Search

Among the known particles, the neutron is special because it provides experimental access to all of the four fundamental forces and a wide range of hypothetical interactions. Despite being unstable, free neutrons live long enough to be used as test particles in interferometric, spectroscopic and scattering experiments probing low-energy scales. Recognized already in the 1970s, fundamental concepts of quantum mechanics can be tested in neutron interferometry using silicon perfect single crystals. Besides enabling tests of uncertainty relations or Bell inequalities, neutrons offer the opportunity to observe the effects of gravity and hypothetical dark forces acting on extended matter wavefunctions. Such tests gained importance in the light of recent discoveries of inconsistencies in the understanding of cosmology and the incompatibility between quantum mechanics and general relativity. Experiments with low-energy neutrons are, thus, indispensable tools for probing fundamental physics and represent a complementary approach to particle colliders. In this Review, we discuss the history and experimental methods used at this low-energy frontier of physics and overview the current bounds and limits on quantum mechanical relations and dark energy interactions. Low-energy neutrons are key for understanding fundamental concepts of quantum mechanics and physics beyond the standard model. This Review addresses topics such as matter-wave interferometry, quantum mechanical relations and hypothetical dark sector models and interactions.

Einstein’s theory of general relativity and quantum theory form the two major pillars of modern physics. However, certain inertial properties of a particle’s intrinsic spin are inconspicuous while the inertial properties of mass are well known. Here, by performing a neutron interferometric experiment, we observe phase shifts arising as a consequence of the spin’s coupling with the angular velocity of a rotating magnetic field. This coupling is a purely quantum mechanical extension of the Sagnac effect. The resulting phase shifts linearly depend on the frequency of the rotation of the magnetic field. Our results agree with the predictions derived from the Pauli–Schrödinger equation.

Nanocomposites enable us to tune parameters that are crucial for use of such materials for neutron-optics applications such as diffraction gratings by careful choice of properties such as species (isotope) and concentration of contained nanoparticles. Nanocomposites for neutron optics have so far successfully been deployed in protonated form, containing high amounts of $^1$H atoms, which exhibit rather strong neutron absorption and incoherent scattering. At a future stage of development, chemicals containing $^1$H could be replaced by components with more favourable isotopes, such as $^2$H or $^{19}$F. In this note, we present results of Monte-Carlo simulations of the transmissivity of various nanocomposite materials for thermal and very-cold neutron spectra. The results are compared to experimental transmission data. Our simulation results for deuterated and fluorinated nanocomposite materials predict a decrease of absorption- and scattering-losses down to about 2 % for very-cold neutrons., submitted to NIMA

We present a detailed analysis of the time series of time-stamped neutron counts obtained by single-neutron interferometry. The neutron counting statistics display the usual Poissonian behavior, but the variance of the neutron counts does not. Instead, the variance is found to exhibit a dependence on the phase-shifter setting which can be explained by a probabilistic model that accounts for fluctuations of the phase shift. The time series of the detection events exhibit long-time correlations with amplitudes that also depend on the phase-shifter setting. These correlations appear as damped oscillations with a period of about 2.8 s. By simulation, we show that the correlations of the time differences observed in the experiment can be reproduced by assuming that, for a fixed setting of the phase shifter, the phase shift experienced by the neutrons varies periodically in time with a period of 2.8 s. The same simulations also reproduce the behavior of the variance. Our analysis of the experimental data suggests that time-stamped data of singleparticle interference experiments may exhibit transient features that require a description in terms of non-stationary processes, going beyond the standard quantum model of independent random events.

In their original framework weak values must be measured by weak measurements that are minimally disturbing, meaning that the coupling between an investigated quantum system and a measurement device has no influence on the evolution of the system. However, under certain circumstances this weakness of the interaction is not necessary. In that case weak values can still be exactly determined from the statistics of the outcomes of arbitrary-strength generalized measurements. Here, we report an experimental procedure for neutron matter-waves that extends the notion of generalized eigenvalues for the neutron's path system to allow the exact determination of weak values using both strong and weak interactions. Experimental evidence is given that strong interactions outperform weak ones both for precision and accuracy.

