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2. Physicochemical Properties of Nascent vs. Aged Sea Spray Aerosols in the Eastern North Atlantic

Author

Aggarwal, Sneha, primary, Garmash, Olga, additional, Kilgour, Delaney, additional, Jernigan, Chris, additional, Zinke, Julika, additional, Gong, Xianda, additional, Zhou, Shengqian, additional, Zhang, Jiaoshi, additional, Freitas, Gabriel, additional, Cunha, Bruno, additional, Silva, Tercio, additional, Wang, Jian, additional, Bertram, Timothy, additional, Thornton, Joel, additional, Salter, Matthew, additional, Zieger, Paul, additional, and Mohr, Claudia, additional

Published
2023
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3. Overview of the MOSAiC expedition - Atmosphere

Author

Shupe, Matthew D., Rex, Markus, Blomquist, Byron, Persson, P. Ola G., Schmale, Julia, Uttal, Taneil, Althausen, Dietrich, Angot, Hélène, Archer, Stephen, Bariteau, Ludovic, Beck, Ivo, Bilberry, John, Bucci, Silvia, Buck, Clifton, Boyer, Matt, Brasseur, Zoé, Brooks, Ian M., Calmer, Radiance, Cassano, John, Castro, Vagner, Chu, David, Costa, David, Cox, Christopher J., Creamean, Jessie, Crewell, Susanne, Dahlke, Sandro, Damm, Ellen, de Boer, Gijs, Deckelmann, Holger, Dethloff, Klaus, Dütsch, Marina, Ebell, Kerstin, Ehrlich, André, Ellis, Jody, Engelmann, Ronny, Fong, Allison A., Frey, Markus M., Gallagher, Michael R., Ganzeveld, Laurens, Gradinger, Rolf, Graeser, Jürgen, Greenamyer, Vernon, Griesche, Hannes, Griffiths, Steele, Hamilton, Jonathan, Heinemann, Günther, Helmig, Detlev, Herber, Andreas, Heuzé, Céline, Hofer, Julian, Houchens, Todd, Howard, Dean, Inoue, Jun, Jacobi, Hans-Werner, Jaiser, Ralf, Jokinen, Tuija, Jourdan, Olivier, Jozef, Gina, King, Wessley, Kirchgaessner, Amelie, Klingebiel, Marcus, Krassovski, Misha, Krumpen, Thomas, Lampert, Astrid, Landing, William, Laurila, Tiia, Lawrence, Dale, Lonardi, Michael, Loose, Brice, Lüpkes, Christof, Maahn, Maximilian, Macke, Andreas, Maslowski, Wieslaw, Marsay, Christopher, Maturilli, Marion, Mech, Mario, Morris, Sara, Moser, Manuel, Nicolaus, Marcel, Ortega, Paul, Osborn, Jackson, Pätzold, Falk, Perovich, Donald K., Petäjä, Tuukka, Pilz, Christian, Pirazzini, Roberta, Posman, Kevin, Powers, Heath, Pratt, Kerri A., Preußer, Andreas, Quéléver, Lauriane, Radenz, Martin, Rabe, Benjamin, Rinke, Annette, Sachs, Torsten, Schulz, Alexander, Siebert, Holger, Silva, Tercio, Solomon, Amy, Sommerfeld, Anja, Spreen, Gunnar, Stephens, Mark, Stohl, Andreas, Svensson, Gunilla, Uin, Janek, Viegas, Juarez, Voigt, Christiane, von der Gathen, Peter, Wehner, Birgit, Welker, Jeffrey M., Wendisch, Manfred, Werner, Martin, Xie, ZhouQing, Yue, Fange, Shupe, Matthew D., Rex, Markus, Blomquist, Byron, Persson, P. Ola G., Schmale, Julia, Uttal, Taneil, Althausen, Dietrich, Angot, Hélène, Archer, Stephen, Bariteau, Ludovic, Beck, Ivo, Bilberry, John, Bucci, Silvia, Buck, Clifton, Boyer, Matt, Brasseur, Zoé, Brooks, Ian M., Calmer, Radiance, Cassano, John, Castro, Vagner, Chu, David, Costa, David, Cox, Christopher J., Creamean, Jessie, Crewell, Susanne, Dahlke, Sandro, Damm, Ellen, de Boer, Gijs, Deckelmann, Holger, Dethloff, Klaus, Dütsch, Marina, Ebell, Kerstin, Ehrlich, André, Ellis, Jody, Engelmann, Ronny, Fong, Allison A., Frey, Markus M., Gallagher, Michael R., Ganzeveld, Laurens, Gradinger, Rolf, Graeser, Jürgen, Greenamyer, Vernon, Griesche, Hannes, Griffiths, Steele, Hamilton, Jonathan, Heinemann, Günther, Helmig, Detlev, Herber, Andreas, Heuzé, Céline, Hofer, Julian, Houchens, Todd, Howard, Dean, Inoue, Jun, Jacobi, Hans-Werner, Jaiser, Ralf, Jokinen, Tuija, Jourdan, Olivier, Jozef, Gina, King, Wessley, Kirchgaessner, Amelie, Klingebiel, Marcus, Krassovski, Misha, Krumpen, Thomas, Lampert, Astrid, Landing, William, Laurila, Tiia, Lawrence, Dale, Lonardi, Michael, Loose, Brice, Lüpkes, Christof, Maahn, Maximilian, Macke, Andreas, Maslowski, Wieslaw, Marsay, Christopher, Maturilli, Marion, Mech, Mario, Morris, Sara, Moser, Manuel, Nicolaus, Marcel, Ortega, Paul, Osborn, Jackson, Pätzold, Falk, Perovich, Donald K., Petäjä, Tuukka, Pilz, Christian, Pirazzini, Roberta, Posman, Kevin, Powers, Heath, Pratt, Kerri A., Preußer, Andreas, Quéléver, Lauriane, Radenz, Martin, Rabe, Benjamin, Rinke, Annette, Sachs, Torsten, Schulz, Alexander, Siebert, Holger, Silva, Tercio, Solomon, Amy, Sommerfeld, Anja, Spreen, Gunnar, Stephens, Mark, Stohl, Andreas, Svensson, Gunilla, Uin, Janek, Viegas, Juarez, Voigt, Christiane, von der Gathen, Peter, Wehner, Birgit, Welker, Jeffrey M., Wendisch, Manfred, Werner, Martin, Xie, ZhouQing, and Yue, Fange

