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It is known that the electromagnetic vacuum is responsible for the Lamb shift, which is a crucial phenomenon in quantum electrodynamics (QED). In circuit QED, the readout or bus resonators that are dispersively coupled can result in a significant Lamb shift of the qubit. However, previous approaches or proposals for controlling the Lamb shift in circuit QED demand overheads in circuit designs or non-perturbative renormalization of the system's eigenbases, which can impose formidable limitations.In this work, we propose and demonstrate an all-microwave method for controlling the Lamb shift of fixed-frequency transmons. We employ the drive-induced longitudinal coupling between the transmon and resonator. By simply using an off-resonant monochromatic drive near the resonator frequency, we can control the net Lamb shift up to 30 MHz and engineer it to zero with the drive-induced longitudinal coupling without facing the aforementioned challenges. Our work establishes an efficient way of engineering the fundamental effects of the electromagnetic vacuum and provides greater flexibility in non-parametric frequency controls of multilevel systems.

Harmonic oscillators belong to the most fundamental concepts in physics and are central to many current research fields such as circuit QED, cavity optomechanics and photon-pressure systems. Here, we engineer a microwave mode in a superconducting LC circuit that mimics the dynamics of a negative mass oscillator, and couple it via photon-pressure to a second low-frequency circuit. We demonstrate that the effective negative mass dynamics lead to an inversion of dynamical backaction and to sideband-cooling of the low-frequency circuit by a blue-detuned pump field, which can be intuitively understood by the inverted energy ladder of a negative mass oscillator.

Microwave driving is a ubiquitous technique for superconducting qubits (SCQs), but the dressed states description based on the conventionally used perturbation theory cannot fully capture the dynamics in the strong driving limit. Comprehensive studies beyond these approximations applicable to transmon-based circuit quantum electrodynamics (QED) systems are unfortunately rare as the relevant works have been mainly limited to single-mode or two-state systems. In this work, we investigate a microwave-dressed transmon coupled to a single quantized mode over a wide range of driving parameters. We reveal that the interaction between the transmon and resonator as well as the properties of each mode is significantly renormalized in the strong driving limit. Unlike previous theoretical works, we establish a non-recursive, and non-Floquet theory beyond the perturbative regimes, which excellently quantifies the experiments. This work expands our fundamental understanding of dressed cavity QED-like systems beyond the conventional approximations. Our work will also contribute to fast quantum gate implementation, qubit parameter engineering, and fundamental studies on driven nonlinear systems.

Photon-pressure coupling between two superconducting circuits is a promising platform for investigating radiation-pressure coupling in novel parameter regimes and for the development of radio-frequency (RF) quantum photonics and quantum-limited RF sensing. So far, the intrinsic Josephson nonlinearity of photon-pressure coupled circuits has not been considered a potential resource for enhanced devices or novel experimental schemes. Here, we implement photon-pressure coupling between a RF circuit and a microwave cavity containing a superconducting quantum interference device (SQUID) which can be operated as a Josephson parametric amplifier (JPA). We demonstrate a Kerr-based enhancement of the photon-pressure single-photon coupling rate and an increase of the cooperativity by one order of magnitude in the amplifier regime. In addition, we characterize the upconverted and Kerr-amplified residual thermal fluctuations of the RF circuit, and observe that the intracavity amplification reduces the measurement imprecision. Finally, we demonstrate that RF mode sideband-cooling is surprisingly not limited to the effective amplifier mode temperature arising from quantum noise amplification, which we explain by non-trivial bath dynamics due to a two-stage amplification process. Our results demonstrate how Kerr nonlinearities and in particular Josephson parametric amplification can be utilized as resource for enhanced photon-pressure systems and Kerr cavity optomechanics.

Quantum materials can display physical phenomena rooted in the geometry of electronic wavefunctions. The corresponding geometric tensor is characterized by an emergent field known as Berry curvature (BC). Large BCs typically arise when electronic states with different spin, orbital or sublattice quantum numbers hybridize at finite crystal momentum. In all materials known to date, the BC is triggered by the hybridization of a single type of quantum number. Here, we report the discovery of the first material system having both spin and orbital-sourced BC: LaAlO$_3$/SrTiO$_3$ interfaces grown along the [111] direction. We detect independently these two sources and directly probe the BC associated to the spin quantum number through measurements of an anomalous planar Hall effect. The observation of a nonlinear Hall effect with time-reversal symmetry signals large orbital-mediated BC dipoles. The coexistence of different forms of BC enables the combination of spintronic and optoelectronic functionalities in a single material., Comment: 32 pages, 25 figures, accepted in Nature Materials

Quantum information processing requires fast manipulations of quantum systems in order to overcome dissipative effects. We propose a method to accelerate quantum dynamics and obtain a target state in a shorter time relative to unmodified dynamics, and apply the theory to a system consisting of two linearly coupled qubits. We extend the technique to accelerate quantum adiabatic evolution in order to rapidly generate a desired target state, thereby realizing a shortcut to adiabaticity. Further, we address experimental limitations to the rate of change of control parameters for quantum devices which often limit one's ability to generate a desired target state with high fidelity. We show that an initial state following decelerated dynamics can reach a target state while varying control parameters more slowly, enabling more experimentally feasible driving schemes.