Topology-optimized 3D-printed magnets are interesting for Larmor spin-rotators in neutron optics in general, and in neutron interferometry in particular. Using 3D-printed magnets instead of magnetic coils avoids heat dissipation, which is the the main cause of loss in fringe visibility, due to temperature gradients in the interferometer. This study applies the technique to implement an arbitrary neutronic phase gate, for rotations of up to $4\ensuremath{\pi}$ of the neutron's spinor wave function in one arm of the interferometer. This is achieved by varying the distance between the 3D-printed magnets, while maintaining homogeneity of the magnetic action over the neutron beam's profile.

Devices for manipulation of the neutron spin are vital for experiments in neutron optics such as neutron interferometry. Here we introduce a new type of such devices which are based on a magnetic material that can be 3D printed in complex shapes. We have constructed a spin flipper wherein the angle of spin rotation can be adjusted by variation of the distance between magnetized pieces. As the device does not contain any heat dissipating coils we expect interferometric measurements to become more stable and hence more accurate. Results of an experiment using polarized neutrons verify the device's functionality, and indicate the potential of the new method. A second experiment for demonstration of the 4π spinor symmetry of fermionic wave functions is in progress.

The canonical commutation relation is the hallmark of quantum theory, and Heisenberg's uncertainty relation is a direct consequence of it. Although various formulations of uncertainty relations have been tested in experiments a direct test of the commutation relation has hitherto not been performed. The reason for this is that whereas in quantum mechanics, observables are usually represented by Hermitian operators, the product of two noncommuting observables as occurring in the commutator relation is, in general, non-Hermitian. Here, we present a theoretical scheme for a direct test of the commutation relation and report its experimental realization. More precisely, we provide an experimental verification of the canonical commutation relation between two qubit observables based on a measurement scheme widely known as “weak measurement.” In our neutron interferometric setup, we perform the measurement of a single anomalous weak value of a relevant path-qubit observable where the coupled spin-energy degree of freedom serves as an ancilla.

Previous experimental tests of quantum contextuality based on the Bell-Kochen-Specker (BKS) theorem have demonstrated that not all observables among a given set can be assigned noncontextual eigenvalue predictions, but have never identified which specific observables must fail such assignment. We now remedy this shortcoming by showing that BKS contextuality can be confined to particular observables by pre- and postselection, resulting in anomalous weak values that we measure using modern neutron interferometry. We construct a confined contextuality witness from weak values, which we measure experimentally to obtain a $5\sigma$ average violation of the noncontextual bound, with one contributing term violating an independent bound by more than $99\sigma$. This weakly measured confined BKS contextuality also confirms the quantum pigeonhole effect, wherein eigenvalue assignments to contextual observables apparently violate the classical pigeonhole principle., Comment: 8 pages, 7 figures

Over the past few years, Heisenberg's error-disturbance uncertainty relation has experienced increased attention since several experimental publications verified the theoretical findings of Ozawa predicting the violation and thus necessary reformulation of Heisenberg's relation. However, soon after their appearance, an alternative theory was presented by Busch and co-workers, which proclaimed the validity of Heisenberg's relation and thus gave rise to heated debates. Here, we present an experimental comparison of the competing approaches by applying them to the same neutron optical measurement apparatus. Empirical results for the different definitions of error and disturbance are presented for special input states and configurations of the apparatus to illustrate the opposing approaches. The inequalities restricting errors and disturbances are particularly emphasized. Despite the strong controversy, in the case of projectively measured qubit observables, both approaches lead to equal outcomes.