Abstract

With the Arctic rapidly changing, the needs to observe, understand, and model the changes are essential. To support these needs, an annual cycle of observations of atmospheric properties, processes, and interactions were made while drifting with the sea ice across the central Arctic during the Multidisciplinary drifting Observatory for the Study of Arctic Climate (MOSAiC) expedition from October 2019 to September 2020. An international team designed and implemented the comprehensive program to document and characterize all aspects of the Arctic atmospheric system in unprecedented detail, using a variety of approaches, and across multiple scales. These measurements were coordinated with other observational teams to explore cross-cutting and coupled interactions with the Arctic Ocean, sea ice, and ecosystem through a variety of physical and biogeochemical processes. This overview outlines the breadth and complexity of the atmospheric research program, which was organized into 4 subgroups: atmospheric state, clouds and precipitation, gases and aerosols, and energy budgets. Atmospheric variability over the annual cycle revealed important influences from a persistent large-scale winter circulation pattern, leading to some storms with pressure and winds that were outside the interquartile range of past conditions suggested by long-term reanalysis. Similarly, the MOSAiC location was warmer and wetter in summer than the reanalysis climatology, in part due to its close proximity to the sea ice edge. The comprehensiveness of the observational program for characterizing and analyzing atmospheric phenomena is demonstrated via a winter case study examining air mass transitions and a summer case study examining vertical atmospheric evolution. Overall, the MOSAiC atmospheric program successfully met its objectives and was the most comprehensive atmospheric measurement program to date conducted over the Arctic sea ice. The obtained data will support a broad range of coupled-system