In this work, we analytically and numerically study the sideband transition dynamics of the driven quantum Rabi model (QRM). We focus in particular on the conditions when the external transverse drive fields induce first-order sideband transitions. Inducing sideband transitions between two different systems is an essential technique for various physical models, including the QRM. However, despite its importance, a precise analytical study has not been reported yet that successfully explains the sideband transition rates in a driven QRM applicable for all system parameter configurations. In our study, we analytically derive the sideband transition rates based on second-order perturbation theory, not relying on the rotating wave approximation (RWA) \cite{RWA}. Our formula are valid for all ranges of drive frequencies and system's parameters. Our analytical derived formula agrees well with the numerical results in a regime of moderate drive amplitudes. Interestingly, we have found a non-trivial longitudinal drive effect derived from the transverse drive Hamiltonian. This accounts for significant corrections to the sideband transition rates that are expected without considering the derived longitudinal effect. Using this approach, one can precisely estimate the sideband transition rates in the QRM not confining themselves within specific parameter regimes. This provides important contributions for understanding experiments described by the driven QRM.

Nonlinear damping, a force of friction that depends on the amplitude of motion, plays an important role in many electrical, mechanical and even biological oscillators. In novel technologies such as carbon nanotubes, graphene membranes or superconducting resonators, the origin of nonlinear damping is sometimes unclear. This presents a problem, as the damping rate is a key figure of merit in the application of these systems to extremely precise sensors or quantum computers. Through measurements of a superconducting circuit, we show that nonlinear damping can emerge as a direct consequence of quantum fluctuations and the conservative nonlinearity of a Josephson junction. The phenomenon can be understood and visualized through the flow of quasi-probability in phase space, and accurately describes our experimental observations. Crucially, the effect is not restricted to superconducting circuits: we expect that quantum fluctuations or other sources of noise give rise to nonlinear damping in other systems with a similar conservative nonlinearity, such as nano-mechanical oscillators or even macroscopic systems.

The field of cavity optomechanics has achieved groundbreaking photonic control and detection of mechanical oscillators, based on their coupling to linear electromagnetic modes. Lately, however, there is an uprising interest in exploring cavity nonlinearities as a powerful new resource in radiation-pressure interacting systems. Here, we present a flux-mediated optomechanical device combining a nonlinear Josephson-based superconducting quantum interference cavity with a mechanical nanobeam. We demonstrate how the intrinsic Kerr nonlinearity of the microwave circuit can be used for a counter-intuitive blue-detuned sideband-cooling scheme based on multi-tone cavity driving and intracavity four-wave-mixing. Based on the large single-photon coupling rate of the system of up to $g_0 = 2\pi\cdot 3.6\,$kHz and a high mechanical quality factor $Q_\mathrm{m} \approx 4\cdot 10^{5}$, we achieve an effective four-wave cooperativity of $\mathcal{C}_\mathrm{fw} > 100$ and demonstrate four-wave cooling of the mechanical oscillator close to its quantum groundstate, achieving a final occupancy of $n_\mathrm{m} \sim 1.6$. Our results significantly advance the recently developed platform of flux-mediated optomechanics and demonstrate how cavity Kerr nonlinearities can be utilized for novel control schemes in cavity optomechanics.

Attempting to reconcile general relativity with quantum mechanics is one of the great undertakings of contemporary physics. Here we present how the incompatibility between the two theories arises in the simple thought experiment of preparing a heavy object in a quantum superposition. Following Penrose's analysis of the problem, we determine the requirements on physical parameters to perform experiments where both theories potentially interplay. We use these requirements to compare different systems, focusing on mechanical oscillators which can be coupled to superconducting circuits., Comment: arXiv admin note: text overlap with arXiv:2004.09153

