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We demonstrate a chip-integrated emission spectroscope capable of retrieving the temperature of the light sources. It consists of a single photon detector with low dark counts and a sweeping on-chip filter with 2 pm spectral resolution in the visible and near-infrared regimes. With wildfire sensing applications in mind, we test our system with a hollow cathode lamp to simulate the K-line emission, and show how the models of Doppler and collision broadening in the plasma can be used for temperature retrieval. With favorable device parameters, high spectral resolution, and a novel temperature retrieval capability, our technique may find broad applications in environmental monitoring, astrophysics, plasma physics, and so on., Comment: 12 pages, 13 figures

Modern quantum technologies using matter are designed as closed quantum systems to isolate them from interactions with the environment. This design paradigm greatly constrains the scalability and limits practical implementation of such systems. Here, we introduce a novel computing paradigm, entropy computing, that works by conditioning a quantum reservoir thereby enabling the stabilization of a ground state. In this work, we experimentally demonstrate the feasibility of entropy computing by building a hybrid photonic-electronic computer that uses measurement-based feedback to solve non-convex optimization problems. The system functions by using temporal photonic modes to create qudits in order to encode probability amplitudes in the time-frequency degree of freedom of a photon. This scheme, when coupled with electronic interconnects, allows us to encode an arbitrary Hamiltonian into the system and solve non-convex continuous variables and combinatorial optimization problems. We show that the proposed entropy computing paradigm can act as a scalable and versatile platform for tackling a large range of NP-hard optimization problems.

We demonstrate parametric all-optical modulation in a periodically-poled lithium niobate microring resonator on chip. It employs quantum Zeno blockade between two distinct waves, a signal and a pump, through their sum-frequency generation at a large per-photon efficiency of 8.2 MHz. With nanosecond pump pulses at 6 mW peak power, 85.7% modulation extinction is observed, marking over 30~times efficiency improvement across various previous implementations. With only 2 mW pump peak power, 43.0% modulation extinction is observed for a doubly-stronger signal at 4 mW. This demonstrates, for the first time, that optical transistors with cascadability and fan-out are possible with just parametric nonlinear optics. These results, together with inherent advantages in such photonic integrated circuits, open the door to scalable technology for all-optical and quantum information processing.

We report on multi-photon statistics of correlated twin beams produced in a periodic poled micro-ring resonator on thin-film lithium niobate. Owing to high cavity confinement and near perfect quasi-phase matching, the photons pairs are produced efficiently in single modes at rates reaching 27 MHz per $\mu$W pump power. By using a pump laser whose pulse width impedance matches with the cavity, those photons are further created in single longitudinal modes with purity reaching 99\%, without relying on later-on filtering. With a dual-channel photon-number resolving detection system, we obtain directly the joint detection probabilities of multi-photon states up to three photons, with high coincidence to accidental contrast for each. Used as a single photon source, it gives heralded $g_H^{(2)}(0)$ around 0.04 at a single photon rate of 650 kHz on chip. The findings of our research highlight the potential of this nanophotonic platform as a promising platform for generating non-classical, few-photon states with ideal indistinguishability, for fundamental quantum optics studies and information applications., Comment: 7 pages

We demonstrate a photon-sensitive, three-dimensional camera by active near-infrared illumination and fast time-of-flight gating. It uses pico-second pump pulses to selectively up-convert the backscattered photons according to their spatiotemporal modes via sum-frequency generation in a \c{hi}2 nonlinear crystal, which are then detected by electron-multiplying CCD with photon sensitive detection. As such, it achieves sub-millimeter depth resolution, exceptional noise suppression, and high detection sensitivity. Our results show that it can accurately reconstruct the surface profiles of occluded targets placed behind highly scattering and lossy obscurants of 14 optical depth (round trip), using only milliwatt illumination power. This technique may find applications in biomedical imaging, environmental monitoring, and wide-field light detection and ranging, Comment: 8 pages, 7 figures