The indeterminacy inherent in quantum measurements is an outstanding character of quantum theory, which manifests itself typically in the uncertainty principle. In the last decade, several universally valid forms of error-disturbance uncertainty relations were derived for completely general quantum measurements for arbitrary states. Subsequently, Branciard established a form that is optimal for spin measurements for some pure states. However, the bound in his inequality is not stringent for mixed states. One of the present authors recently derived a new bound tight in the corresponding mixed state case. Here, a neutron-optical experiment is carried out to investigate this new relation: it is tested whether error and disturbance of quantum measurements disappear or persist in mixing up the measured ensemble. The attainability of the new bound is experimentally observed, falsifying the tightness of Branciard's bound for mixed spin states.

A novel method was recently proposed and experimentally realized for characterizing a quantum state by directly measuring its complex probability amplitudes in a particular basis using so-called weak values. Recently Vallone and Dequal showed theoretically that weak measurements are not a necessary condition to determine the weak value [Phys. Rev. Lett. 116, 040502 (2016)]. Here we report a measurement scheme used in a matter-wave interferometric experiment in which the neutron path system's quantum state was characterized via direct measurements using both strong and weak interactions. Experimental evidence is given that strong interactions outperform weak ones. Our results are not limited to neutron interferometry, but can be used in a wide range of quantum systems., 5 pages, 3 figures

The uncertainty principle generally prohibits determination of certain pairs of quantum mechanical observables with arbitrary precision and forms the basis of indeterminacy in quantum mechanics. It was Heisenberg who used the famous gamma-ray microscope thought experiment to illustrate this indeterminacy. A lower bound was set for the product of the measurement error of an observable and the disturbance caused by the measurement. Later on, the uncertainty relation was reformulated in terms of standard deviations, which focuses solely on indeterminacy of predictions and neglects unavoidable recoil in measuring devices. A correct formulation of the error-disturbance relation, taking recoil into account, is essential for a deeper understanding of the uncertainty principle. However, the validity of Heisenberg's original error-disturbance uncertainty relation is justifed only under limited circumstances. Another error-disturbance relation, derived by rigorous and general theoretical treatments of quantum measurements, is supposed to be universally valid. Here, we report a neutron optical experiment that records the error of a spin-component measurement as well as the disturbance caused on another spin-component measurement. The results confirm that both error and disturbance completely obey the new, more general relation but violate the old one in a wide range of an experimental parameter., 11 pages, 5 figures, Nature Physics (in press)

The Kochen-Specker theorem theoretically shows evidence of the incompatibility of noncontextual hidden variable theories with quantum mechanics. Quantum contextuality is a more general concept than quantum non-locality which is quite well tested in experiments by using Bell inequalities. Within neutron interferometry we performed an experimental test of the Kochen-Specker theorem with an inequality, which identifies quantum contextuality, by using spin-path entanglement in a single neutron system. Here entanglement is achieved not between different particles, but between degrees of freedom, i.e., between spin and path degree of freedom. Appropriate combinations of the spin analysis and the position of the phase shifter allow an experimental verification of the violation of an inequality of the Kochen-Specker theorem. The observed value of (2.291 +/- 0.008), which is above the threshold of 1, clearly shows that quantum mechanical predictions cannot be reproduced by noncontextual hidden variable theories., Comment: 5 pages, 3 figures

A neutron optical experiment is presented to investigate the paths taken by neutrons in a three-beam interferometer. In various beam-paths of the interferometer, the energy of the neutrons is partially shifted so that the faint traces are left along the beam-path. By ascertaining an operational meaning to "the particle's path", which-path information is extracted from these faint traces with minimal-perturbations. Theory is derived by simply following the time evolution of the wave function of the neutrons, which clarifies the observation in the framework of standard quantum mechanics. Which-way information is derived from the intensity, sinusoidally oscillating in time at different frequencies, which is considered to result from the interfering cross terms between stationary main component and the energy-shifted which-way signals. Final results give experimental evidence that the (partial) wave functions of the neutrons in each beam path are superimposed and present in multiple locations in the interferometer., 8 pages,4 figures

Non-local correlations between subsystems sufficiently separated in spacetime have been extensively discussed in the light of the Einstein, Podolsky and Rosen (EPR) paradox, together with Bell's inequality. Within quantum terminology, such a non-locality can be interpreted as a consequence of the entanglement of subsystems. A more general concept, i.e., quantum contextuality, compared to non-locality, can be introduced to describe other striking phenomena predicted by quantum theory. As examples of quantum contextuality, we report several neutron interferometer experiments: a violation of a Bell-like inequality, a Kochen–Specker-like phenomenon, a quantum state tomography. Entanglement is achieved not between the particles, but between the degrees of freedom of a single-particle. Furthermore, an experiment dealing with triple entanglement is presented.