Observing quantum phenomena in macroscopic objects, and the potential discovery of a fundamental limit in the applicability of quantum mechanics, has been a central topic of modern experimental physics. Highly coherent and heavy micro-mechanical oscillators controlled by superconducting circuits are a promising system for this task. Here, we focus in particular on the electrostatic coupling of motion to a weakly anharmonic circuit, namely the transmon qubit. In the case of a megahertz mechanical oscillator coupled to a gigahertz transmon, we explain the difficulties in bridging the large electro-mechanical frequency gap. To remedy this issue, we explore the requirements to reach phonon-number resolution in the resonant coupling of a megahertz transmon and a mechanical oscillator., Comment: Code used to generate the figures available in Zenodo with the DOI identifier 10.5281/zenodo.4292367

Driving quantum systems periodically in time plays an essential role in the coherent control of quantum states. The rotating wave approximation (RWA) is a good approximation technique for weak and nearly-resonance driven fields. However, these experiments sometimes require large detuning and strong driving fields, for which the RWA may not hold. In this work, we experimentally, numerically, and analytically explore strongly driven two-mode Josephson circuits in the regime of strong driving and large detuning. Specifically, we investigate beam-splitter and two-mode squeezing interaction between the two modes induced by driving a two-photon sideband transition. Using numerical simulations, we observe that the RWA is unable to correctly capture the amplitude of the sideband transition rates. We verify this finding using an analytical model that is based on perturbative corrections. We find that the breakdown of the RWA in the regime studied does not lead to qualitatively different dynamics, but gives the same results as the RWA theory at higher drive strengths, enhancing the coupling rates compared to what one would predict. This is an interesting consequence compared to the carrier transition case, where the breakdown of the RWA results in qualitatively different time evolution of the quantum state. Our work provides an insight into the behavior of time-periodically driven systems beyond the RWA. We also provide a robust theoretical framework for including these findings in the calculation and calibration of quantum protocols in circuit quantum electrodynamics.

We perform extensive analysis of graphene Josephson junctions embedded in microwave circuits. By comparing a diffusive junction at 15 mK with a ballistic one at 15 mK and 1 K, we are able to reconstruct the current-phase relation.

Superconducting cavities with high quality factors play an essential role in circuit quantum electrodynamics and quantum computing. In measurements of the the intrinsic loss rates of high frequency modes, it can be challenging to design an appropriate coupling to the measurement circuit in such a way that the resulting signal is sufficiently strong but also that this coupling does not lead to unwanted loading circuit, obscuring the intrinsic internal loss rates. Here, we propose and demonstrate a spectroscopic probe of high-Q resonators based on the phenomena of electromagnetically-induced transparency (EIT) between the resonator and qubit in the weak dispersive coupling regime. Applying a sideband drive signal to the qubit, we observe an interference dip originated from EIT in the qubit spectroscopy, originating from the quantum interference between the qubit probe signal and sideband transition. From the width and the depth of the dip, we are able to extract the single-photon linewidth of the resonator from an analytical model. Working in a previously unexplored regime in which the qubit has a larger linewidth than the resonator reduces the technical challenge of making a high-coherence qubit and is advantageous for remaining in the weakly-invasive limit of coupling to the resonator. Furthermore, the sideband and the dispersive coupling between the resonator and the qubit can be tuned $in~situ$ controlling the strength of the sideband drive power. This $in-situ$ tuneability allows the technique to be applied for efficient measurement of the resonator loss rate for any quality factor below a fixed upper bound, on the order of $10^8$ for our device, allowing a wide range of quality factors to probed using a single design.

We have studied electrical transport as a function of carrier density, temperature and bias in multi-terminal devices consisting of hexagonal boron nitride (h-BN) encapsulated titanium trisulfide (TiS$_3$) sheets. Through the encapsulation with h-BN, we observe metallic behavior and high electron mobilities. Below $\sim$60 K an increase in the resistance, and non-linear transport with plateau-like features in the differential resistance are present, in line with the expected charge density wave (CDW) formation. Importantly, the critical temperature and the threshold field of the CDW phase can be controlled through the back-gate.

We present the design, measurement and analysis of a current sensor based on a process of Josephson parametric upconversion in a superconducting microwave cavity. Terminating a coplanar waveguide with a nanobridge constriction Josephson junction, we observe modulation sidebands from the cavity that enable highly sensitive, frequency-multiplexed output of small currents for applications such as transition-edge sensor array readout. We derive an analytical model to reproduce the measurements over a wide range of bias currents, detunings and input powers. Tuning the frequency of the cavity by more than \SI{100}{\mega\hertz} with DC current, our device achieves a minimum current sensitivity of \SI{8.9}{\pico\ampere\per\sqrt{\hertz}}. Extrapolating the results of our analytical model, we predict an improved device based on our platform, capable of achieving sensitivities down to \SI{50}{\femto\ampere\per\sqrt{\hertz}}}, or even lower if one could take advantage of parametric amplification in the Josephson cavity. Taking advantage of the Josephson architecture, our approach can provide higher sensitivity than kinetic inductance designs, and potentially enables detection of currents ultimately limited by quantum noise.