Published
2022

4. Overview of the MOSAiC expedition: Atmosphere

Author

Shupe, Matthew D, Rex, Markus, Blomquist, Byron, Persson, POG, Schmale, J, Uttal, Taneil, Althausen, Dietrich, Angot, Hélène, Archer, Stephen, Bariteau, Ludovic, Beck, Ivo, Bilberry, John, Boyer, Matt, Brasseur, Zoe, Brooks, Ian M, Bucci, Silvia, Buck, Clifton, Calmer, Radiance, Cassano, John, Castro, Vagner, Chu, David, Costa, David, Cox, Christopher J, Creamean, Jessie, Crewell, Susanne, Dahlke, Sandro, Damm, Ellen, De Boer, G, Deckelmann, Holger, Dethloff, Klaus, Dütsch, Marina, Ebell, Kerstin, Ehrlich, André, Ellis, Jody, Engelmann, Ronny, Fong, Allison A, Frey, Markus M, Gallagher, Michael R, Ganzeveld, L, Gradinger, Rolf, Graeser, Juergen, Greenamyer, Vernon, Griesche, Hannes, Griffiths, Steele, Hamilton, Jonathan, Heinemann, Günther, Helmig, Detlev, Herber, Andreas, Heuzé, Céline, Hofer, Julian, Houchens, Todd, Howard, Dean, Inoue, Jun, Jacobi, Hans-Werner, Jaiser, Ralf, Jokinen, Tuija, Jourdan, Olivier, Jozef, Gina, King, Wessley, Kirchgaessner, Amelie, Klingebiel, Marcus, Krassovski, Misha, Krumpen, Thomas, Lampert, Astrid, Landing, William M, Laurila, Tiia, Lawrence, Dale, Lonardi, Michael, Loose, Brice, Lüpkes, Christof, Maahn, Max, Macke, Andreas, Marsay, Christopher, Maslowski, Wieslaw, Maturilli, Marion, Mech, Mario, Morris, Sara, Moser, Manuel, Nicolaus, Marcel, Ortega, Paul, Osborn, Jackson, Pätzold, Falk, Perovich, Donald K, Petäjä, Tuukka, Pilz, Christian, Pirazzini, Roberta, Posman, Kevin, Powers, Heath, Pratt, Kerri A, Preußer, Andreas, Quelever, Lauriane, Rabe, Benjamin, Radenz, Martin, Rinke, Annette, Sachs, Torsten, Schulz, Alexander, Siebert, Holger, Silva, Tercio, Solomon, Amy, Sommerfeld, Anja, Spreen, Gunnar, Stevens, Mark, Stohl, Andreas, Svensson, Gunilla, Uin, Janek, Viegas, Juarez, Voigt, Christiane, von der Gathen, Peter, Wehner, Birgit, Welker, Jeffrey M, Wendisch, Manfred, Werner, Martin, Xie, ZhouQing, Yue, Fange, Shupe, Matthew D, Rex, Markus, Blomquist, Byron, Persson, POG, Schmale, J, Uttal, Taneil, Althausen, Dietrich, Angot, Hélène, Archer, Stephen, Bariteau, Ludovic, Beck, Ivo, Bilberry, John, Boyer, Matt, Brasseur, Zoe, Brooks, Ian M, Bucci, Silvia, Buck, Clifton, Calmer, Radiance, Cassano, John, Castro, Vagner, Chu, David, Costa, David, Cox, Christopher J, Creamean, Jessie, Crewell, Susanne, Dahlke, Sandro, Damm, Ellen, De Boer, G, Deckelmann, Holger, Dethloff, Klaus, Dütsch, Marina, Ebell, Kerstin, Ehrlich, André, Ellis, Jody, Engelmann, Ronny, Fong, Allison A, Frey, Markus M, Gallagher, Michael R, Ganzeveld, L, Gradinger, Rolf, Graeser, Juergen, Greenamyer, Vernon, Griesche, Hannes, Griffiths, Steele, Hamilton, Jonathan, Heinemann, Günther, Helmig, Detlev, Herber, Andreas, Heuzé, Céline, Hofer, Julian, Houchens, Todd, Howard, Dean, Inoue, Jun, Jacobi, Hans-Werner, Jaiser, Ralf, Jokinen, Tuija, Jourdan, Olivier, Jozef, Gina, King, Wessley, Kirchgaessner, Amelie, Klingebiel, Marcus, Krassovski, Misha, Krumpen, Thomas, Lampert, Astrid, Landing, William M, Laurila, Tiia, Lawrence, Dale, Lonardi, Michael, Loose, Brice, Lüpkes, Christof, Maahn, Max, Macke, Andreas, Marsay, Christopher, Maslowski, Wieslaw, Maturilli, Marion, Mech, Mario, Morris, Sara, Moser, Manuel, Nicolaus, Marcel, Ortega, Paul, Osborn, Jackson, Pätzold, Falk, Perovich, Donald K, Petäjä, Tuukka, Pilz, Christian, Pirazzini, Roberta, Posman, Kevin, Powers, Heath, Pratt, Kerri A, Preußer, Andreas, Quelever, Lauriane, Rabe, Benjamin, Radenz, Martin, Rinke, Annette, Sachs, Torsten, Schulz, Alexander, Siebert, Holger, Silva, Tercio, Solomon, Amy, Sommerfeld, Anja, Spreen, Gunnar, Stevens, Mark, Stohl, Andreas, Svensson, Gunilla, Uin, Janek, Viegas, Juarez, Voigt, Christiane, von der Gathen, Peter, Wehner, Birgit, Welker, Jeffrey M, Wendisch, Manfred, Werner, Martin, Xie, ZhouQing, and Yue, Fange

