian modes and show that it is possible to derive effective Heisenberg-Langevin equations without resorting to the rotating wave, two level or Markov approximations. A well-behaved time domain perturbation theory is derived to systematically account for the nonlinearity of the transmon. We apply this method to the problem of spontaneous emission, capturing accurately the non-Markovian features of the qubit dynamics, valid for any qubit-resonator coupling strength., Comment: 30 pages, 13 figures

The generalized Gross-Pitaevskii equation (gGPE) is an effective phenomenological description for the dynamics of incoherently pumped exciton-polariton condensates. However, a brute force numerical simulation of the gGPE provides little physical insight into condensate formation under arbitrary pumping configurations, and is demanding in terms of computational resources. We introduce in this paper a modal description of polariton condensation under incoherent pumping of arbitrary spatial profile, based on eigenmodes of the non-Hermitian generator of the linearized dynamics. A pump-dependent basis is then introduced to formulate a temporal coupled-mode theory that captures condensate dynamics in the presence of all nonlinear interactions. Simulations using a single set of modes for a given pumping and trapping configuration agree very well with a full integration of the gGPE in diverse dynamical regimes, supporting the validity of this modal description, while also providing a speedup in simulation times., Comment: 17 pages, 12 figures; updated to published version

Pure dephasing processes limit the fidelities achievable in driven-dissipative schemes for stabilization of entangled states of qubits. We propose a scheme which, combined with already existing entangling methods, purifies the desired entangled state by driving out of equilibrium auxiliary dissipative cavity modes coupled to the qubits. We lay out the specifics of our scheme and compute its efficiency in the particular context of two superconducting qubits in a cavity-QED architecture, where the strongly coupled auxiliary modes provided by collective cavity excitations can drive and sustain the qubits in maximally entangled Bell states with fidelities reaching 90% for experimentally accessible parameters., Comment: 11 pages, 7 figures

We propose and study the use of photon-mediated interactions for the generation of long-range steady-state entanglement between N atoms. Through the judicious use of coherent drives and the placement of the atoms in a network of Cavity QED systems, a balance between their unitary and dissipative dynamics can be precisely engineered to stabilize a long-range correlated state of qubits in the steady state. We discuss the general theory behind such a scheme, and present an example of how it can be used to drive a register of N atoms to a generalized W state and how the entanglement can be sustained indefinitely. The achievable steady-state fidelities for entanglement and its scaling with the number of qubits are discussed for presently existing superconducting quantum circuits. While the protocol is primarily discussed for a superconducting circuit architecture, it is ideally realized in any Cavity QED platform that permits controllable delivery of coherent electromagnetic radiation to specified locations., Comment: 9 pages, 6 figures

The quantum dynamics of open many-body systems poses a challenge for computational approaches. Here we develop a stochastic scheme based on the positive P phase-space representation to study the nonequilibrium dynamics of coupled spin-boson networks that are driven and dissipative. Such problems are at the forefront of experimental research in cavity and solid state realizations of quantum optics, as well as cold atom physics, trapped ions and superconducting circuits. We demonstrate and test our method on a driven, dissipative two-site system, each site involving a spin coupled to a photonic mode, with photons hopping between the sites, where we find good agreement with Monte Carlo Wavefunction simulations. In addition to numerically reproducing features recently observed in an experiment [Phys. Rev. X 4, 031043 (2014)], we also predict a novel steady state quantum dynamical phase transition for an asymmetric configuration of drive and dissipation., Comment: 15 pages, 8 figures

We propose a scheme for driving a dimer of spatially separated qubits into a maximally entangled non-equilibrium steady state. A photon-mediated retarded interaction between the qubits is realized by coupling them to two tunnel-coupled leaky cavities where each cavity is driven by a coherent microwave tone. The proposed cooling mechanism relies on striking the right balance between the unitary and driven-dissipative dynamics of the qubit subsystem. We map the dimer to an effective transverse-field XY model coupled to a non-equilibrium bath that can be suitably engineered through the choice of drive frequencies and amplitudes. We show that both singlet and triplet states can be obtained with remarkable fidelities. The proposed protocol can be implemented with a superconducting circuit architecture that was recently experimentally realized and paves the way to achieving large-scale entangled systems that are arbitrarily long lived., Comment: 5 pages, 3 figures. Published version

We present a theoretical and experimental study of photonic and electronic transport properties of a voltage biased InAs semiconductor double quantum dot (DQD) that is dipole-coupled to a superconducting transmission line resonator. We obtain the Master equation for the reduced density matrix of the coupled system of cavity photons and DQD electrons accounting systematically for both the presence of phonons and the effect of leads at finite voltage bias. We subsequently derive analytical expressions for transmission, phase response, photon number and the non-equilibrium steady state electron current. We show that the coupled system under finite bias realizes an unconventional version of a single-atom laser and analyze the spectrum and the statistics of the photon flux leaving the cavity. In the transmission mode, the system behaves as a saturable single-atom amplifier for the incoming photon flux. Finally, we show that the back action of the photon emission on the steady-state current can be substantial. Our analytical results are compared to exact Master equation results establishing regimes of validity of various analytical models. We compare our findings to available experimental measurements., Comment: 13 pages, 9 Figures, 1 Table