We propose a scheme for controlling a radio-frequency mechanical resonator at the quantum level using a superconducting qubit. The mechanical part of the circuit consists of a suspended micrometer-long beam that is embedded in the loop of a superconducting quantum interference device (SQUID) and is connected in parallel to a transmon qubit. Using realistic parameters from recent experiments with similar devices, we show that this configuration can enable a tuneable optomechanical interaction in the single-photon ultrastrong-coupling regime, where the radiation-pressure coupling strength is larger than both the transmon decay rate and the mechanical frequency. We investigate the dynamics of the driven system for a range of coupling strengths and find an optimum regime for ground-state cooling, consistent with previous theoretical investigations considering linear cavities. Furthermore, we numerically demonstrate a protocol for generating hybrid discrete- and continuous-variable entanglement as well as mechanical Schr\"{o}dinger cat states, which can be realised within the current state of the art. Our results demonstrate the possibility of controlling the mechanical motion of massive objects using superconducting qubits at the single-photon level and could enable applications in hybrid quantum technologies as well as fundamental tests of quantum mechanics.

Quantum circuits constructed from Josephson junctions and superconducting electronics are key to many quantum computing and quantum optics applications. Designing these circuits involves calculating the Hamiltonian describing their quantum behavior. Here we present QuCAT, or "Quantum Circuit Analyzer Tool", an open-source framework to help in this task. This open-source Python library features an intuitive graphical or programmatical interface to create circuits, the ability to compute their Hamiltonian, and a set of complimentary functionalities such as calculating dissipation rates or visualizing current flow in the circuit., Comment: Corrected error in fig. 2 in v4

Microwave optomechanical circuits have been demonstrated in the past years to be extremely powerfool tools for both, exploring fundamental physics of macroscopic mechanical oscillators as well as being promising candidates for novel on-chip quantum limited microwave devices. In most experiments so far, the mechanical oscillator is either used as a passive device element and its displacement is detected using the superconducting cavity or manipulated by intracavity fields. Here, we explore the possibility to directly and parametrically manipulate the mechanical nanobeam resonator of a cavity electromechanical system, which provides additional functionality to the toolbox of microwave optomechanical devices. In addition to using the cavity as an interferometer to detect parametrically modulated mechanical displacement and squeezed thermomechanical motion, we demonstrate that parametric modulation of the nanobeam resonance frequency can realize a phase-sensitive parametric amplifier for intracavity microwave photons. In contrast to many other microwave amplification schemes using electromechanical circuits, the presented technique allows for simultaneous cooling of the mechanical element, which potentially enables this type of optomechanical microwave amplifier to be quantum-limited.

In transition metal dichalcogenides, defects have been found to play an important role, affecting doping, spin-valley relaxation dynamics, and assisting in proximity effects of spin-orbit coupling. Here, we study localized states in $\mathrm{WS}_2$ and how they affect tunneling through van der Waals heterostructures of h-BN/graphene/$\mathrm{WS}_2$/metal. The obtained conductance maps as a function of bias and gate voltage reveal single-electron transistor behavior (Coulomb blockade) with a rich set of transport features including excited states and negative differential resistance regimes. Applying a perpendicular magnetic field, we observe a shift in the energies of the quantum levels and information about the orbital magnetic moment of the localized states is extracted.

Massive mechanical resonators operating at the quantum scale can enable a large variety of applications in quantum technologies, as well as fundamental tests of quantum theory. Of crucial importance in that direction, is both their integrability into state-of-the-art quantum platforms as well as the ability to prepare them in generic quantum states using well-controlled high-fidelity operations. Here, we propose a scheme for controlling a radio-frequency mechanical resonator at the quantum scale using two superconducting transmon qubits that can be integrated on the same chip. Specifically, we consider two qubits coupled via a capacitor in parallel to a superconducting quantum interference device (SQUID), which has a suspended mechanical beam embedded in one of its arms. Following a theoretical analysis of the quantum system, we find that this configuration, in combination with an in-plane magnetic field, can give rise to a tuneable three-body interaction in the single-photon strong-coupling regime, while enabling suppression of the stray qubit-qubit coupling. Using state-of-the-art parameters and qubit operations at single-excitation levels, we numerically demonstrate the possibility of ground-state cooling as well as high-fidelity preparation of mechanical quantum states and qubit-phonon entanglement, i.e. states having negative Wigner functions and obeying non-classical correlations. Our work significantly extends the quantum control toolbox of radio-frequency mechanical resonators and may serve as a promising architecture for integrating such mechanical elements with transmon-based quantum processors.