We present a neutron polarimetric experiment where two kinds of spinor precessions are observed: one is induced by different total energy of neutrons (zero-field precession) and the other is induced by a stationary guide field (Larmor precession). A characteristic of the former is the dependence of the energy-difference, which is in practice tuned by the frequency of the interacting oscillating magnetic field. In contrast the latter completely depends on the strength of the guide field, namely Larmor frequency. Our neutron-polarimetric experiment exhibits individual tuning as well as specific properties of each spinor precession, which assures the use of both spin precessions for multi-entangled spinor manipulation., 12 pages, 4 figures

Weak values, introduced more than 25 years ago, underwent a metamorphosis from a theoretical curiosity to a powerful resource in photonics for exploring foundations of quantum mechanics, as well as a practical laboratory tool. Due to the tiny coherence volume of particles used in matter-wave optics, a straightforward implementation of weak measurements is not feasible. We have overcome this hurdle by developing a method to weakly measure a massive particle's spin component. A neutron optical approach is realized by utilizing neutron interferometry, where the neutron's spin is coupled weakly to its spatial degree of freedom. Here, we present how one can fully characterize the weak value of the Pauli spin operator ${\stackrel{\ifmmode \hat{}\else \^{}\fi{}}{\ensuremath{\sigma}}}_{z}$ of neutrons by extracting its real and imaginary components, as well as its modulus. The results show good agreement with theoretical predictions and demonstrate that the (spin) weak value is actually accessible for a purely quantum system of massive particles.

Information-theoretic definitions for noise and disturbance in quantum measurements were given in Phys. Rev. Lett. 112, 050401 (2014) and a state-independent noise-disturbance uncertainty relation was obtained. Here, we derive a tight noise-disturbance uncertainty relation for complementary qubit observables and carry out an experimental test. Successive projective measurements on the neutron's spin-1/2system, together with a correction procedure which reduces the disturbance, are performed. Our experimental results saturate the tight noise-disturbance uncertainty relation for qubits when an optimal correction procedure is applied., Comment: 5 pages, 5 figures plus Supplemental Material (5 pages, 4 figures)

We have measured the non-cyclic geometric phase acquired during a unitary SU(2) evolution of a neutron spinor wave function for the mixed state case. The data is in good agreement with theory, verifying the predicted values for the mixed state geometric phase.

We have measured the Pancharatnam relative phase for spin- 1 / 2 states. In a neutron polarimetry experiment the minima and maxima of intensity modulations, giving the Pancharatnam phase, were determined. We also considered general SU ( 2 ) evolution for mixed states. The results are in good agreement with theory.

According to Bell’s theorem, every theory based on local realism is at variance with certain predictions of quantum mechanics. A theory that maintains realism but abandons reliance on locality, which has been proposed by Leggett, is incompatible with experimentally observable quantum correlations. In our experiment correlation measurements of spin-energy entangled single-neutrons violate a Leggett-type inequality by more than 7.6 standard deviations. The experimental data falsify the contextual realistic model and are fully in favor of quantum mechanics.