We report here the experimental observation of a dynamical quantum phase transition in a strongly interacting open photonic system. The system studied, comprising a Jaynes-Cummings dimer realized on a superconducting circuit platform, exhibits a dissipation driven localization transition. Signatures of the transition in the homodyne signal and photon number reveal this transition to be from a regime of classical oscillations into a macroscopically self-trapped state manifesting revivals, a fundamentally quantum phenomenon. This experiment also demonstrates a small-scale realization of a new class of quantum simulator, whose well controlled coherent and dissipative dynamics is suited to the study of quantum many-body phenomena out of equilibrium., Comment: 34 pages, 13 figures, includes supplementary material; significant additions to theory sections

We investigate the single-photon transport properties of a one-dimensional coupled cavity array (CCA) containing a single qubit in its central site by coupling the CCA to two transmission lines supporting propagating bosonic modes with linear dispersion. We find that even in the nominally weak light-matter coupling regime, the transmission through a long array exhibits two ultra-narrow resonances corresponding to long-lived self-protected polaritonic states localized around the site containing the qubit. The lifetime of these states is found to increase exponentially with the number of array sites in sharp distinction to the polaritonic Bloch modes of the cavity array., Comment: 4 pages, 4 figures

We investigate the near-critical dynamics of atomic density fluctuations in the non-equilibrium self-organization transition of an optically driven quantum gas coupled to a single mode of a cavity. In this system cavity-mediated long-range interactions between atoms, tunable by the drive strength, lead to softening of an excitation mode recently observed in experiments. This phenomenon has previously been studied within a two-mode approximation for the collective motional degrees of freedom of the atomic condensate which results in an effective open-system Dicke model. Here, including the full spectrum of atomic modes we find a finite lifetime for a roton-like mode in the Bogoliubov excitation spectrum that is strongly pump-dependent. The corresponding decay rate and critical exponents for the phase-transition are calculated explaining the non-monotonic pump-dependent atomic damping rate observed in recent experiments. We compute the near-critical behavior of the intra-cavity field fluctuations, that has been previously shown to be enhanced with respect to the equilibrium Dicke model in a two-mode approximation. We highlight the role of the finite size of the system in the suppression of it below the expectations of the open Dicke model., Comment: 6 pages, 6 figures

We study the coherence and fluorescence properties of the coherently pumped and dissipative Jaynes-Cummings-Hubbard model describing polaritons in a coupled-cavity array. At weak hopping we find strong signatures of photon blockade similar to single-cavity systems. At strong hopping the state of the photons in the array depends on its size. While the photon blockade persists in a dimer consisting of two coupled cavities, a coherent state forms on an extended lattice, which can be described in terms of a semi-classical model.

The interaction between a single confined spin and the spins of a Fermionic reservoir leads to one of the most spectacular phenomena of many body physics -- the Kondo effect. Here we report the observation of Kondo correlations in optical absorption measurements on a single semiconductor quantum dot tunnel-coupled to a degenerate electron gas. In stark contrast to transport experiments, absorption of a single photon leads to an abrupt change in the system Hamiltonian and a quantum quench of Kondo correlations. By inferring the characteristic power law exponents from the experimental absorption line-shapes, we find a unique signature of the quench in the form of an Anderson orthogonality catastrophe, originating from a vanishing overlap between the initial and final many-body wave-functions. We also show that the power-law exponents that determine the degree of orthogonality can be tuned by applying an external magnetic field which gradually turns the Kondo correlations off. Our experiments demonstrate that optical measurements on single artificial atoms offer new perspectives on many-body phenomena previously studied exclusively using transport spectroscopy. Moreover, they initiate a new paradigm for quantum optics where many-body physics influences electric field and intensity correlations.

We show that coherent optical manipulation of a single confined spin is possible even in the absence of spin-orbit coupling. To this end, we consider the non-Markovian dynamics of a single valence orbital hole spin that has optically induced spin exchange coupling to a low temperature partially polarized electron gas. We show that the fermionic nature of the reservoir induces a coherent component to the hole spin dynamics that does not generate entanglement with the reservoir modes. We analyze in detail the competition of this reservoir-assisted coherent contribution with dissipative components displaying markedly different behavior at different time scales and determine the fidelity of optically controlled spin rotations., Comment: 4 pages, 3 figures

A single confined spin interacting with a solid-state environment has emerged as one of the fundamental paradigms of mesoscopic physics. In contrast to standard quantum optical systems, decoherence that stems from these interactions can in general not be treated using the Born-Markov approximation at low temperatures. Here we study the non-equilibrium dynamics of a single-spin in a semiconductor quantum dot adjacent to a fermionic reservoir and show how the dynamics can be revealed in detail in an optical absorption experiment. We show that the highly asymmetrical optical absorption lineshape of the resulting Kondo exciton consists of three distinct frequency domains, corresponding to short, intermediate and long times after the initial excitation, which are in turn described by the three fixed points of the single-impurity Anderson Hamiltonian. The zero-temperature power-law singularity dominating the lineshape is linked to dynamically generated Kondo correlations in the photo-excited state. We show that this power-law singularity is tunable with gate voltage and magnetic field, and universal., Comment: 15 pages, 10 figures