We experimentally demonstrate a programmable parametric mode sorter of high-dimensional signals in a composite spatiotemporal Hilbert space through mode-selective quantum frequency up-conversion. As a concrete example and with quantum communication applications in mind, we consider the Laguerre-Gaussian and Hermite-Gaussian modes as the spatial and temporal state basis for the signals, respectively. By modulating the spatiotemporal profiles of the up-conversion pump, we demonstrate the faithful selection of single photons in those modes and their superposition modes. Our results show an improvement in the quantum mode-sorting performance by coupling the up-converted light into a single-mode fiber and/or operating the upconversion at the edge of phase matching. By optimizing pump temporal profiles only, we achieve more than 12 dB extinction for mutually unbiased basis (MUB) sets of the spatiotemporal modes. This fully programmable and efficient system could serve as a viable resource for quantum communications, quantum computation, and quantum metrology., Comment: 25 pages, 7 Figures

Quantum random number (QRNG) beacons distinguish themselves from classical counterparts by providing intrinsic unpredictability originating from the fundamental laws of quantum mechanics. Most demonstrations have focused on certifiable randomness generators to guarantee the public that their genuineness is independent from imperfect implementations. These efforts however do not benefit applications where multiple distrusted users need a common set of random numbers, as they must rely on the honesty of beacon owners. In this paper, we formally introduce a design and proof-of-principle experiment of the first consensus protocol producing QRNs in a decentralized environment (dQRNG). Such protocol allows N number of participants contribute in the generation process and publicly verify numbers they collect. Security of the protocol is guaranteed given(N-1) dishonest participants. Our method is thus suited for distribute systems that requires a bias-resistant, highly secure, and public-verifiable random beacon., Comment: 9 pages, 9 figures, poster presented at Quantum Cryptography conference QCrypt 2021

Non-line-of-sight (NLOS) optical imaging and sensing of objects imply new capabilities valuable to autonomous technology, machine vision, and other applications. Existing NLOS imaging methods rely heavily on the prowess of computational algorithms to reconstruct the images from weak triply scattered signals. Here, we introduce a new approach to NLOS imaging and sensing using the picosecond gated single photon detection generated by quantum frequency conversion. With exceptional signal isolation, this approach can reliably sense obscured objects around the corner and substantially simplify the data processing needed for position retrieval and surface profiling. For each pixel, only $4 \times 10^{-3}$ photons are needed to be detected per pulse to position and profile occluded objects with high resolution. Furthermore, the vibration frequencies of different objects can be resolved by analyzing the photon number fluctuation received within in a ten-picosecond window, allowing NLOS acoustic sensing. Our results highlight the prospect of photon efficient NLOS imaging and sensing for real-world applications.

We experimentally demonstrate a mode-selective quantum frequency converter over a compound spatio-temporal Hilbert space. We show that our method can achieve high-extinction for high-dimensional quantum state tomography by selectively upconverting the signal modes with a modulated and delayed pump. By preparing the pump in optimized modes through adaptive feedback control, selective frequency conversion is demonstrated with up to 30 dB extinction. The simultaneous operations over high-dimensional degrees of freedom in both spatial and temporal domains can serve as a viable resource for photon-efficient quantum communications and computation., Comment: 9 pages, 11 figures

The conversion and interaction between quantum signals at a single-photon level are essential for scalable quantum photonic information technology. Using a fully-optimized, periodically-poled lithium niobate microring, we demonstrate ultra-efficient sum-frequency generation on chip. The external quantum efficiency reaches $(65\pm3)\%$ with only $(104\pm4)$ $\mu$W pump power, improving the state-of-the-art by over one order of magnitude. At the peak conversion, $3\times10^{-5}$ noise photon is created during the cavity lifetime, which meets the requirement of quantum applications using single-photon pulses. Using pump and signal in single-photon coherent states, we directly measure the conversion probability produced by a single pump photon to be $10^{-5}$ -- breaking the record by 100 times -- and the photon-photon coupling strength to be 9.1 MHz. Our results mark a new milestone toward quantum nonlinear optics at the ultimate single photon limit, creating new background in highly integrated photonics and quantum optical computing., Comment: 11 pages, 6 figures, email: jchen59@stevens.edu & yhuang5@stevens.edu

