Ellsworth J. Welton, Giuseppe Salerno, Maxim Eremenko, Stefano Corradini, Luca Merucci, Aurélie Riandet, Sergey Khaykin, Irène Xueref-Remy, Gérard Ancellet, Clémence Bellon, Dario Stelitano, Lorenzo Guerrieri, Pasquale Sellitto, Bernard Legras, Alessia Sannino, Simone Lolli, Antonella Boselli, Juan Cuesta, Henda Guermazi, Laboratoire Interuniversitaire des Systèmes Atmosphériques (LISA (UMR_7583)), Institut national des sciences de l'Univers (INSU - CNRS)-Université Paris-Est Créteil Val-de-Marne - Paris 12 (UPEC UP12)-Centre National de la Recherche Scientifique (CNRS)-Université Paris Cité (UPCité), Osservatorio Etneo di Catania, Istituto Nazionale di Geofisica e Vulcanologia - Sezione di Catania (INGV), Istituto Nazionale di Geofisica e Vulcanologia-Istituto Nazionale di Geofisica e Vulcanologia, Istituto Nazionale di Geofisica e Vulcanologia - Sezione di Roma (INGV), Istituto Nazionale di Geofisica e Vulcanologia, Osservatorio Nazionale Terremoti, Institut méditerranéen de biodiversité et d'écologie marine et continentale (IMBE), Avignon Université (AU)-Aix Marseille Université (AMU)-Institut de recherche pour le développement [IRD] : UMR237-Centre National de la Recherche Scientifique (CNRS), TROPO - LATMOS, Laboratoire Atmosphères, Milieux, Observations Spatiales (LATMOS), Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Institut national des sciences de l'Univers (INSU - CNRS)-Sorbonne Université (SU)-Centre National de la Recherche Scientifique (CNRS)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Institut national des sciences de l'Univers (INSU - CNRS)-Sorbonne Université (SU)-Centre National de la Recherche Scientifique (CNRS), Istituto di Metodologie per l'Analisi Ambientale (IMAA), Consiglio Nazionale delle Ricerche [Potenza] (CNR), NASA Goddard Space Flight Center (GSFC), Dipartimento di Fisica 'Ettore Pancini', University of Naples Federico II = Università degli studi di Napoli Federico II, Laboratoire de Météorologie Dynamique (UMR 8539) (LMD), Institut national des sciences de l'Univers (INSU - CNRS)-École polytechnique (X)-École des Ponts ParisTech (ENPC)-Sorbonne Université (SU)-Centre National de la Recherche Scientifique (CNRS)-Département des Géosciences - ENS Paris, École normale supérieure - Paris (ENS-PSL), Université Paris sciences et lettres (PSL)-Université Paris sciences et lettres (PSL)-École normale supérieure - Paris (ENS-PSL), Université Paris sciences et lettres (PSL)-Université Paris sciences et lettres (PSL), Institut national des sciences de l'Univers (INSU - CNRS)-Université Paris-Est Créteil Val-de-Marne - Paris 12 (UPEC UP12)-Centre National de la Recherche Scientifique (CNRS)-Université de Paris (UP), Sorbonne Université (SU)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Centre National de la Recherche Scientifique (CNRS)-Institut national des sciences de l'Univers (INSU - CNRS)-Sorbonne Université (SU)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Centre National de la Recherche Scientifique (CNRS)-Institut national des sciences de l'Univers (INSU - CNRS), Università degli studi di Napoli Federico II, École normale supérieure - Paris (ENS Paris), and Université Paris sciences et lettres (PSL)-Université Paris sciences et lettres (PSL)-École normale supérieure - Paris (ENS Paris)
soumis a JGR Atmospheres - First posted online: Fri, 8 Oct 2021; International audience; During the extended activity of Mount Etna volcano in February-April 2021, three distinct paroxysmal events took place from 21 to 26 February, which were associated with a very uncommon transport of the injected upper-tropospheric plumes towards the north. Using a synergy of observations and modelling, we characterised the emissions and three-dimensional dispersion for these three plumes, we monitor their downwind distribution and optical properties, and we estimate their radiative impacts at selected locations. With a satellite-based source inversion, we estimate the emitted sulphur dioxide (SO2) mass at an integrated value of 55 kt and plumes injections at up to 12 km altitudes, which qualifies this series as an extreme event for Mount Etna. Then, we combine Lagrangian dispersion modelling, initialised with measured temporally-resolved SO2 emission fluxes and altitudes, with satellite observations to track the dispersion of the three individual plumes. The transport towards the north allowed the height-resolved downwind monitoring of the plumes at selected observatories in France, Italy and Israel, using LiDARs and photometric aerosol observations. Volcanic-specific aerosol optical depths in the visible spectral range ranging from about 0.004 to 0.03 and local daily average shortwave radiative forcing ranging from about -0.2 to -1.2 W/m2 (at the top of atmosphere) and from about -0.2 to -3.0 W/m2 (at the surface) are found. The composition (possible presence of ash), aerosol optical depth and radiative forcing of the plume has a large inter- and intra-plume variability and thus depend strongly on the position of the sampled section of the plumes.