Abstract

With the Arctic rapidly changing, the needs to observe, understand, and model the changes are essential. To support these needs, an annual cycle of observations of atmospheric properties, processes, and interactions were made while drifting with the sea ice across the central Arctic during the Multidisciplinary drifting Observatory for the Study of Arctic Climate (MOSAiC) expedition from October 2019 to September 2020. An international team designed and implemented the comprehensive program to document and characterize all aspects of the Arctic atmospheric system in unprecedented detail, using a variety of approaches, and across multiple scales. These measurements were coordinated with other observational teams to explore cross- cutting and coupled interactions with the Arctic Ocean, sea ice, and ecosystem through a variety of physical and biogeochemical processes. This overview outlines the breadth and complexity of the atmospheric research program, which was organized into 4 subgroups: atmospheric state, clouds and precipitation, gases and aerosols, and energy budgets. Atmospheric variability over the annual cycle revealed important influences from a persistent large-scale winter circulation pattern, leading to some storms with pressure and winds that were outside the interquartile range of past conditions suggested by long-term reanalysis. Similarly, the MOSAiC location was warmer and wetter in summer than the reanalysis climatology, in part due to its close proximity to the sea ice edge.The comprehensiveness of the observational program for characterizing and analyzing atmospheric phenomena is demonstrated via a winter case study examining air mass transitions and a summer case study examining vertical atmospheric evolution. Overall, the MOSAiC atmospheric program successfully met its objectives and was the most comprehensive atmospheric measurement program to date conducted over the Arctic sea ice. The obtained data will support a broad range of coupled-system