We present measurements of weak localization on hexagonal boron nitride encapsulated bilayer MoS$_2$. From the analysis we obtain information regarding the phase-coherence and the spin diffusion of the electrons. We find that the encapsulation with boron nitride provides higher mobilities in the samples, and the phase-coherence shows improvement, while the spin relaxation does not exhibit any significant enhancement compared to non-encapsulated MoS$_2$. The spin relaxation time is in the order of a few picoseconds, indicating a fast intravalley spin-flip rate. Lastly, the spin-flip rate is found to be independent from electron density in the current range, which can be explained through counteracting spin-flip scattering processes based on electron-electron Coulomb scattering and extrinsic Bychkov-Rashba spin-orbit coupling.

In this report, we present nanoelectromechanical resonators fabricated with thin exfoliated crystals of a high-T$_c$ cuprate superconductor Bi$_2$Sr$_2$Ca$_1$Cu$_2$O$_{8+\delta}$. The mechanical readout is performed by capacitively coupling their motion to a coplanar waveguide microwave cavity fabricated with a superconducting alloy of molybdenum-rhenium. We demonstrate mechanical frequency tunability with external dc-bias voltage, and quality factors up to 36600. Our spectroscopic and time-domain measurements show that mechanical dissipation in these systems is limited by the contact resistance arising from resistive outer layers. The temperature dependence of dissipation indicates the presence of tunneling states, further suggesting that their intrinsic performance could be as good as other two-dimensional atomic crystals such as graphene., Comment: 13 pages, 5 figures

Detecting weak radio-frequency electromagnetic fields plays a crucial role in wide range of fields, from radio astronomy to nuclear magnetic resonance imaging. In quantum mechanics, the ultimate limit of a weak field is a single-photon. Detecting and manipulating single-photons at megahertz frequencies presents a challenge as, even at cryogenic temperatures, thermal fluctuations are significant. Here, we use a gigahertz superconducting qubit to directly observe the quantization of a megahertz radio-frequency electromagnetic field. Using the qubit, we achieve quantum control over thermal photons, cooling to the ground-state and stabilizing photonic Fock states. Releasing the resonator from our control, we directly observe its re-thermalization dynamics with the bath with nanosecond resolution. Extending circuit quantum electrodynamics to a new regime, we enable the exploration of thermodynamics at the quantum scale and allow interfacing quantum circuits with megahertz systems such as spin systems or macroscopic mechanical oscillators., Comment: Changes in v2: condensed main part, error in Table S1 corrected. Raw data and code available in Zenodo with the identifier 10.5281/zenodo.2551258

High-gain and low-noise signal amplification is a valuable tool in various cryogenic microwave experiments. A microwave optomechanical device, in which a vibrating capacitor modulates the frequency of a microwave cavity, is one technique that is able to amplify microwave signals with high gain and large dynamical range. Such optomechanical amplifiers typically rely on strong backaction of microwave photons on the mechanical mode achieved in the sideband-resolved limit of optomechanics. Here, we observe microwave amplification in an optomechanical cavity in the extremely unresolved sideband limit. A large gain is observed for any detuning of the single pump tone within the cavity linewidth, a clear indication that the amplification is not induced by dynamical backaction. By being able to amplify for any detuning of the pump signal, the amplification center frequency can be tuned over the entire range of the broad cavity linewidth. Additionally, by providing microwave amplification without mechanical amplification, we predict that using this scheme it is possible to achieve near-quantum-limited microwave amplification despite a large thermal occupation of the mechanical mode.

We explore the superconducting phase diagram of the two-dimensional electron system at the LaAlO3/SrTiO3 interface by monitoring the frequencies of the cavity modes of a coplanar waveguide resonator fabricated in the interface itself. We determine the phase diagram of the superconducting transition as a function of temperature and electrostatic gating, finding that both the superfluid density and the transition temperature follow a dome shape, but that the two are not monotonically related. The ground state of this 2DES is interpreted as a Josephson junction array, where a transition from long- to short-range order occurs as a function of the electronic doping. The synergy between correlated oxides and superconducting circuits is revealed to be a promising route to investigate these exotic compounds, complementary to standard magneto-transport measurements., Comment: 5 pages, 4 figures and 10 pages of supplementary material

Phase engineering of MoS2 transistors has recently been demonstrated and has led to record low contact resistances. The phase patterning of MoS2 flakes with laser radiation has also been realized via spectroscopic methods, which invites the potential of controlling the metallic and semiconducting phases of MoS2 transistors by simple light exposure. Nevertheless, the fabrication and demonstration of laser patterned MoS2 devices starting from the metallic polymorph has not been demonstrated yet. Here, we study the effects of laser radiation on 1T/1T'-MoS2 transistors with the prospect of driving an in-situ phase transition to the 2H-polymorph through light exposure. We find that although the Raman peaks of 2H-MoS2 become more prominent and the ones from the 1T/1T' phase fade after the laser exposure, the semiconducting properties of the laser patterned devices are not fully restored and the laser treatment ultimately leads to degradation of the transport channel.