We propose and demonstrate a single-photon sensitive technique for optical vibrometry. It uses high speed photon counting to sample the modulated backscattering from a vibrating target. Designed for remote vibration sensing with ultralow photon flux, we show that this technique can detect small displacements down to 110 nm and resolve vibration frequencies from DC up to several kilohertz, with less than 0.01 detected photons per pulse. This single-photon sensitive optical vibrometry may find important applications in acousto-optic sensing and imaging, especially in photon-starved environments.

Thin-film lithium niobate (TFLN) is superior for integrated nanophotonics due to its outstanding properties in nearly all aspects: strong second-order nonlinearity, fast and efficient electro-optic effects, wide transparency window, and little two photon absorption and free carrier scattering. Together, they permit highly integrated nanophotonic circuits capable of complex photonic processing by incorporating disparate elements on the same chip. Yet, there has to be a demonstration that synergizes those superior properties for system advantage. Here we demonstrate such a chip that capitalizes on TFLNs favorable ferroelectricity, high second-order nonlinearity, and strong electro-optic effects. It consists of a monolithic circuit integrating a Z-cut, quasi-phase matched microring with high quality factor and a phase modulator used in active feedback control. By Pound-Drever-Hall locking, it realizes stable frequency doubling at about 50% conversion with only milliwatt pump, marking the highest by far among all nanophotonic platforms with milliwatt pumping. Our demonstration addresses a long-outstanding challenge facing cavity-based optical processing, including frequency conversion, frequency comb generation, and all-optical switching, whose stable performance is hindered by photorefractive or thermal effects. Our results further establish TFLN as an excellent material capable of optical multitasking, as desirable to build multi-functional chip devices., Comment: 11 pages, 6 figures, jchen59@stevens.edu yhuang5@stevens.edu

Quantum photon sources of high rate, brightness, and purity are increasingly desirable as quantum information systems are quickly scaled up and applied to many fields. Using a periodically poled lithium niobate microresonator on chip, we demonstrate photon-pair generation at high rates of 8.5 MHz and 36.3 MHz using only 3.4-$\mu$W and 13.4-$\mu$W pump power, respectively, marking orders of magnitude improvement over the state-of-the-art. The measured coincidence to accidental ratio is well above 100 at those high rates and reaches $14,682\pm 4427$ at a lower pump power. The same chip enables heralded single-photon generation at tens of megahertz rates, each with low auto-correlation $g^{(2)}_{H}(0)=0.008$ and $0.097$ for the microwatt pumps. Such distinct performance, facilitated by the chip device's noiseless and giant optical nonlinearity, will contribute to the forthcoming pervasive adoption of quantum optical information technologies., Comment: 5 pages, 3 figures

Thin-film lithium niobate on insulator (LNOI) has emerged as a superior integrated-photonics platform for linear, nonlinear, and electro-optics. Here we combine quasi-phase-matching, dispersion engineering, and tight mode confinement to realize nonlinear parametric processes with both high efficiency and wide wavelength tunability. On a millimeter-long, Z-cut LNOI waveguide, we demonstrate ultra-efficient ($1900\pm500 \% $W$^{-1}$cm$^{-2}$) and highly tunable (-1.71 nm/K) second-harmonic generation from 1530 to 1583 nm by type-0 quasi-phase-matching. Our technique is applicable to optical harmonic generation, quantum light sources, frequency conversion, and many other photonic information processing across visible to mid-IR spectral bands.

We demonstrate efficient second harmonic generation in a quasi-phase-matched, high quality factor ($Q_0 \approx 5.3\times 10^5$) racetrack microresonator. The observed normalized conversion efficiency is about $3.8\%~mW^{-1}$.