Published
2022

5. Overview of the MOSAiC expedition-Atmosphere INTRODUCTION

Author

Shupe, Matthew D., Rex, Markus, Blomquist, Byron, Persson, P. Ola G., Schmale, Julia, Uttal, Taneil, Althausen, Dietrich, Angot, Helene, Archer, Stephen, Bariteau, Ludovic, Beck, Ivo, Bilberry, John, Bucci, Silvia, Buck, Clifton, Boyer, Matt, Brasseur, Zoe, Brooks, Ian M., Calmer, Radiance, Cassano, John, Castro, Vagner, Chu, David, Costa, David, Cox, Christopher J., Creamean, Jessie, Crewell, Susanne, Dahlke, Sandro, Damm, Ellen, de Boer, Gijs, Deckelmann, Holger, Dethloff, Klaus, Duetsch, Marina, Ebell, Kerstin, Ehrlich, Andre, Ellis, Jody, Engelmann, Ronny, Fong, Allison A., Frey, Markus M., Gallagher, Michael R., Ganzeveld, Laurens, Gradinger, Rolf, Graeser, Juergen, Greenamyer, Vernon, Griesche, Hannes, Griffiths, Steele, Hamilton, Jonathan, Heinemann, Guenther, Helmig, Detlev, Herber, Andreas, Heuze, Celine, Hofer, Julian, Houchens, Todd, Howard, Dean, Inoue, Jun, Jacobi, Hans-Werner, Jaiser, Ralf, Jokinen, Tuija, Jourdan, Olivier, Jozef, Gina, King, Wessley, Kirchgaessner, Amelie, Klingebiel, Marcus, Krassovski, Misha, Krumpen, Thomas, Lampert, Astrid, Landing, William, Laurila, Tiia, Lawrence, Dale, Lonardi, Michael, Loose, Brice, Luepkes, Christof, Maahn, Maximilian, Macke, Andreas, Maslowski, Wieslaw, Marsay, Christopher, Maturilli, Marion, Mech, Mario, Morris, Sara, Moser, Manuel, Nicolaus, Marcel, Ortega, Paul, Osborn, Jackson, Paetzold, Falk, Perovich, Donald K., Petaja, Tuukka, Pilz, Christian, Pirazzini, Roberta, Posman, Kevin, Powers, Heath, Pratt, Kerri A., Preusser, Andreas, Quelever, Lauriane, Radenz, Martin, Rabe, Benjamin, Rinke, Annette, Sachs, Torsten, Schulz, Alexander, Siebert, Holger, Silva, Tercio, Solomon, Amy, Sommerfeld, Anja, Spreen, Gunnar, Stephens, Mark, Stohl, Andreas, Svensson, Gunilla, Uin, Janek, Viegas, Juarez, Voigt, Christiane, von der Gathen, Peter, Wehner, Birgit, Welker, Jeffrey M., Wendisch, Manfred, Werner, Martin, Xie, ZhouQing, Yue, Fange, Shupe, Matthew D., Rex, Markus, Blomquist, Byron, Persson, P. Ola G., Schmale, Julia, Uttal, Taneil, Althausen, Dietrich, Angot, Helene, Archer, Stephen, Bariteau, Ludovic, Beck, Ivo, Bilberry, John, Bucci, Silvia, Buck, Clifton, Boyer, Matt, Brasseur, Zoe, Brooks, Ian M., Calmer, Radiance, Cassano, John, Castro, Vagner, Chu, David, Costa, David, Cox, Christopher J., Creamean, Jessie, Crewell, Susanne, Dahlke, Sandro, Damm, Ellen, de Boer, Gijs, Deckelmann, Holger, Dethloff, Klaus, Duetsch, Marina, Ebell, Kerstin, Ehrlich, Andre, Ellis, Jody, Engelmann, Ronny, Fong, Allison A., Frey, Markus M., Gallagher, Michael R., Ganzeveld, Laurens, Gradinger, Rolf, Graeser, Juergen, Greenamyer, Vernon, Griesche, Hannes, Griffiths, Steele, Hamilton, Jonathan, Heinemann, Guenther, Helmig, Detlev, Herber, Andreas, Heuze, Celine, Hofer, Julian, Houchens, Todd, Howard, Dean, Inoue, Jun, Jacobi, Hans-Werner, Jaiser, Ralf, Jokinen, Tuija, Jourdan, Olivier, Jozef, Gina, King, Wessley, Kirchgaessner, Amelie, Klingebiel, Marcus, Krassovski, Misha, Krumpen, Thomas, Lampert, Astrid, Landing, William, Laurila, Tiia, Lawrence, Dale, Lonardi, Michael, Loose, Brice, Luepkes, Christof, Maahn, Maximilian, Macke, Andreas, Maslowski, Wieslaw, Marsay, Christopher, Maturilli, Marion, Mech, Mario, Morris, Sara, Moser, Manuel, Nicolaus, Marcel, Ortega, Paul, Osborn, Jackson, Paetzold, Falk, Perovich, Donald K., Petaja, Tuukka, Pilz, Christian, Pirazzini, Roberta, Posman, Kevin, Powers, Heath, Pratt, Kerri A., Preusser, Andreas, Quelever, Lauriane, Radenz, Martin, Rabe, Benjamin, Rinke, Annette, Sachs, Torsten, Schulz, Alexander, Siebert, Holger, Silva, Tercio, Solomon, Amy, Sommerfeld, Anja, Spreen, Gunnar, Stephens, Mark, Stohl, Andreas, Svensson, Gunilla, Uin, Janek, Viegas, Juarez, Voigt, Christiane, von der Gathen, Peter, Wehner, Birgit, Welker, Jeffrey M., Wendisch, Manfred, Werner, Martin, Xie, ZhouQing, and Yue, Fange

