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In optical conventional lasers, chirped pulse amplification (CPA) has become an extremely powerful technique for the generation of ultrashort pulses in the infrared and visible spectral ranges. In this contribution we report the successful implementation of CPA in a seeded XUV FEL. A second experiment, using a two-stage harmonic generation scheme (FERMI FEL-2) has the objective to generate coherent and phase-tailored few-femtosecond FEL pulses, with gigawatt peak power in the sub-10 nm spectral range. This second experiment is still in progress. We will discuss the main scientific and technical bottlenecks and the implications.

The transverse coherence of the source is an important property for FEL experiments. Theory and simulations indicated different features for seeded and unseeded FELs but so far no direct comparison has been pursued experimentally on the same facility. At FERMI one has the unique possibility to test both configurations (SASE and seeding) within the same operating conditions. In this contribution we present the experimental results of the characterization of transverse coherence with special attention to the evolution of such property.

The advent of free electron lasers (FELs) in the soft and hard X-ray spectral region has opened the possibility to probe electronic, magnetic and structural dynamics, in both diluted and condensed matter samples, with femtosecond time resolution. In particular, FELs strongly enhanced the capabilities of several analytical techniques, which took advantage of the high degree of transverse coherence provided. FELs based on the harmonic up-conversion of an external seed laser are characterised also by a high degree of longitudinal coherence, since electrons inherit the coherence properties of the seed. At the present state of the art, the shortest wavelength delivered to user experiments by an externally seeded FEL light source is about 4 nm. We show here that pulses with a high longitudinal degree of coherence (first and second order) covering the water window and with photon energy extending up to 790 eV can be generated by exploiting the so-called nonlinear harmonic regime, which allows generation of radiation at harmonics of the resonant FEL wavelength. Moreover, we report the results of two proof-of-principle experiments: one measuring the oxygen K-edge absorption in water ($\sim$ 530 eV), the other analysing the spin dynamics of Fe and Co through magnetic small angle x-ray scattering at their L-edges (707 eV and 780 eV)

FERMI is implementing a development plan to keep the facility in a world-leading position on the base of the requests coming from the user community and the advises from the Scientific Advisory Council and the Machine Advisory Committee. The ultimate goal of this plan consists in doubling the maximum photon energy available and in reducing the pulse duration below the characteristic lifetime of the atomic core levels in the source spectral range. An upgrade of FERMI aimed at reaching the oxygen K-edge requires a profound modification of the FEL configurations and of the main components of the machine, including the linac and the undulator lines. One of the most promising approaches for this upgrade is to implement the echo-enabled harmonic generation (EEHG) scheme, relying on two external lasers to precisely control the spectrotemporal properties of the FEL pulse. The conversion to EEHG of the first stage of the double-stage harmonic cascade presently in use on FEL-2, would allow to reach harmonics as high as 120, enabling to generate coherent pulses down to 2 nm. The main aspects of the upgrade strategy will be discussed in this contribution.