Chip-integrated nonlinear photonics holds the key for advanced optical information processing with superior performance and novel functionalities. Here, we present an optimally mode-matched, periodically poled lithium niobate nanowaveguide for efficient parametric frequency conversions on chip. Using a 4-mm nanowaveguide with subwavelength mode confinement, we demonstrate second harmonic generation with efficiency over $2200\%~W^{-1}cm^{-2}$, and broadband difference frequency generation with similar efficiency over a 4.5-THz spectral span. These allow us to generate correlated photon pairs over multiple frequency channels via spontaneous parametric down conversion, all in their fundamental spatial modes, with a coincidence to accidental ratio as high as 600. The high efficiency and dense integrability of the present chip devices may pave a viable route to scalable nonlinear applications in both classical and quantum domains.

With exotic propagation properties, optical Airy beams have been well studied for innovative applications in communications, biomedical imaging, micromachining, and so on. Here we extend those studies to the quantum domain, creating quantum correlated photons in finite-energy Airy transverse modes via spontaneous parametric down conversion and sub-sequential spatial light modulation. Through two-photon coincidence measurements, we verify their Airy spatial wavefunctions, propagation along a parabolic trajectory, and that the spatial modulation does not introduce any observable degradation of quantum correlation between the photons. These results suggest the feasibility of using spatially structured photons for practically advantageous quantum applications., Comment: 6 pages, 4 figures

Quantum correlated, highly non-degenerate photons can be used to synthesize disparate quantum nodes and link quantum processing over incompatible wavelengths, thereby constructing heterogeneous quantum systems for otherwise unattainable superior performance. Existing techniques for correlated photons have been concentrated in the visible and near-IR domains, with the photon pairs residing within one octave. Here, we demonstrate direct generation and detection of high-purity photon pairs at room temperature that are four octaves apart, one at 780 nm to match the rubidium D2 line, and the other at 3950 nm that falls in a transparent, low-scattering optical window for free space applications. The pairs are created via spontaneous parametric downconversion in a lithium niobate waveguide with specially designed geometry and periodic poling. The 780 nm photons are measured with a silicon avalanche photodiode, and the 3950 nm photons are measured with an upconversion photon detector using a similar waveguide, which attains 34% internal conversion efficiency. Quantum correlation measurement yields a high coincidence-to-accidental ratio of 54, which indicates the strong correlation with the extremely non-degenerate photon pairs. Our system bridges existing quantum technology to the challenging mid-IR regime, where unprecedented applications are expected in metrology, sensing, communications, medical diagnostics, and so on., Comment: 32 pages, 6 figures

When overlapping in an optical medium with nonlinear susceptibility, light waves can interact with each other, changing their phases, wavelengths, shapes, and so on. Such nonlinear effects, discovered over a half century ago, have given rise to a breadth of important applications. Applying to quantum-mechanical signals, however, they face fundamental challenges arising from the multimode nature of the interacting electromagnetic fields, such as phase noises and Raman scattering. Quantum Zeno blockade allows strong interaction of light waves without them physically overlapping, thus providing a viable solution for those challenges, as indicated in recent bulk-optics experiments. Here, we report on the observation of quantum Zeno blockade on chip, where a light wave is modulated by another in a distinct "interaction-free" manner. For quantum applications, we also verify its operations on a single-photon level. Our results promise a scalable platform for overcoming several grand challenges faced by nonlinear optics and quantum information processing, enabling, e.g., manipulation and interaction of quantum signals without decoherence.