Abstract

With the Arctic rapidly changing, the needs to observe, understand, and model the changes are essential. To support these needs, an annual cycle of observations of atmospheric properties, processes, and interactions were made while drifting with the sea ice across the central Arctic during the Multidisciplinary drifting Observatory for the Study of Arctic Climate (MOSAiC) expedition from October 2019 to September 2020. An international team designed and implemented the comprehensive program to document and characterize all aspects of the Arctic atmospheric system in unprecedented detail, using a variety of approaches, and across multiple scales. These measurements were coordinated with other observational teams to explore crosscutting and coupled interactions with the Arctic Ocean, sea ice, and ecosystem through a variety of physical and biogeochemical processes. This overview outlines the breadth and complexity of the atmospheric research program, which was organized into 4 subgroups: atmospheric state, clouds and precipitation, gases and aerosols, and energy budgets. Atmospheric variability over the annual cycle revealed important influences from a persistent large-scale winter circulation pattern, leading to some storms with pressure and winds that were outside the interquartile range of past conditions suggested by long-term reanalysis. Similarly, the MOSAiC location was warmer and wetter in summer than the reanalysis climatology, in part due to its close proximity to the sea ice edge. The comprehensiveness of the observational program for characterizing and analyzing atmospheric phenomena is demonstrated via a winter case study examining air mass transitions and a summer case study examining vertical atmospheric evolution. Overall, the MOSAiC atmospheric program successfully met its objectives and was the most comprehensive atmospheric measurement program to date conducted over the Arctic sea ice. The obtained data will support a broad range of coupled-system s

Published
2022

6. Overview of the MOSAiC expedition: Atmosphere

Author

Shupe, Matthew, Rex, Markus, Blomquist, Byron, Ola, P, Persson, G, Schmale, Julia, Uttal, Taneil, Althausen, Dietrich, Lè Ne Angot, Hé, Archer, Stephen, Bariteau, Ludovic, Beck, Ivo, Bilberry, John, Bucci, Silvia, Buck, Clifton, Boyer, Matt, Brasseur, Zoé, Brooks, Ian, Cassano, John, Castro, Vagner, Chu, David, Costa, David, Cox, Christopher, Creamean, Jessie, Crewell, Susanne, Dahlke, Sandro, Damm, Ellen, de Boer, Gijs, Deckelmann, Holger, Dethloff, Klaus, Dütsch, Marina, Ebell, Kerstin, Ehrlich, André, Ellis, Jody, Engelmann, Ronny, Fong, Allison, Frey, Markus, Gallagher, Michael, Ganzeveld, Laurens, Gradinger, Rolf, Graeser, Jürgen, Greenamyer, Vernon, Griesche, Hannes, Griffiths, Steele, Hamilton, Jonathan, Heinemann, Günther, Helmig, Detlev, Herber, Andreas, Line Heuzé, Cé, Hofer, Julian, Houchens, Todd, Inoue, Jun, Jacobi, Hans-Werner, Jaiser, Ralf, Jokinen, Tuija, Jourdan, Olivier, King, Wessley, Kirchgaessner, Amelie, Klingebiel, Marcus, Krassovski, Misha, Krumpen, Thomas, Lampert, Astrid, Landing, William, Laurila, Tiia, Lawrence, Dale, Lonardi, Michael, Loose, Brice, Lüpkes, Christof, Maahn, Maximilian, Macke, Andreas, Maslowski, Wieslaw, Marsay, Christopher, Maturilli, Marion, Mech, Mario, Morris, Sara, Moser, Manuel, Nicolaus, Marcel, Ortega, Paul, Osborn, Jackson, Pätzold, Falk, Perovich, Donald, Petäjä, Tuukka, Pilz, Christian, Pirazzini, Roberta, Posman, Kevin, Powers, Heath, Pratt, Kerri, Preusser, Andreas, Qué Lé Ver, Lauriane, Radenz, Martin, Rabe, Benjamin, Rinke, Annette, Sachs, Torsten, Schulz, Alexander, Siebert, Holger, Silva, Tercio, Solomon, Amy, Sommerfeld, Anja, Spreen, Gunnar, Stephens, Mark, Stohl, Andreas, Svensson, Gunilla, Uin, Janek, Viegas, Juarez, Voigt, Christiane, von Der Gathen, Peter, Wehner, Birgit, Welker, Jeffrey, Wendisch, Manfred, Werner, Martin, Xie, Zhouqing, Yue, Fange, Jourdan, Olivier, Laboratoire de Météorologie Physique (LaMP), and Institut national des sciences de l'Univers (INSU - CNRS)-Université Clermont Auvergne [2017-2020] (UCA [2017-2020])-Centre National de la Recherche Scientifique (CNRS)

Subjects
[SDU.OCEAN]Sciences of the Universe [physics]/Ocean, Atmosphere, Arctic, Field campaign, Atmosphere, [SDU.OCEAN] Sciences of the Universe [physics]/Ocean, Atmosphere
Abstract