In its original formulation, Heisenberg's uncertainty principle dealt with the relationship between the error of a quantum measurement and the thereby induced disturbance on the measured object. Meanwhile, Heisenberg's heuristic arguments have turned out to be correct only for special cases. A new universally valid relation was derived by Ozawa in 2003. Here, we demonstrate that Ozawa's predictions hold for projective neutron-spin measurements. The experimental inaccessibility of error and disturbance claimed elsewhere has been overcome using a tomographic method. By a systematic variation of experimental parameters in the entire configuration space, the physical behavior of error and disturbance for projective spin-1/2 measurements is illustrated comprehensively. The violation of Heisenberg's original relation, as well as, the validity of Ozawa's relation become manifest. In addition, our results conclude that the widespread assumption of a reciprocal relation between error and disturbance is not valid in general., 17 pages, 13 figures

Heisenberg's uncertainty principle is probably the most famous statement of quantum physics and its essential aspects are well described by a formulations in terms of standard deviations. However, a naive Heisenberg-type error-disturbance relation is not valid. An alternative universally valid relation was derived by Ozawa in 2003. Though universally valid Ozawa's relation is not optimal. Recently, Branciard has derived a tight error-disturbance uncertainty relation (EDUR), describing the optimal trade-off between error and disturbance. Here, we report a neutron-optical experiment that records the error of a spin-component measurement, as well as the disturbance caused on another spin-component to test EDURs. We demonstrate that Heisenberg's original EDUR is violated, and the Ozawa's and Branciard's EDURs are valid in a wide range of experimental parameters, applying a new measurement procedure referred to as two-state method.

Heisenberg’s uncertainty principle in a formulation of uncertainties, intrinsic to any quantum system, is rigorously proven and demonstrated in various quantum systems. Nevertheless, Heisenberg’s original formulation of the uncertainty principle was given in terms of a reciprocal relation between the error of a position measurement and the thereby induced disturbance on a subsequent momentum measurement. However, a naive generalization of a Heisenberg-type error-disturbance relation for arbitrary observables is not valid. An alternative universally valid relation was derived by Ozawa in 2003. Though universally valid, Ozawa’s relation is not optimal. Recently, Branciard has derived a tight error-disturbance uncertainty relation (EDUR), describing the optimal trade-off between error and disturbance under certain conditions. Here, we report a neutron-optical experiment that records the error of a spin-component measurement, as well as the disturbance caused on another spin-component to test EDURs. We demonstrate that Heisenberg’s original EDUR is violated, and Ozawa’s and Branciard’s EDURs are valid in a wide range of experimental parameters, as well as the tightness of Branciard’s relation.

We implemented a triply entangled Greenberger-Horne-Zeilinger(GHZ)-like state and coherently manipulated the spin, path, and energy degrees of freedom in a single neutron system. The GHZ-like state was analyzed with an inequality derived by Mermin: we determined the four expectation values and finally obtained M = 2.558 +/- 0.004 > 2, which exhibits a clear violation of the noncontextual assumption and confirms quantum contextuality., 4 pages, 2figures

Geometric phase phenomena in single neutrons have been observed in polarimeter and interferometer experiments. Interacting with static and time dependent magnetic fields, the state vectors acquire a geometric phase tied to the evolution within spin subspace. In a polarimeter experiment the non-additivity of quantum phases for mixed spin input states is observed. In a Si perfect-crystal interferometer experiment appearance of geometric phases, induced by interaction with an oscillating magnetic field, is verified. The total system is characterized by an entangled state, consisting of neutron and radiation fields, governed by a Jaynes-Cummings Hamiltonian. In addition, the influence of the geometric phase on a Bell measurement, expressed by the Clauser-Horne-Shimony-Holt (CHSH) inequality, is studied. It is demonstrated that the effect of geometric phase can be balanced by an appropriate change of Bell angles., Comment: 17 pages, 9 figures