A new conceptual key generation scheme is presented by using intrinsic quantum correlations of single photons between Alice and Bob. The intrinsic bi-partite correlation functions allow key bit to be generated through high level communication language i.e. a key bit is directly encoded to shared correlation functions not to the state and detection of a photon at Bob does not mean key bit. These make the scheme robust against intercept-resend attack because Alice and Bob can always check the errors in their measurements and reveal the presence of Eve in their channel without leaking any key bit information. The laser source is located in the middle of Alice and Bob, consists of two modes (x,y), relatively random phase-modulated $(\pm \frac{\pi}{2})$ weak coherent states combined in a perfect 50/50 beam splitter. The scheme is strictly relied on the perfect beam splitter and mean photon number less than 1, where more than one photon in a coherent pulse will introduce more errors in Bob even without the presence of Eve. From the percentage of errors in Bob, we can estimate the amount of information will be leaked to Eve in the photon-number splitting attack. This scheme can preserve the randomness of phase-randomized light source for doubling the communication distance as in original Ekert's protocol and providing the raw key generation rate a factor of 2 higher than weak coherent light protocols., Comment: 13 pages, 1 figure, 1 table

We present a scheme for key distribution based on bi-partite correlation of single photons. Alice keeps an ancilla photon and sends a signal photon to Bob, where intrinsic bi-partite correlation of these photons is obtained through first order intensity correlation in their detectors. The key bits are distributed through sharing four bi-partite correlation functions and photon counting. The scheme consists of two parts; first, Alice prepares deterministic photon states and Bob measures the photon states based on his random choice on correlation functions. Second, Alice guesses Bob's choice of correlation functions and sets the key bits by sending out photon states. Bob verifies the key bits through the photon states regardless Alice made a right or wrong guess. We called this key distribution scheme as prepare-measure-guess-verify (PMGV) protocol. We discuss the protocol by using a highly attenuated laser light, and then point out the advantages of using a fiber based correlated photon-pair to achieve better performance in security, communication distance and success rate of key distribution., Comment: 12 pages, 5 figures

Intrinsic quantum correlations of weak coherent states are observed between two parties through a novel detection scheme, which can be used as a supplement to the existence decoy-state BB84 and differential phase-shift quantum key distribution (DPS-QKD) protocols. In a proof-of-principle experiment, we generate bi-partite correlations of weak coherent states using weak local oscillator fields in two spatially separated balanced homodyne detections. We employ nonlinearity of post-measurement method to obtain the bi-partite correlations from two single-field interferences at individual homodyne measurement. This scheme is then used to demonstrate bits correlations between two parties over a distance of 10 km through a transmission fiber. We believe that the scheme can add another physical layer of security to these protocols for quantum key distribution., Comment: 10 pages, 4 figures

We present a new approach for constructing optical phase-space-time-frequency tomography (OPSTFT) of an optical wave field. This tomography can be measured by using a novel four-window optical imaging system based on two local oscillator fields balanced heterodyne detection. The OPSTFT is a Wigner distribution function of two independent Fourier Transform pairs, i.e., phase-space and time-frequency. From its theoretical and experimental aspects, it can provide information of position, momentum, time and frequency of a spatial light field with precision beyond the uncertainty principle. We simulate the OPSTFT for a light field obscured by a wire and a single-line absorption filter. We believe that the four-window system can provide spatial and temporal properties of a wave field for quantum image processing and biophotonics., Comment: 11 pages, 6 figures

We present direct measurement of Kirkwood-Rihaczek (KR) distribution for spatial properties of coherent light beam in terms of position and momentum (angle) coordinates. We employ a two-local oscillator (LO) balanced heterodyne detection (BHD) to simultaneously extract distribution of transverse position and momentum of a light beam. The two-LO BHD could measure KR distribution for any complex wave field (including quantum mechanical wave function) without applying tomography methods (inverse Radon transformation). Transformation of KR distribution to Wigner, Glauber Sudarshan P- and Husimi or Q- distributions in spatial coordinates are illustrated through experimental data. The direct measurement of KR distribution could provide local information of wave field, which is suitable for studying particle properties of a quantum system. While Wigner function is suitable for studying wave properties such as interference, and hence provides nonlocal information of the wave field. The method developed here can be used for exploring spatial quantum state for quantum mapping and computing, optical phase space imaging for biomedical applications., Comment: 27 pages, 14 figures