International audience; With the Arctic rapidly changing, the needs to observe, understand, and model the changes are essential. To support these needs, an annual cycle of observations of atmospheric properties, processes, and interactions were made while drifting with the sea ice across the central Arctic during the Multidisciplinary drifting Observatory for the Study of Arctic Climate (MOSAiC) expedition from October 2019 to September 2020. An international team designed and implemented the comprehensive program to document and characterize all aspects of the Arctic atmospheric system in unprecedented detail, using a variety of approaches, and across multiple scales. These measurements were coordinated with other observational teams to explore crosscutting and coupled interactions with the Arctic Ocean, sea ice, and ecosystem through a variety of physical and biogeochemical processes. This overview outlines the breadth and complexity of the atmospheric research program, which was organized into 4 subgroups: atmospheric state, clouds and precipitation, gases and aerosols, and energy budgets. Atmospheric variability over the annual cycle revealed important influences from a persistent large-scale winter circulation pattern, leading to some storms with pressure and winds that were outside the interquartile range of past conditions suggested by long-term reanalysis. Similarly, the MOSAiC location was warmer and wetter in summer than the reanalysis climatology, in part due to its close proximity to the sea ice edge.The comprehensiveness of the observational program for characterizing and analyzing atmospheric phenomena is demonstrated via a winter case study examining air mass transitions and a summer case study examining vertical atmospheric evolution. Overall, the MOSAiC atmospheric program successfully met its objectives and was the most comprehensive atmospheric measurement program to date conducted over the Arctic sea ice. The obtained data will support a broad range of coupled-system scientific research and provide an important foundation for advancing multiscale modeling capabilities in the Arctic.

Published
2022

8. Semantic Information Generation from Classification and Information Extraction

Author

de Morais Sampaio Silva, Tércio, de Freitas, Frederico Luiz Gonçalves, Cobra Teske, Rafael, Bittencourt, Guilherme, Kanade, Takeo, editor, Kittler, Josef, editor, Kleinberg, Jon M., editor, Mattern, Friedemann, editor, Mitchell, John C., editor, Naor, Moni, editor, Nierstrasz, Oscar, editor, Pandu Rangan, C., editor, Steffen, Bernhard, editor, Sudan, Madhu, editor, Terzopoulos, Demetri, editor, Tygar, Dough, editor, Vardi, Moshe Y., editor, Weikum, Gerhard, editor, Koch, Nora, editor, Fraternali, Piero, editor, and Wirsing, Martin, editor

Published
2004
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12. Raman‐scattering studies of pressure‐induced phase transitions in perovskite‐like acetamidninium manganese formate.

Author

Mączka, Mirosław, da Silva, Tercio Almeida, and Paraguassu, Waldeci

Subjects
*PEROVSKITE, *RAMAN scattering, *PHASE transitions, *FORMATES, *METAL-organic frameworks
Abstract

Abstract: We report high‐pressure Raman scattering studies of acetamidninium manganese formate, which show evidence for two pressure‐induced phase transitions between 0.7 and 1.4 GPa and above 5.3 GPa. The first transition is related to distortion of the manganese formate framework whereas the second one affects significantly the structure of the acetamidinium cation. Significant narrowing of the lattice bands suggests that the intermediate and high‐pressure phases are ordered. High‐pressure experiments also indicate different structures of the intermediate phases observed upon compression and decompression. However, release of pressure to ambient value leads to recovery of the initial ambient‐pressure phase. [ABSTRACT FROM AUTHOR]

Published
2018
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13. Effect of solvent, temperature and pressure on the stability of chiral and perovskite metal formate frameworks of [NH2NH3][M(HCOO)3] (M = Mn, Fe, Zn).

Author

Mączka, Mirosław, Pasińska, Katarzyna, Ptak, Maciej, Paraguassu, Waldeci, da Silva, Tercio Almeida, Sieradzki, Adam, and Pikul, Adam