We review our recent work leading to steady-state solutions of the semiclassical (Maxwell-Bloch) equations of a laser. These are coupled non-linear partial differential equations in space and time which have previously been solved either by fully time-dependent numerical simulations or by using major approximations which neglect non-linear modal interactions and/or the openness of the laser system. We have found a time-independent technique for determining these stationary solutions which can treat lasers of arbitrary complexity and degree of openness. Our method has been shown to agree with time-dependent numerical solutions to high accuracy and has been applied to find the electric field patterns (lasing modes) of random lasers, which lack a laser cavity and are so strongly damped that the linear system has no detectable resonances. Our work provides a link between an important non-linear wave system and the field of quantum/wave chaos in linear systems., Comment: 22 pages, 10 figures, final version, selected for the cover illustration of the journal Nonlinearity in 2009

We generalize and test the recent "ab initio" self-consistent (AISC) time-independent semiclassical laser theory. This self-consistent formalism generates all the stationary lasing properties in the multimode regime (frequencies, thresholds, internal and external fields, output power and emission pattern) from simple inputs: the dielectric function of the passive cavity, the atomic transition frequency, and the transverse relaxation time of the lasing transition. We find that the theory gives excellent quantitative agreement with full time-dependent simulations of the Maxwell-Bloch equations after it has been generalized to drop the slowly-varying envelope approximation. The theory is infinite order in the non-linear hole-burning interaction; the widely used third order approximation is shown to fail badly., Comment: 8 pages, 4 figures

Unlike conventional lasers, diffusive random lasers (DRLs) have no resonator to trap light and no high-Q resonances to support lasing. Due to this lack of sharp resonances the DRL has presented a challenge to conventional laser theory. We present a theory able to treat the DRL rigorously, and provide results on the lasing spectra, internal fields and output intensities of DRLs. Typically DRLs are highly multimode lasers, emitting light at a number of wavelengths. We show that the modal interactions through the gain medium in such lasers are extremely strong and lead to a uniformly spaced frequency spectrum, in agreement with recent experimental observations., Comment: 13 pages, 4 figures. Supplementary information available at arXiv:0805.4497

We study a mesoscopic interacting quantum dot described by the "universal Hamiltonian" that is coupled to a Kondo spin. The ferromagnetic exchange interaction within the dot leads to a stepwise increase of the ground state spin; this Stoner staircase is modified non-trivially by the Kondo interaction. We find that the spin-transition steps move to lower values of the exchange coupling for weak Kondo interaction, but shift back up for sufficiently strong Kondo coupling. The problem is solved numerically by diagonalizing the system Hamiltonian in a customized good-spin basis and analytically in the weak and strong Kondo coupling limits. The interplay of Kondo and ferromagnetic exchange can be probed with experimentally tunable parameters., Comment: 4 pages, 3 figures

We demonstrate that electron-phonon interaction in quantum dots embedded in one-dimensional systems leads to pronounced, non-Markovian decoherence of optical transitions. The experiments we present focus on the lineshape of photoluminescence from low-temperature axially localized carbon nanotube excitons. The independent boson model that we use to model the phonon interactions reproduces with very high accuracy the broad and asymmetric emission lines and the weak red-detuned radial breathing mode replicas observed in the experiments. The intrinsic phonon-induced pure-dephasing of the zero-phonon line is two orders of magnitude larger than the lifetime broadening and is a hallmark of the reduced dimensionality of the phonon bath. The non-Markovian nature of this decoherence mechanism may have adverse consequences for applications of one-dimensional systems in quantum information processing., Comment: 4 pages, 3 figures

We show that spin-orbit coupling in a quantum dot molecule allows for coherent manipulation of two electron spin states using Raman transitions. Such two-electron spin states defined by the singlet and triplet states of two exchange coupled quantum dots can have favorable coherence properties. In addition, two of the four metastable ground states in this system can be used as auxiliary states that could facilitate implementation of tasks such as mapping of spin states to that of a single propagating photon. We find that even weak spin-orbit effects -- manifesting themselves as slightly different g-factors for the electron and the hole -- would allow for the coherent Raman coupling of the singlet-triplet states. We also discuss the possibilities for implementing quantum optical techniques for spin preparation and manipulation., Comment: 8 pages, 6 figures

A self-consistent integral equation is formulated and solved iteratively which determines the steady-state lasing modes of open multi-mode lasers. These modes are naturally decomposed in terms of frequency dependent biorthogonal modes of a linear wave equation and not in terms of resonances of the cold cavity. A one-dimensional cavity laser is analyzed and the lasing mode is found to have non-trivial spatial structure even in the single-mode limit. In the multi-mode regime spatial hole-burning and mode competition is treated exactly. The formalism generalizes to complex, chaotic and random laser media., Comment: 4 pages, 3 figures