Carbon nanotubes continue to be model systems for studies of confinement and interactions. This is particularly true in the case of so-called "ultra-clean" carbon nanotube devices offering the study of quantum dots with extremely low disorder. The quality of such systems, however, has increasingly revealed glaring discrepancies between experiment and theory. Here we address the outstanding anomaly of exceptionally large orbital magnetic moments in carbon nanotube quantum dots. We perform low temperature magneto-transport measurements of the orbital magnetic moment and find it is up to seven times larger than expected from the conventional semiclassical model. Moreover, the magnitude of the magnetic moment monotonically drops with the addition of each electron to the quantum dot directly contradicting the widely accepted shell filling picture of single-particle levels. We carry out quasiparticle calculations, both from first principles and within the effective-mass approximation, and find the giant magnetic moments can only be captured by considering a self-energy correction to the electronic band structure due to electron-electron interactions., Comment: 15 pages and 10 figures including supplemental materials

Josephson junctions (JJ) are a fundamental component of microwave quantum circuits, such as tunable cavities, qubits and parametric amplifiers. Recently developed encapsulated graphene JJs, with supercurrents extending over micron distance scales, have exciting potential applications as a new building block for quantum circuits. Despite this, the microwave performance of this technology has not been explored. Here, we demonstrate a microwave circuit based on a ballistic graphene JJ embedded in a superconducting cavity. We directly observe a gate-tunable Josephson inductance through the resonance frequency of the device and, using a detailed RF model, we extract this inductance quantitatively. We also observe the microwave losses of the device, and translate this into sub-gap resistances of the junction at {\mu}eV energy scales, not accessible in DC measurements. The microwave performance we observe here suggests that graphene Josephson junctions are a feasible platform for implementing coherent quantum circuits., Comment: 43 pages, 20 figures

We have studied temperature- and electric-field dependent carrier transport in single flakes of MoS$_{2}$ treated with n-butyllithium. The temperature dependence of the four-terminal resistance follows the Efros-Shklovskii variable range hopping conduction mechanism. From measurements in the Ohmic and non-Ohmic regime, we estimate the localization length and the average hopping length of the carriers, as well as the effective dielectric constant. Furthermore, comparison between two- and four-probe measurements yield a contact resistance that increases significantly with decreasing temperature.

When a two level system (TLS) is coupled to an electromagnetic resonator, its transition frequency changes in response to the quantum vacuum fluctuations of the electromagnetic field, a phenomenon known as the Lamb shift. Remarkably, by replacing the TLS by a harmonic oscillator, normal mode splitting leads to a quantitatively similar shift, without taking quantum fluctuations into account. In a weakly-anharmonic system, lying in between the harmonic oscillator and a TLS, the origins of such shifts can be unclear. An example of this is the dispersive shift of a transmon qubit in circuit quantum electrodynamics (QED). Although often referred to as a Lamb shift, the dispersive shift observed in spectroscopy in circuit QED could contain a significant contribution from normal-mode splitting that is not driven by quantum fluctuations, raising the question: how much of this shift is quantum in origin? Here, we treat normal-mode splitting separately from shifts induced by quantum vacuum fluctuations in the Hamiltonian of a weakly-anharmonic system, providing a framework for understanding the extent to which observed frequency shifts can be attributed to quantum fluctuations.

We report on a technique for applying a DC bias in a 3D microwave cavity. We achieve this by isolating the two halves of the cavity with a dielectric and directly using them as DC electrodes. As a proof of concept, we embed a variable capacitance diode in the cavity and tune the resonant frequency with a DC voltage, demonstrating the incorporation of a DC bias into the 3D cavity with no measurable change in its quality factor at room temperature. We also characterize the architecture at millikelvin temperatures and show that the split cavity design maintains a quality factor $Q_\text{i} \sim 8.8 \times 10^5$, making it promising for future quantum applications.