Abstract

We report the synthesis, crystal structure, and thermal, Raman, infrared and magnetic properties of [NH2NH3][M(HCOO)3] (HyM) compounds (M = Mn, Zn, Fe). Our results show that synthesis from methanol solution leads to perovskite polymorphs while that from 1-methyl-2-pyrrolidinone or its mixture with methanol allows obtaining chiral polymorphs. Perovskite HyFe, chiral HyFe and chiral HyMn undergo phase transitions at 347, 336 and 296 K, respectively, with symmetry changes from Pnma to Pna21, P63 to P212121 and P63 to P21. X-ray diffraction and Raman studies show that the phase transitions are governed by dynamics of the hydrazinium ions. Low-temperature magnetic studies show that these compounds exhibit magnetic ordering below 9–12.5 K. Since the low-temperature structures of chiral HyMn and perovskite HyFe are polar, these compounds are possible multiferroic materials. We also report high-pressure Raman scattering studies of chiral and perovskite HyZn, which show much larger stiffness of the latter phase. These studies also show that the ambient pressure polar phases are stable up to at least 1.4 and 4.1 GPa for the chiral and perovskite phase, respectively. Between 1.4 and 2.0 GPa (for chiral HyZn) and 4.1 and 5.2 GPa (for perovskite HyZn) pressure-induced transitions are observed associated with changes in the zinc-formate framework. Strong broadening of Raman bands and the decrease in their number for the high-pressure phase of chiral HyZn suggest that this phase is disordered and has higher symmetry than the ambient pressure one. [ABSTRACT FROM AUTHOR]

Published
2016
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18. Raman and IR Studies of Pressure- and Temperature-Induced Phase Transitions in [(CH2)3NH2][Zn(HCOO)3].

Author

Mączka, Mirosław, da Silva, Tercio Almeida, Paraguassu, Waldeci, Ptak, Maciej, and Hermanowicz, Krzysztof

Subjects
*PHASE transitions, *RAMAN spectra, *AZETIDINE, *CATIONS, *BANDWIDTHS
Abstract

Temperature- and pressure-dependent studies of Raman and IR spectra have been performed on azetidinium zinc formate, [(CH2)3NH2][Zn(HCOO)3]. Vibrational spectra showed distinct anomalies in mode frequencies and bandwidths near 250 and 300 K, which were attributed to structural phase transitions associated with the gradual freezing of ring-puckering motions of the azetidinium cation. Pressure-dependent studies revealed a pressure-induced transition near 0.4 GPa. Raman spectra indicate that the structure of the room-temperature intermediate phase observed near 0.4 GPa is the same as the monoclinic structure observed at ambient pressure below 250 K. The second phase transition was found near 2.4 GPa. This transition has strong first-order character and is associated with strong distortion of both the zinc formate framework and azetidinium cations. The last phase transition was found near 7.0 GPa. This transition leads to lowering of the symmetry and further distortion of the zinc formate framework, whereas the azetidinium cation structure is weakly affected. [ABSTRACT FROM AUTHOR]

Published
2014
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20. Effect of solvent, temperature and pressure on the stability of chiral and perovskite metal formate frameworks of [NH 2 NH 3 ][M(HCOO) 3 ] (M = Mn, Fe, Zn).

Author

Mączka M, Pasińska K, Ptak M, Paraguassu W, da Silva TA, Sieradzki A, and Pikul A

Abstract

We report the synthesis, crystal structure, and thermal, Raman, infrared and magnetic properties of [NH 2 NH 3 ][M(HCOO) 3 ] (HyM) compounds (M = Mn, Zn, Fe). Our results show that synthesis from methanol solution leads to perovskite polymorphs while that from 1-methyl-2-pyrrolidinone or its mixture with methanol allows obtaining chiral polymorphs. Perovskite HyFe, chiral HyFe and chiral HyMn undergo phase transitions at 347, 336 and 296 K, respectively, with symmetry changes from Pnma to Pna2 1 , P6 3 to P2 1 2 1 2 1 and P6 3 to P2 1 . X-ray diffraction and Raman studies show that the phase transitions are governed by dynamics of the hydrazinium ions. Low-temperature magnetic studies show that these compounds exhibit magnetic ordering below 9-12.5 K. Since the low-temperature structures of chiral HyMn and perovskite HyFe are polar, these compounds are possible multiferroic materials. We also report high-pressure Raman scattering studies of chiral and perovskite HyZn, which show much larger stiffness of the latter phase. These studies also show that the ambient pressure polar phases are stable up to at least 1.4 and 4.1 GPa for the chiral and perovskite phase, respectively. Between 1.4 and 2.0 GPa (for chiral HyZn) and 4.1 and 5.2 GPa (for perovskite HyZn) pressure-induced transitions are observed associated with changes in the zinc-formate framework. Strong broadening of Raman bands and the decrease in their number for the high-pressure phase of chiral HyZn suggest that this phase is disordered and has higher symmetry than the ambient pressure one.

Published
2016
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