Free-electron lasers (FELs) are currently the most advanced class of light sources, by virtue of their unique capability to lase high-brightness and ultrashort pulses characterized by wavelengths spanning the Extreme-Ultraviolet (EUV), the Soft (SXR) and Hard (HXR) X-Ray spectral domains, alongside with temporal duration lying in the femtosecond (fs) timescale [1]. Specifically, the advent of FELs light sources has recently allowed to perform, in a time-resolved fashion approach, both established spectroscopies, daily employed at synchrotron light sources, and novel non-linear optical methods, mostly combining FELs and laser pulses. Nonetheless, the next step to push the ultrafast X-Ray science standards is widely recognized to be linked to go beyond the current time-resolved schemes, so performing experiments engaging exclusively EUV, SXR and HXR pulses. Indeed, exciting (and probing) matter at its (or nearby) electronic resonance is largely speculated to be one of the key for discriminating and revealing the microscopic mechanisms hiding behind some of the most exotic phases of physical, chemical, and biological systems. Such a challenge calls the design of optical devices capable to both split and delay (in time) FELs pulses, without impacting on their coherence properties, and fully user-friendly in terms of preserving the perfect overlap of the resulting focal spots, even in the few microns spatial domain, a well-known trademark for focusing EUV, SXR and HXR pulses at FELs light sources [2]. At the seeded FERMI FEL (Trieste, Italy) this goal is committed by the novel optical device known as AC/DC, which stands for the Auto Correlator/Delay Creator. AC/DC is purposely designed to double the incoming FEL photon beam into two exact pulse replicas, splitting it by inserting a grazing incidence flat mirror, and further delaying in time, in a controlled way, one of the two pulses, with an intrinsic temporal resolution of approximately 360 attoseconds. A detailed description of AC/DC is highlighted here. Specifically, strong emphasis is dedicated to the opto-mechanical design and the laser-based feedback system, purposely designed and implemented to compensate in real-time any potential drift and pointing mismatch affecting the FEL optical trajectory, ascribable to both mechanical imperfections and residual paraxial errors appearing during a temporal delay scan [3]. [1] Bostedt C., Boutet S., Fritz D.M., Huang Z., Lee H.J., Lemke H.T., Robert A., Schlotter W.F., Turner J.J., Williams G.J., Linac Coherent Light Source: The first five years. Rev. Mod. Phys.88, 015007 (2016) [2] Manfredda M., Fava C., Gobessi R., Mahne N., Raimondi L., Simoncig A., Zangrando M., The evolution of KAOS, a multipurpose active optics system for EUV/Soft X-rays, Synchrotron Radiation News, 0, 0, (2022) DOI: 10.1080/08940886.2022.2066432 . [3] Simoncig A., Manfredda M., Gaio G., Mahne N., Raimondi M., Fava C., Gerusina S., Gobessi R., Abrami A., Capotondi F., De Angelis D., Menk R., Pancaldi M., Pedersoli E., Zangrando M., AC/DC: The FERMI FEL Split and Delay Optical Device for Ultrafast X-rays Science, Photonics, 9(5), 314, 2022

FERMI is studying a series of developments to keep the facility in a world-leading position on the base of the requests coming from the user community, the Scientific Advisory Council and the Machine Advisory Committee. The ultimate goal of the development plan consists in doubling the photon energy range and reducing the pulse duration below the characteristic lifetime of the atomic core levels located in the energy range of the source. One of the most promising approaches is the echo-enabled harmonic generation (EEHG) scheme, relying on two external lasers to precisely control the spectro-temporal properties of the FEL pulse. The implementation of EEHG in the double-stage harmonic cascade presently in use on FEL-2, would allow harmonics as high as 120 enabling to generate coherent pulses down to 2 nm starting from UV lasers. An upgrade of FERMI aimed at reaching the oxygen K-edge requires a profound modification of the FEL configurations and of the main components of the machine, including the linac and the undulator lines. The main aspects of the upgrade strategy will be discussed in this presentation., Proceedings of the 13th International Particle Accelerator Conference, IPAC2022, Bangkok, Thailand

Charge transport processes at interfaces which are governed by complex interfacial electronic structure play a crucial role in catalytic reactions, energy storage, photovoltaics, and many biological processes. Here, the first soft X-ray second harmonic generation (SXR-SHG) interfacial spectrum of a buried interface (boron/Parylene-N) is reported. SXR-SHG shows distinct spectral features that are not observed in X-ray absorption spectra, demonstrating its extraordinary interfacial sensitivity. Comparison to electronic structure calculations indicates a boron-organic separation distance of 1.9 ��, wherein changes as small as 0.1 �� result in easily detectable SXR-SHG spectral shifts (ca. 100s of meV). As SXR-SHG is inherently ultrafast and sensitive to individual atomic layers, it creates the possibility to study a variety of interfacial processes, e.g. catalysis, with ultrafast time resolution and bond specificity., 19 pages

FERMI is the seeded Free Electron Laser (FEL) user facility at the Elettra laboratory in Trieste, operating in the VUV to EUV and soft X-rays spectral range; the radiation produced by the seeded FEL is characterized by wavelength stability, low temporal jitter and longitudinal coherence in the range 100-4 nm. During 2018 a dedicated experiment has shown the potential of the Echo Enabled Harmonic Generation (EEHG) scheme [1] to cover most of this spectral range with a single stage cascade [2]. Such a scheme, combined to an increment of the beam energy and of the accelerator performances, could extend the FERMI operating range toward the oxygen k-edge. With this perspective, we present the development plans under consideration for the next 3 to 5 years. These include an upgrade of the linac and of the existing FEL lines, consisting in the conversion of FEL-1 first, and FEL-2 successively, into EEHG seeded FELs., Proceedings of the 39th Free Electron Laser Conference, FEL2019, Hamburg, Germany