With the introduction of superconducting circuits into the field of quantum optics, many novel experimental demonstrations of the quantum physics of an artificial atom coupled to a single-mode light field have been realized. Engineering such quantum systems offers the opportunity to explore extreme regimes of light-matter interaction that are inaccessible with natural systems. For instance the coupling strength $g$ can be increased until it is comparable with the atomic or mode frequency $\omega_{a,m}$ and the atom can be coupled to multiple modes which has always challenged our understanding of light-matter interaction. Here, we experimentally realize the first Transmon qubit in the ultra-strong coupling regime, reaching coupling ratios of $g/\omega_{m}=0.19$ and we measure multi-mode interactions through a hybridization of the qubit up to the fifth mode of the resonator. This is enabled by a qubit with 88% of its capacitance formed by a vacuum-gap capacitance with the center conductor of a coplanar waveguide resonator. In addition to potential applications in quantum information technologies due to its small size and localization of electric fields in vacuum, this new architecture offers the potential to further explore the novel regime of multi-mode ultra-strong coupling., Comment: 15 pages, 9 figures

In this experiment, we couple a superconducting Transmon qubit to a high-impedance $645\ \Omega$ microwave resonator. Doing so leads to a large qubit-resonator coupling rate $g$, measured through a large vacuum Rabi splitting of $2g\simeq 910$ MHz. The coupling is a significant fraction of the qubit and resonator oscillation frequencies $\omega$, placing our system close to the ultra-strong coupling regime ($\bar{g}=g/\omega=0.071$ on resonance). Combining this setup with a vacuum-gap Transmon architecture shows the potential of reaching deep into the ultra-strong coupling $\bar{g} \sim 0.45$ with Transmon qubits.

Circuit quantum electrodynamics (QED) studies the interaction of artificial atoms, open transmission lines and electromagnetic resonators fabricated from superconducting electronics. While the theory of an artificial atom coupled to one mode of a resonator is well studied, considering multiple modes leads to divergences which are not well understood. Here, we introduce a first-principles model of a multimode resonator coupled to a Josephson junction atom. Studying the model in the absence of any cutoff, in which the coupling rate to mode number $n$ scales as $\sqrt{n}$ for $n$ up to $\infty$, we find that quantities such as the Lamb shift do not diverge due to a natural rescaling of the bare atomic parameters that arises directly from the circuit analysis. Introducing a cutoff in the coupling from a non-zero capacitance of the Josephson junction, we provide a physical interpretation of the decoupling of higher modes in the context of circuit analysis. In addition to explaining the convergence of the quantum Rabi model with no cutoff, our work also provides a useful framework for analyzing the ultra-strong coupling regime of multimode circuit QED.

We investigate superconducting interference device (SQUID) with two asymmetric Josephson junctions coupled to a mechanical resonator embedded in the loop of the SQUID. We quantize this system in the case when the frequency of the mechanical resonator is much lower than the cavity frequency of the SQUID and in the case when they are comparable. In the first case, the radiation pressure and cross-Kerr type interactions arise and are modified by asymmetry. Cross-Kerr type coupling is the leading term at the extremum points where radiation pressure is zero. In the second case, the main interaction is single-photon beam splitter, which exists only at finite asymmetry. Another interaction in this regime is of cross-Kerr type, which exists at all asymmetries, but generally much weaker than the beam splitter interaction. Increasing magnetic field can substantially enhance optomechanical couplings strength with the potential for the radiation pressure coupling to reach the single-photon strong coupling regime, even the ultrastrong coupling regime, in which the single-photon coupling rate exceeds the mechanical frequency., Comment: 8 pages, 6 figures

Carbon nanotubes (CNTs) are a promising material for high-performance electronics beyond silicon. But unlike silicon, the nature of the transport band gap in CNTs is not fully understood. The transport gap in CNTs is predicted to be strongly driven by electron-electron (e-e) interactions and correlations, even at room temperature. Here, we use dielectric liquids to screen e-e interactions in individual suspended ultra-clean CNTs. Using multiple techniques, the transport gap is measured as dielectric screening is increased. Changing the dielectric environment from air to isopropanol, we observe a 25% reduction in the transport gap of semiconducting CNTs, and a 32% reduction in the band gap of narrow-gap CNTs. Additional measurements are reported in dielectric oils. Our results elucidate the nature of the transport gap in CNTs, and show that dielectric environment offers a mechanism for significant control over the transport band gap., Comment: Updates in this version: Additional comparison between theory and experiment, including band gap renormalization calculations for narrow gap CNTs compared to wide-gap CNTs

Superconducting coplanar waveguide (CPW), resonators are powerful and versatile tools used in areas ranging from radiation detection to circuit quantum electrodynamics. Their potential for low intrinsic losses makes them attractive as sensitive probes of electronic properties of bulk materials and thin films. Here we use superconducting MoRe CPW resonators, to investigate the high-frequency (up to 0.3 GHz) and low temperature (down to 3.5 K) permittivity of SrTiO3, a non-linear dielectric on the verge of a ferroelectric transition (quantum paraelectricity). We perform a quantitative analysis of its dielectric properties as a function of external dc bias (up to +-15V), rf power and mode number and discuss our results within the framework of the most recent theoretical models. We also discuss the origin of a fatigue effect that reduces the tunability of the dielectric constant of SrTiO3, which we relate to the presence of oxygen vacancies.