The influence of the geometric phase on a Bell measurement, as proposed by Bertlmann et al. in [Phys. Rev. A 69, 032112 (2004)], and expressed by the Clauser-Horne-Shimony-Holt (CHSH) inequality, has been observed for a spin-path entangled neutron state in an interferometric setup. It is experimentally demonstrated that the effect of geometric phase can be balanced by a change in Bell angles. The geometric phase is acquired during a time dependent interaction with two radio-frequency (rf) fields. Two schemes, polar and azimuthal adjustment of the Bell angles, are realized and analyzed in detail. The former scheme, yields a sinusoidal oscillation of the correlation function S, dependent on the geometric phase, such that it varies in the range between 2 and 2\sqrt{2} and, therefore, always exceeds the boundary value 2 between quantum mechanic and noncontextual theories. The latter scheme results in a constant, maximal violation of the Bell-like-CHSH inequality, where S remains 2\sqrt2 for all settings of the geometric phase., 10 pages 9 figures

Violation of a Bell-like inequality for a spin-energy entangled neutron state has been confirmed in a polarimetric experiment. The proposed inequality, in Clauser-Horne-Shimony-Holt (CHSH) formalism, relies on correlations between the spin and energy degree of freedom in a single-neutron system. The entangled states are generated utilizing a suitable combination of two radio-frequency fields in a neutron polarimeter setup. The correlation function S is determined to be 2.333+/-0.005, which violates the Bell-like CHSH inequality by more than 66 standard deviations., 4 pages 2 figures

We performed an experimental test of the Kochen-Specker theorem based on an inequality derived from the Peres-Mermin proof, using spin-path (momentum) entanglement in a single neutron system. Following the strategy proposed by Cabello et al. [Phys. Rev. Lett. 100, 130404 (2008)], a Bell-like state was generated and three expectation values were determined. The observed violation 2.291 +/- 0.008 > 1 clearly shows that quantum mechanical predictions cannot be reproduced by noncontextual hidden variables theories., REVTeX4, 4 pages, 3 figures

We have observed the stationary interference oscillations of a triple-entangled neutron state in an interferometric experiment. Time-dependent interaction with two radio-frequency (rf) fields enables coherent manipulation of an energy degree of freedom in a single neutron. The system is characterized by a multiply entangled state governed by a Jaynes-Cummings Hamiltonian. The experimental results confirm coherence of the manipulation as well as the validity of the description., 4 pages, 3 figures

In a neutron polarimetry experiment the mixed state relative phases between spin eigenstates are determined from the maxima and minima of measured intensity oscillations. We consider evolutions leading to purely geometric, purely dynamical and combined phases. It is experimentally demonstrated that the sum of the individually determined geometric and dynamical phases is not equal to the associated total phase which is obtained from a single measurement, unless the system is in a pure state., RevTex, 4 pages, 4 figures, accepted by PRL

According to Bell's theorem, no theory based on the joint assumption of realism and locality can reproduce certain predictions of quantum mechanics. Another class of realistic models, proposed by Leggett, that demands realism but abandons reliance on locality, is predicted to be in conflict with quantum mechanics. In this paper, we report on an experimental test of a contextual realistic model analogous to the model of Leggett performed with matter waves, more precisely with neutrons. Correlation measurements of the spin-energy entangled single-particle system show violation of a Leggett-type inequality by more than 7.6 standard deviations. Our experimental data falsify the contextual realistic model and are fully in favor of quantum mechanics.

Entanglement is a remarkable peculiarity in quantum mechanics. It occurs in quantum systems that consist of space-like separated parts, or in systems whose observables belong to disjoint Hilbert spaces. The latter is the case in single-neutron systems. Entangled states are renowned for exhibiting non-classical correlations between observables of individual sub-systems. In a perfect Si-crystal interferometer experiment entanglement between three degrees of freedom in a single-neutron system is created. The prepared entanglement of spin, path and energy is induced by interaction with an oscillating magnetic field. The generated Greenberger-Horne-Zeilinger (GHZ) state is analyzed with an inequality derived by Mermin, yielding a value M = 2.558(4) 2, which exhibits a clear violation of the classical assumption. In addition observation of a GHZ entanglement, consisting of spin, momentum and total energy, in a neutron polarimetric experiment is presented. Here the advantages of neutron polarimetry, such as high contrast or insensitivity to ambient disturbances, are utilized resulting in final value of M = 3.936(2) 2.