We report on observations of thickness dependent Josephson coupling and multiple Andreev reflections (MAR) in vertically stacked molybdenum disulfide (MoS2) - molybdenum rhenium (MoRe) Josephson junctions. MoRe, a chemically inert superconductor, allows for oxide free fabrication of high transparency vertical MoS2 devices. Single and bilayer MoS2 junctions display relatively large critical currents (up to 2.5 uA) and the appearance of sub-gap structure given by MAR. In three and four layer thick devices we observe orders of magnitude lower critical currents (sub-nA) and reduced quasiparticle gaps due to proximitized MoS2 layers in contact with MoRe. We anticipate that this device architecture could be easily extended to other 2D materials., Comment: 18 pages, 6 figures including Supporting Information

The ability to exfoliate layered materials down to the single layer limit has opened the opportunity to understand how a gradual reduction in dimensionality affects the properties of bulk materials. Here we use this top-down approach to address the problem of superconductivity in the two-dimensional limit. The transport properties of electronic devices based on 2H tantalum disulfide flakes of different thicknesses are presented. We observe that superconductivity persists down to the thinnest layer investigated (3.5 nm), and interestingly, we find a pronounced enhancement in the critical temperature from 0.5 K to 2.2 K as the layers are thinned down. In addition, we propose a tight-binding model, which allows us to attribute this phenomenon to an enhancement of the effective electron-phonon coupling constant. This work provides evidence that reducing dimensionality can strengthen superconductivity as opposed to the weakening effect that has been reported in other 2D materials so far., Comment: 54 pages

The semiconducting p-n junction is a simple device structure with great relevance for electronic and optoelectronic applications. The successful integration of low-dimensional materials in electronic circuits has opened the way forward for producing gate-tunable p-n junctions. In that context, here we present an organic (Cu-phthalocyanine)-2D layered material (MoS2) hybrid p-n junction with both gate-tunable diode characteristics and photovoltaic effect. Our proof-of-principle devices show multifunctional properties with diode rectifying factors of up to 10^4, while under light exposure they exhibit photoresponse with a measured external quantum efficiency of ~ 11 %. As for their photovoltaic properties, we found open circuit voltages of up to 0.6 V and optical-to-electrical power conversion efficiency of 0.7 %. The extended catalogue of known organic semiconductors and two-dimensional materials offer the prospect for tailoring the properties and the performance of the resulting devices, making organic-2D p-n junctions promising candidates for future technological applications., Comment: 32 pages

We study mechanical dissipation of the fundamental mode of millimeter-sized, high quality-factor ($Q$) metalized silicon nitride membranes at temperatures down to 14 mK using a three-dimensional optomechanical cavity. Below 200 mK, high-$Q$ modes of the membranes show a diverging increase of $Q$ with decreasing temperature, reaching $Q=1.27\times10^8$ at 14 mK, an order of magnitude higher than reported before. The ultra-low dissipation makes the membranes highly attractive for the study of optomechanics in the quantum regime, as well as for other applications of optomechanics such as microwave to optical photon conversion., Comment: 12 pages, 4 figures

In many hybrid quantum systems, a superconducting circuit is required that combines DC-control with a coplanar waveguide (CPW) microwave resonator. The strategy thus far for applying a DC voltage or current bias to microwave resonators has been to apply the bias through a symmetry point in such a way that it appears as an open circuit for certain frequencies. Here, we introduce a microwave coupler for superconducting CPW cavities in the form of a large shunt capacitance to ground. Such a coupler acts as a broadband mirror for microwaves while providing galvanic connection to the center conductor of the resonator. We demonstrate this approach with a two-port $\lambda/4$-transmission resonator with linewidths in the MHz regime ($Q\sim10^3$) that shows no spurious resonances and apply a voltage bias up to $80$ V without affecting the quality factor of the resonator. This resonator coupling architecture, which is simple to engineer, fabricate and analyse, could have many potential applications in experiments involving superconducting hybrid circuits., Comment: 15 pages, 12 figures